English
Related papers

Related papers: Thermopower of Single-Molecule Devices

200 papers

We employ the functional renormalization group to study the effects of phonon-assisted tunneling on the nonequilibrium steady-state transport through a single level molecular quantum dot coupled to electronic leads. Within the framework of…

Strongly Correlated Electrons · Physics 2018-12-18 A. Khedri , T. A. Costi , V. Meden

Molecular junctions are a versatile test bed for investigating thermoelectricity on the nanoscale1-10 and contribute to the design of new cost-effective environmentally-friendly organic thermoelectric materials11. It has been suggested that…

Organic molecules have recently gained attention as novel sources of single photons. We present a joint experiment--theory analysis of the temperature-dependent emission spectra, zero-phonon linewidth, and second-order correlation function…

A variational solution of the coupled electron-phonon Boltzmann equations is used to calculate the phonon drag contribution to the thermopower in a 1-D system. A simple formula is derived for the temperature dependence of the phonon drag in…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 V. W. Scarola , G. D. Mahan

Thermoelectric materials convert heat into electricity through thermally driven charge transport in solids, or vice versa for cooling. To be competitive with conventional energy-generation technologies, a thermoelectric material must…

We propose a passive single-photon detector based on the bipolar thermoelectric effect occurring in tunnel junctions between two different superconductors thanks to spontaneous electron-hole symmetry breaking. Our thermoelectric detector…

Mesoscale and Nanoscale Physics · Physics 2023-05-04 Federico Paolucci , Gaia Germanese , Alessandro Braggio , Francesco Giazotto

We use a many-body rate-equation approach to calculate the thermopower of a quantum dot in the presence of an exchange interaction. At temperatures much smaller than the single-particle level spacing, the known quantum jumps…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Gabriel Billings , A. Douglas Stone , Y. Alhassid

The thermoelectric power of nondegenerate Kane semiconductors with due regard for the electron and phonon heating, and their thermal and mutual drags is investigated. The electron spectrum is taken in the Kane two-band form. It is shown…

Statistical Mechanics · Physics 2009-11-07 M. M. Babaev , T. M. Gassym , M. Tas , M. Tomak

Using the conformal field theory partition function of a Coulomb-blockaded quantum dot, constructed by two quantum point contacts in a Laughlin quantum Hall bar, we derive the finite-temperature thermodynamic expression for the thermopower…

Strongly Correlated Electrons · Physics 2014-06-24 Lachezar S. Georgiev

The thermoelectric properties of single- and polycrystalline FeGa3 are systematically investigated over a wide temperature range. At low temperatures, below 20 K, previously not known pronounced peaks in the thermal conductivity (400-800 W…

The thermoelectric power S is studied within the one-dimensional Hubbard model using the linear response theory and the numerical exact-diagonalization method for small systems. While both the diagonal and off-diagonal dynamical correlation…

Strongly Correlated Electrons · Physics 2009-11-10 M. M. Zemljic , P. Prelovsek

We study thermoelectric properties of inhomogeneous nanogranular materials for weak tunneling conductance between the grains, g_t < 1. We calculate the thermopower and figure of merit taking into account the shift of the chemical potential…

Mesoscale and Nanoscale Physics · Physics 2009-10-16 A. Glatz , I. S. Beloborodov

The detailed characterization of non-trivial coherence properties of composite quantum systems of increasing size is an indispensable prerequisite for scalable quantum computation, as well as for understanding of nonequilibrium many-body…

We compute the transient dynamics of phonons in contact with high energy "hot" charge carriers in 12 polar and non-polar semiconductors, using a first-principles Boltzmann transport framework. For most materials, we find that the decay in…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Sridhar Sadasivam , Maria K. Y. Chan , Pierre Darancet

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin

The thermal transport across metal-insulator interface can be characterized by electron-phonon interaction through which an electron lead is coupled to a phonon lead if phonon-phonon coupling at the interface is very weak. We investigate…

Materials Science · Physics 2013-10-17 Lifa Zhang , Jing-Tao Lü , Jian-Sheng Wang , Baowen Li

We study theoretically phonon-assisted relaxation processes in a system consisting of one or two electrons confined in two vertically stacked self-assembled quantum dots. The calculation is based on a k.p approximation for single particle…

Mesoscale and Nanoscale Physics · Physics 2010-09-14 Krzysztof Gawarecki , Michał Pochwała , Anna Grodecka-Grad , Paweł Machnikowski

We report on inelastic electron tunneling spectroscopy measurements carried out on single molecules incorporated into a mechanically controllable break-junction of Au and Pt electrodes at low temperature. Here we establish a correlation…

Mesoscale and Nanoscale Physics · Physics 2010-11-16 Youngsang Kim , Hyunwook Song , Florian Strigl , Hans-Fridtjof Pernau , Takhee Lee , Elke Scheer

We study theoretically the length dependence of both conductance and thermopower in metal-molecule-metal junctions made up of dithiolated oligophenylenes contacted to gold electrodes. We find that while the conductance decays exponentially…

Mesoscale and Nanoscale Physics · Physics 2009-05-24 F. Pauly , J. K. Viljas , J. C. Cuevas

We investigate the time evolution of the thermopower in a vibrating quantum dot suddenly shifted into the Kondo regime via a gate voltage by adopting the time-dependent non-crossing approximation and linear response Onsager relations.…

Strongly Correlated Electrons · Physics 2015-06-05 Ali Goker , Berna Uyanik