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We have derived the local electric field inside graded metal-dielectric composite films with weak nonlinearity analytically, which further yields the effective linear dielectric constant and third-order nonlinear susceptibility of the…

Materials Science · Physics 2007-05-23 J. P. Huang , L. Dong , K. W. Yu

We have developed a nonlinear differential effective dipole approximation (NDEDA), in an attempt to investigate the effective linear and third-order nonlinear susceptibility of composite media in which graded spherical inclusions with weak…

Materials Science · Physics 2007-05-23 L. Gao , J. P. Huang , K. W. Yu

Recent years have seen increased interest to plasmonic enhancement of nonlinear optical effects, yet there remains an uncertainty of what are the limits of this enhancement. We present a simple and physically transparent theory of plasmonic…

Optics · Physics 2017-07-26 Jacob B Khurgin , Greg Sun

We generalize the Bergman-Milton spectral representation, originally derived for a two-component composite, to extract the spectral density function for the effective dielectric constant of a graded composite. This work has been motivated…

Soft Condensed Matter · Physics 2007-05-23 L. Dong , Mikko Karttunen , K. W. Yu

In this paper we analyze the effects of nonlocality on the optical properties of a system consisting of a thin metallic film separated from a graphene sheet by a hexagonal boron nitride (hBN) layer. We show that nonlocal effects in the…

Achieving efficient nonlinear optical frequency conversion in small volumes is key for future on-chip photonic devices that would provide a higher-speed alternative to modern electronics. However, the already intrinsically low conversion…

Mesoscale and Nanoscale Physics · Physics 2018-05-23 Vasily Kravtsov , Sultan AlMutairi , Ronald Ulbricht , A. Ryan Kutayiah , Alexey Belyanin , Markus B. Raschke

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

Mesoscale and Nanoscale Physics · Physics 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

Plasmonics enables deep-subwavelength concentration of light and has become important for fundamental studies as well as real-life applications. Two major existing platforms of plasmonics are metallic nanoparticles and metallic films.…

We reanalyze the seminal work by Dolan and Osheroff [Phys. Rev. Lett. $\textbf{43}$, 721 (1979)] which reported anomalous low-temperature conduction of high-resistivity thin-film metal strips. We argue that the observed logarithmic increase…

Mesoscale and Nanoscale Physics · Physics 2023-02-17 Juhn-Jong Lin , Zhi-Qing Li , Chih-Yuan Wu , Sheng-Shiuan Yeh

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Metallic nanostructures can support so-called plasma oscillations (plasmons). Plasmons allow for the concentration of the energy from light, down to sizes well below the conventional diffraction limit known from optics. Plasmonics thus…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Christian Frydendahl

We study the effective second-harmonic generation (SHG) susceptibility in graded metallic films by invoking the local field effects exactly, and further numerically demonstrate that the graded metallic films can serve as a novel optical…

Optics · Physics 2009-11-10 J. P. Huang , K. W. Yu

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

We demonstrate that the effective third-order nonlinear susceptibility of a graphene sheet can be enhanced by more than two orders of magnitude by patterning it into a graphene metasurface. In addition, in order to gain deeper physical…

Optics · Physics 2019-06-07 Jian Wei You , Nicolae C. Panoiu

Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an…

Nanophotonic devices offer an unprecedented ability to concentrate light into small volumes which can greatly increase nonlinear effects. However, traditional plasmonic materials suffer from low damage thresholds and are not compatible with…

The effective linear and third-order nonlinear optical properties of metallic colloidal crystal immersed in a graded-index host fluid are investigated theoretically. The local electric fields are extracted self-consistently based on the…

Materials Science · Physics 2007-05-23 J. J. Xiao , K. W. Yu

Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…

We introduce an effect of metallization of dielectric nanofilms by strong, adiabatically varying electric fields. The metallization causes optical properties of a dielectric film to become similar to those of a plasmonic metal (strong…

Mesoscale and Nanoscale Physics · Physics 2010-07-15 Maxim Durach , Anastasia Rusina , Matthias F. Kling , Mark I. Stockman

Regular arrays of metal nanoparticles on metal films have tuneable optical resonances that can be applied for surface enhanced Raman scattering or biosensing. With the aim of developing more surface selective geometries we investigate…

Mesoscale and Nanoscale Physics · Physics 2012-09-13 Andreas Hohenau , Joachim R. Krenn
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