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We investigate the statistical mechanics of an inhomogeneous Coulomb fluid composed of charged particles with static polarizability. We derive the weak- and the strong-coupling approximations and evaluate the partition function in a planar…

Soft Condensed Matter · Physics 2013-04-22 Vincent Démery , David S. Dean , Rudolf Podgornik

Inspired by recent experiments and simulations on pattern formation in biomolecules by optical tweezers, a theoretical description based on reference interaction site model (RISM) integral equation method is developed to calculate the…

Soft Condensed Matter · Physics 2016-02-17 Sandipan Dutta , Y. S. Jho

A variational approach is considered to calculate the free energy and the conformational properties of a polyelectrolyte chain in $d$ dimensions. We consider in detail the case of pure Coulombic interactions between the monomers, when…

Soft Condensed Matter · Physics 2007-05-23 G. Migliorini , V. G. Rostiashvili , T. A. Vilgis

Charge-stabilized colloidal suspensions can be conveniently described by formally reducing the macroion-microion mixture to an equivalent one-component system of pseudo-particles. Within this scheme, the utility of a linear response…

Soft Condensed Matter · Physics 2009-10-31 A. R. Denton

We consider the complexation of highly charged semiflexible polyelectrolytes with oppositely charged macroions. On the basis of scaling arguments we discuss how the resulting complexes depend on the persistence length of the…

Soft Condensed Matter · Physics 2009-11-07 H. Schiessel , R. F. Bruinsma , W. M. Gelbart

We simulate model systems of charged spherical particles in their counterion solution and measure the thermodynamic pressure and the pair distribution function from which we derive effective potentials of mean force. For a system with only…

Soft Condensed Matter · Physics 2007-05-23 Niels Gronbech-Jensen , Keith M Beardmore , Philip Pincus

Ionic microgel particles are intriguing systems in which the properties of thermo-responsive polymeric colloids are enriched by the presence of charged groups. In order to rationalize their properties and predict the behaviour of microgel…

Soft Condensed Matter · Physics 2021-01-28 G. Del Monte , F. Camerin , A. Ninarello , N. Gnan , L. Rovigatti , E. Zaccarelli

An analytical description of polymer melts and their mixtures as liquids of interacting soft colloidal particles is obtained from liquid-state theory. The derived center-of-mass pair correlation functions with no adjustable parameters…

Soft Condensed Matter · Physics 2009-11-10 G. Yatsenko , E. J. Sambriski , M. A. Nemirovskaya , M. Guenza

We present a theory which allows us to calculate the interaction potential between charge-regulated metal nanoparticles inside an acid-electrolyte solution. The approach is based on the recently introduced model of charge regulation which…

Soft Condensed Matter · Physics 2020-12-11 Amin Bakhshandeh , Alexandre P. dos Santos , Yan Levin

We explore the mechanical response of a single polyelectrolyte chain under tension in good and poor solvents using a combination of simulation and theory. In poor solvents, where the equilibrium state of the chain is a collapsed globule, we…

Soft Condensed Matter · Physics 2009-05-29 Ajay S. Panwar , Mark A. Kelly , Buddhapriya Chakrabarti , M. Muthukumar

The collapse of flexible polyelectrolytes in a solution of multivalent counterions is studied by means of a two state model. The states correspond to rod-like and spherically collapsed conformations respectively. We focus on the very dilute…

Soft Condensed Matter · Physics 2009-10-31 Francisco J. Solis , Monica Olvera de la Cruz

We explore the role of electron correlation in quasi one dimensional quantum wires as the range of the interaction potential is changed and their thickness is varied by performing exact quantum Monte Carlo simulations at various electronic…

Strongly Correlated Electrons · Physics 2009-11-13 L. Shulenburger , M. Casula , G. Senatore , R. M. Martin

We study a simple model of conducting polymers in which a single electron propagates through a randomly tangled chain. The model has the geometry of a small-world network, with a small density $p$ of crossings of the chain acting as…

Disordered Systems and Neural Networks · Physics 2007-05-23 Jorge Quintanilla , Vivaldo L. Campo

In this thesis we study the lateral electrostatic interaction between a pair of non-identical, moderately charged colloidal particles trapped at an electrolyte interface in the limit of short inter-particle separations. Using a simplified…

Soft Condensed Matter · Physics 2017-10-17 Timo Schmetzer

We discuss the reliability of integral-equation methods based on several commonly used closure relations in determining the phase diagram of coarse-grained models of soft-matter systems characterized by mutually interacting soft and…

Soft Condensed Matter · Physics 2015-10-28 Roberto Menichetti , Andrea Pelissetto , Giuseppe D'Adamo , Carlo Pierleoni

Representing polyether-salt systems by chains of interacting coordination shells, defined by the cation and by its nearest ligands, we derive the interaction potential between closest shells -- the inter-shells potential -- in terms of…

chem-ph · Physics 2009-10-28 L. D. Carlos , A. L. L. Videira

We investigate the phenomenon of counterion condensation in a solution of highly charged rigid polyelectrolytes within the cell model. A method is proposed which -- based on the charge distribution function -- identifies both the fraction…

Soft Condensed Matter · Physics 2009-10-31 Markus Deserno , Christian Holm , Sylvio May

We use the recently developed soft-potential-enhanced Poisson-Boltzmann (SPB) theory to study the interaction between two parallel polyelectrolytes (PEs) in monovalent ionic solutions in the weak-coupling regime. The SPB theory is fitted to…

Soft Condensed Matter · Physics 2022-09-28 Xiang Yang , Alberto Scacchi , Hossein Vahid , Maria Sammalkorpi , Tapio Ala-Nissila

We develop a first-principle equation of state of salt-free polyelectrolyte solution in the limit of infinitely long flexible polymer chains in the framework of a field-theoretical formalism beyond the linear Debye-Hueckel theory and…

Soft Condensed Matter · Physics 2015-08-04 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , E. A. Nogovitsyn , M. G. Kiselev

The behavior of polyelectrolytes and polyampholytes in semi-dilute solutions is investigated theoretically. Various statistical charge distributions along the polyelectrolyte chains are considered: smeared, annealed, permuted and quenched.…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland
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