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The Dzyaloshinski-Moriya interaction partially lifts the magnetic frustration of the spin-1/2 oxide SrCu2(BO3)2. It explains the fine structure of the excited triplet state and its unusual magnetic field dependence, as observed in previous…

Strongly Correlated Electrons · Physics 2009-11-07 O. Cepas , K. Kakurai , L. P. Regnault , T. Ziman , J. P. Boucher , N. Aso , M. Nishi , H. Kageyama , Y. Ueda

The orthogonal dimer structure in the SrCu2(BO3)2 spin-1/2 magnet provides a realization of the Shastry-Sutherland model. Using a dimer-product variational wave function, we map out the phase diagram of the Shastry-Sutherland model…

Strongly Correlated Electrons · Physics 2015-03-17 Judit Romhanyi , Keisuke Totsuka , Karlo Penc

Various spin gap excitations have been observed in the two-dimensional dimer system SrCu_2(BO_3)_2 by means of submillimeter wave ESR. The zero-field energy gap of the lowest spin gap excitation shows a splitting into two triplet modes and…

Strongly Correlated Electrons · Physics 2009-10-31 H Nojiri , H. Kageyama , Kenzo Onizuka , Y. Ueda , M. Motokawa

X-band ESR measurements on a single crystal of the highly frustrated SrCu$_2$(BO$_3$)$_2$ system are shown to provide an essential inspection of the magnetic anisotropy present in this compound. The very broad absorption lines seem to be…

Strongly Correlated Electrons · Physics 2007-05-23 A. Zorko , D. Arčon , H. Kageyama , A. Lappas

We report magnetization and heat capacity measurements of single crystal samples of the spin gap compound Sr$_2$Cu(BO$_3$)$_2$. Low-field data show that the material has a singlet ground state comprising dimers with intradimer coupling J =…

Strongly Correlated Electrons · Physics 2011-12-08 Suchitra E. Sebastian , D. Yin , P. Tanedo , G. A. Jorge , N. Harrison , M. Jaime , Y. Mozharivskyj , G. Miller , J. Krzystek , S. A. Zvyagin , I. R. Fisher

Anisotropic spin-spin interactions of the symmetry described by Dzyaloshinsky and Moriya are generally considered weak, as they depend on the spin-orbit couplings. In frustrated spin systems with singlet ground states they can, however,…

Strongly Correlated Electrons · Physics 2009-11-07 O. Cepas , T. Sakai , T. Ziman

Anisotropic spin-spin interactions of Dzyaloshinsky and Moriya symmetry are generally considered weak, as they depend on the spin-orbit couplings. In spin systems with gapped ground states they can, however, have rather strong effects. We…

Strongly Correlated Electrons · Physics 2007-05-23 O. Cepas , T. Ziman

We present a high-field magnetization study of the $S$ = 1/2 antiferromagnetic Heisenberg chain [PM Cu(NO$_3$)$_2$(H$_2$O)$_2$]$_n$. For this material, as result of the Dzyaloshinskii-Moriya interaction and a staggered $g$ tensor, the…

High resolution neutron scattering measurements on a single crystal of SrCu(2-x)Mgx(BO3)2 with x=0.05 reveal the presence of new spin excitations within the gap of this quasi-two dimensional, singlet ground state system. Application of a…

Strongly Correlated Electrons · Physics 2009-11-11 S. Haravifard , S. R. Dunsiger , S. El Shawish , B. D. Gaulin , H. A. Dabkowska , M. T. F. Telling , J. Bonca

Field-dependent specific heat and neutron scattering measurements were used to explore the antiferromagnetic S=1/2 chain compound CuCl2 * 2((CD3)2SO). At zero field the system acquires magnetic long-range order below TN=0.93K with an…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Chen , M. B. Stone , M. Kenzelmann , C. D. Batista , D. H. Reich , C. Broholm

We achieve a comprehensive understanding of the magnetic excitations observed by electric spin resonance and far-infrared spectroscopy in a frustrated spin gap system ${\rm SrCu_2(BO_3)_2}$ by considering the effects of magnetoelectric…

Strongly Correlated Electrons · Physics 2023-04-24 Shin Miyahara

The study of interacting spin systems is of fundamental importance for modern condensed matter physics. On frustrated lattices, magnetic exchange interactions cannot be simultaneously satisfied, and often give rise to competing exotic…

We have investigated the physical effects of the Dzyaloshinskii-Moriya (DM) interaction in copper benzoate. In the low field limit, the spin gap is found to vary as $H^{2/3}\ln ^{1/6}(J/\mu_BH_s)$ ($H_s$: an effective staggered field…

Strongly Correlated Electrons · Physics 2009-11-07 J. Z. Zhao , X. Q. Wang , T. Xiang , Z. B. Su , L. Yu

Magnetic excitations in the isostructural spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 are probed by means of high-field electron spin resonance at sub-terahertz frequencies. Three types of magnetic modes were observed. One mode is gapless and…

We perform a low temperature Raman scattering study of phononic and collective spin excitations in the orthogonal dimers compound SrCu_2(BO_3)_2, focussing on the symmetry and the effects of external fields on the magnetic modes. The zero…

Strongly Correlated Electrons · Physics 2009-11-11 A. Gozar , B. S. Dennis , H. Kageyama , G. Blumberg

We investigated magnetic and thermodynamic properties of $S$ = 1/2 quasi-one-dimensional antiferromagnet KCuMoO$_4$(OH) through single crystalline magnetization and heat capacity measurements. At zero field, it behaves as a uniform $S$ =…

Strongly Correlated Electrons · Physics 2017-11-27 Kazuhiro Nawa , Oleg Janson , Zenji Hiroi

The ground state of the stacked triangular antiferromagnet CsFeBr$_3$ is a spin singlet due to the large single ion anisotropy $D(S^z)^2$. The field-induced magnetic ordering in this compound was investigated by the magnetic susceptibility,…

Strongly Correlated Electrons · Physics 2009-11-07 Y. Tanaka , H. Tanaka , T. Ono , A. Oosawa , K. Morishita , K. Iio , T. Kato , H. Aruga Katori , M. Bartashevich , T. Goto

We apply degenerate perturbation theory to investigate the effects of magnetic anisotropy in the magnetic molecule V15. Magnetic anisotropy is introduced via Dzyaloshinskii-Moriya (DM) interaction in the full Hilbert space of the system.…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 N. P. Konstantinidis , D. Coffey

By using bulk magnetization, electron spin resonance (ESR), heat capacity, and neutron scattering techniques, we characterize the thermodynamic and quantum phase diagrams of Ba$_3$Cr$_2$O$_8$. Our ESR measurements indicate that the low…

Strongly Correlated Electrons · Physics 2015-05-13 M. Kofu , H. Ueda , H. Nojiri , Y. Oshima , T. Zenmoto , K. Rule , S. Gerischer , B. Lake , C. D. Batista , Y. Ueda , S. -H. Lee

We study the effects of external magnetic field on the properties of an ordered Heisenberg antiferromagnet with the Dzyaloshinskii-Moriya (DM) interaction. Using the spin-wave theory quantum correction to the energy, on-site magnetization,…

Strongly Correlated Electrons · Physics 2007-05-23 A. L. Chernyshev
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