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A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector,…

We investigate Perfect Absorption (PA) of radiation, in which incoming energy is entirely dissipated, in a system consisting of molecular spin centers coherently coupled to a planar microwave resonator operated at milliKelvin temperature…

We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting…

Presented are magnetization measurements on a crystal of Cr7Ni antiferromagnetic rings. Irradiation with microwaves at frequencies between 1 and 10 GHz leads to observation of very narrow resonant photon absorption lines which are mainly…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , D. Mailly , G. A. Timco , R. E. P. Winpenny

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

We report the development of the frequency-modulation (FM) method for measuring electron spin resonance (ESR) absorption in the 210-420 GHz frequency range. We demonstrate that using a high-frequency ESR spectrometer without resonating…

Strongly Correlated Electrons · Physics 2010-07-14 Balint Nafradi , Richard Gaal , Titusz Feher , Laszlo Forro

We have developed a novel dc SQUID system with a micro-coil input circuit to act as a local probe of quantum matter and nanosystems. The planar niobium micro-coil pickup loop is located remotely from the SQUID, coupled through a…

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

Quantum Physics · Physics 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

We present pulsed electrically detected magnetic resonance (EDMR) measurements at low magnetic fields using posphorus-doped silicon with natural isotope composition as a model system. Our measurements show that pulsed EDMR experiments, well…

Materials Science · Physics 2015-06-23 L. Dreher , F. Hoehne , H. Morishita , H. Huebl , M. Stutzmann , K. M. Itoh , M. S. Brandt

We combine top-down and bottom-up nanolithography to optimize the coupling of small molecular spin ensembles to $1.4$ GHz on-chip superconducting resonators. Nanoscopic constrictions, fabricated with a focused ion beam at the central…

Light-matter interaction in optomechanical systems is the foundation for ultra-sensitive detection schemes [1,2] as well as the generation of phononic and photonic quantum states [3-10]. Electromechanical systems realize this optomechanical…

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap…

Mesoscale and Nanoscale Physics · Physics 2009-08-28 N. Groll , S. Bertaina , M. Pati , N. S. Dalal , I. Chiorescu

We emulate renormalization group models, such as the Spin-Boson Hamiltonian or the anisotropic Kondo model, from a quantum optics perspective by considering a superconducting device. The infra-red confinement involves photon excitations of…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Karyn Le Hur

Certain species of living creatures are known to orientate themselves in the geomagnetic field. Given the small magnitude of approximately 48 {\mu}T, the underlying quantum mechanical phenomena are expected to exhibit coherence times…

Dilute frozen solutions of the single molecule magnet Ni$_4$ (S=4) have been studied using high frequency D-band (130 GHz) EPR. Despite the random orientation of the molecules, well defined EPR absorption peaks are observed, due to the…

Other Condensed Matter · Physics 2009-11-13 G. de Loubens , A. D. Kent , V. Krymov , G. J . Gerfen , C. C. Beedle , D. N. Hendrickson

We show that the probability of the collision-induced absorption of non-resonant microwave photons by a gas of ultracold molecules is dramatically enhanced near a Feshbach scattering resonance. This can be used for detecting Feshbach…

Atomic Physics · Physics 2010-10-28 Sergey V. Alyabyshev , Roman V. Krems

In this study, novel use of the electromagnetic field profile of a localized spoof surface plasmonic mode to detect electron spin resonance is being reported. The mode is supported on a resonator with a complementary metallic spiral…

Applied Physics · Physics 2021-05-04 Subhadip Roy , Anuvab Nandi , Pronoy Das , Chiranjib Mitra

The electron spin resonance (ESR) of nanoscale molecular magnet ${\rm V}_{15}$ is studied. Since the Hamiltonian of ${\rm V}_{15}$ has a large Hilbert space and numerical calculations of the ESR signal evaluating the Kubo formula with exact…

Statistical Mechanics · Physics 2015-06-24 Manabu Machida , Toshiaki Iitaka , Seiji Miyashita

Magnetic resonance with ensembles of electron spins is nowadays performed in frequency ranges up to 240 GHz and in corresponding magnetic fields of up to 10 T. However, experiments with single electron and nuclear spins so far only reach…

We report on a scanned superconducting quantum interference device (SQUID) microscope operating in a cryogen-free cryostat, with the capability of up to forty RF connections with 20 GHz bandwidth to a device under test. The system utilizes…

Superconductivity · Physics 2025-09-10 Ian W. Haygood , Bochao Xu , John Biesecker , Michael L. Schneider
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