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Helium atoms are strongly attracted to the interstitial channels within a bundle of carbon nanotubes. The strong corrugation of the axial potential within a channel can produce a lattice gas system where the weak mutual attraction between…

Statistical Mechanics · Physics 2009-10-31 M. W. Cole , V. H. Crespi , G. Stan , J. M. Hartman , S. Moroni , M. Boninsegni

We calculate the energy-band structure of a He atom trapped within the interstitial channel between close-packed nanotubes within a bundle and its influence on the specific heat of the adsorbed gas. A robust prediction of our calculations…

Statistical Mechanics · Physics 2009-11-07 A. Siber , H. Buljan

Helium atoms or hydrogen molecules are believed to be strongly bound within the interstitial channels (between three carbon nanotubes) within a bundle of many nanotubes. The effects on adsorption of a nonuniform distribution of tubes are…

Materials Science · Physics 2009-11-10 F. Ancilotto , M. M. Calbi , S. M. Gatica , M. W. Cole

We study the low temperature phase behavior of hydrogen within a bundle of carbon nanotubes. Because the carbon environment weakens the attraction between molecules within the same interstitial channel (IC), the ground state of the…

Materials Science · Physics 2007-05-23 M. K. Kostov , J. C. Lewis , M. W. Cole

We present the first low-temperature thermodynamic investigation of the controlled physisorption of He$^{4}$ gas in carbon single-wall nanotube (SWNT) samples. The vibrational specific heat measured between 100 mK and 6 K demonstrates an…

Materials Science · Physics 2009-11-10 J. C. Lasjaunias , K. Biljakovic , J. L. Sauvajol , P. Monceau

We evaluate the effects of heterogeneity on the density of states of H$_2$ molecules inside interstitial channels within bundles of carbon nanotubes. As temperature (T) falls, the density increases within those tubes having the greatest…

Soft Condensed Matter · Physics 2007-05-23 Francesco Ancilotto , M. Mercedes Calbi , Silvina M. Gatica , Milton W. Cole

An analogue to Raoult's law is determined for the case of a 3He-4He mixture adsorbed in the interstitial channels of a bundle of carbon nanotubes. Unlike the case of He mixtures in other environments, the ratio of the partial pressures of…

Statistical Mechanics · Physics 2009-10-31 George Stan , Jacob M. Hartman , Vincent H. Crespi , Silvina M. Gatica , Milton W. Cole

We explore the properties of atoms confined to the interstitial regions within a carbon nanotube bundle. We find that He and Ne atoms are of ideal size for physisorption interactions, so that their binding energies are much greater there…

Statistical Mechanics · Physics 2007-05-23 G. Stan , V. H. Crespi , M. W. Cole , M. Boninsegni

An overview is presented of the various phases predicted to occur when gases are absorbed within a bundle of carbon nanotubes. The behavior may be characterized by an effective dimensionality, which depends on the species and the…

Soft Condensed Matter · Physics 2007-05-23 M. Mercedes Calbi , Milton W. Cole , Silvina M. Gatica , Mary J. Bojan , George Stan

The heat capacity of a small amount of $^3$He atoms dissolved in submonolayer $^4$He film has been measured. The measured heat capacity is finite and suggests that $^3$He atoms are mobile at an areal density regime higher than that of the…

Other Condensed Matter · Physics 2022-08-16 Masashi Morishita

The radial thermal expansion {\alpha}r of bundles of single-walled carbon nanotubes saturated with 3He up to the molar concentration 9.4% has been investigated in the temperature interval 2.1-9.5 K by high-sensitivity capacitance…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. V. Dolbin , V. B. Esel'son , V. G. Gavrilko , V. G. Manzhelii , N. A. Vinnikov , S. N. Popov , B. Sudqvist

We explore the equations of state and other properties of various quantum fluids (3He, 4He, their mixtures, and H_2) confined within individual carbon nanotubes. Above a threshold number of particles, N_a, the fluid density near the axis…

Statistical Mechanics · Physics 2007-05-23 S. M. Gatica , G. Stan , M. M. Calbi , J. K. Johnson , M. W. Cole

Diffusion Monte Carlo calculations on the adsorption of $^4$He in open-ended single walled (10,10) nanotubes are presented. We have found a first order phase transition separating a low density liquid phase in which all $^4$He atoms are…

Materials Science · Physics 2009-11-13 M. C. Gordillo , J. Boronat , J. Casulleras

Low-temperature thermal conductivity and thermopower of multiwalled carbon nanotubes considered within a bundle of nanotubes are calculated taking into account multiple scattering of electrons on the atoms of impurities (like single carbon…

High Energy Physics - Theory · Physics 2010-12-07 V. Egorushkin , N. Melnikova , A. Ponomarev , A. Reshetnyak

When the electron density of highly crystalline thin films is tuned by chemical doping or ionic liq- uid gating, interesting effects appear including unconventional superconductivity, sizeable spin-orbit coupling, competition with…

Mesoscale and Nanoscale Physics · Physics 2018-12-19 G. Dezi , N. Scopigno , S. Caprara , M. Grilli

We report results of diffusion Monte Carlo calculations for both $^4$He absorbed in a narrow single walled carbon nanotube (R = 3.42 \AA) and strictly one dimensional $^4$He. Inside the tube, the binding energy of liquid $^4$He is…

Statistical Mechanics · Physics 2009-10-31 M. C. Gordillo , J. Boronat , J. Casulleras

Low dimensional fermionic quantum systems are exceptionally interesting because they reveal distinctive physical phenomena, including among others, topologically protected excitations, edge states, frustration, and fractionalization.…

Helium films show various quantum phases that undergo quantum phase transitions by changing coverage n. We found anomalous elastic phenomena in bosonic 4He and fermionic 3He films adsorbed on a glass substrate. The films stiffen under AC…

Strongly Correlated Electrons · Physics 2018-12-12 T. Makiuchi , M. Tagai , Y. Nago , D. Takahashi , K. Shirahama

Intrinsic discrete nature in thermodynamic properties of Fermi gases appears under strongly confined and degenerate conditions. For a rectangular confinement domain, thermodynamic properties of an ideal Fermi gas are expressed in their…

Quantum Gases · Physics 2016-02-24 Alhun Aydin , Altug Sisman

I calculate the quantum states for He atom in the potential of an external groove of the single wall carbon nanotube bundle. The calculated ground state energy is found to be in fair agreement with the experimental estimate which suggests…

Statistical Mechanics · Physics 2009-11-07 Antonio Siber
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