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We have characterized the dynamics of the polar nanoregions in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) through high-resolution neutron backscattering and spin-echo measurements of the diffuse scattering cross section. We find that the diffuse…

Materials Science · Physics 2015-05-18 C. Stock , L. Van Eijck , P. Fouquet , M. Maccarini , P. M. Gehring , Guangyong Xu , H. Luo , X. Zhao , J. -F. Li , D. Viehland

We report lattice dynamical measurements, made using neutron inelastic scattering methods, of the relaxor perovskite PbMg1/3Nb2/3O3 (PMN) at momentum transfers near the edge of the Brillouin zone. Unusual"columns" of phonon scattering that…

Materials Science · Physics 2015-05-13 I. P. Swainson , C. Stock , P. M. Gehring , Guangyong Xu , K. Hirota , Y. Qiu , H. Luo , X. Zhao , J. -F. Li , D. Viehland

The results of diffuse neutron scattering experiment on PbMg1/3Nb2/3O3 single crystal above the Burns temperature are reported. It is shown that the high temperature elastic diffuse component is highly anisotropic in low-symmetry Brillouin…

Materials Science · Physics 2015-03-17 R. G. Burkovsky , S. B. Vakhrushev , K. Hirota , M. Matsuura

The low-energy part of vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ relaxor ferroelectric was studied by inelastic neutron scattering. We observed the coexistence of a resolution-limited central peak with strong quasielastic…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , S. G. Lushnikov , B. Roessli

Local symmetry breaking in complex materials is emerging as an important contributor to materials properties but is inherently difficult to study. Here we follow up an earlier structural observation of such a local symmetry broken phase in…

Diffuse scattering around the (110) reciprocal lattice point has been investigated by elastic neutron scattering in the paraelectric and the relaxor phases of the disordered complex perovskite crystal-Pb(Zn1/3Nb2/3)O3(PZN). The appearance…

Materials Science · Physics 2009-11-07 D. La-Orauttapong , J. Toulouse , J. L. Robertson , Z. -G. Ye

The low-energy part of the vibration spectrum in KNbO$_3$ was studied by cold neutron inelastic scattering in the cubic phase. In addition to acoustic phonons, we observe strong diffuse scattering, which consists of two components. The…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. G. Lushnikov , A. Choubey , P. Gunter

We show that the neutron diffuse scattering in relaxor ferroelectric (1-x)PbZn$_{1/3}$Nb$_{2/3}$O$_{3}$ - x PbTiO$_{3}$ (x=0.07) consists of two components. The first component is strictly elastic but extended in q-space and grows below 600…

Materials Science · Physics 2019-08-12 G. -M. Rotaru , S. N. Gvasaliya , B. Roessli , S. Kojima , S. G. Lushnikov , P. Günter

We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with…

Materials Science · Physics 2009-11-10 Guangyong Xu , G. Shirane , J. R. D. Copley , P. M. Gehring

High energy resolution neutron spin-echo spectroscopy has been used to measure intrinsic width of diffuse scattering discovered earlier in relaxor ferroelectric crystals. The anisotropic and transverse components of the scattering have been…

Materials Science · Physics 2017-09-13 Sergey Vakhrushev , Alexandre Ivanov , Jiri Kulda

Neutron scattering and ultrasonic methods have been used to study the lattice dynamics of two single crystals of Ni-Mn-In Heusler alloys close to Ni$_{50}$Mn$_{34}$In$_{16}$ magnetic superelastic composition. The paper reports the…

We present temperature dependent inelastic neutron scattering measurments, accompanied byab-initio calculations of phonon spectra and elastic properties as a function of pressure to understand anharmonicity of phonons and to study the…

Cold neutron scattering experiments have been performed to explore the energy, temperature, and wave-vector dependence of the diffuse scattering and the transverse acoustic (TA) phonons in the relaxor PbMg(1/3)Nb(2/3)O3. We have observed a…

Materials Science · Physics 2009-11-10 H. Hiraka , S. -H. Lee , P. M. Gehring , Guangyong Xu , G. Shirane

We report the results of inelastic neutron scattering experiments performed with triple-axis spectrometers to investigate the low-temperature collective dynamics in the ordered phase of uranium dioxide. The results are in excellent…

Strongly Correlated Electrons · Physics 2013-12-19 R. Caciuffo , P. Santini , S. Carretta , G. Amoretti , A. Hiess , N. Magnani , L. -P. Regnault , G. H. Lander

The impact of dispersion relations, anisotropy, and Brillouin zone structure on intrinsic phonon scattering rates has been assessed within the harmonic approximation-perturbation theory approach for lattice dynamics. Anisotropic nonlinear…

Materials Science · Physics 2022-06-15 Ahmed Hamed , Anter El-Azab

Single crystals of a ternary relaxor ferroelectric system, 0.29Pb(In1/2Nb1/2)O3-0.45Pb(Mg1/3Nb2/3)O3-0.26PbTiO3, have been studied using triple-axis based elastic and inelastic neutron scattering. Elastic diffuse scattering confirms the…

Materials Science · Physics 2022-08-10 Qian Li , Sergey Danilkin , Guochu Deng , Jian Wang , Zhengrong Li. Ray L. Withers , Zhuo Xu , Yun Liu

The lattice dynamics of the metallic tin {\beta} and {\gamma} polymorphs has been studied by a combination of diffuse scattering, inelastic x-ray scattering and density functional perturbation theory. The non-symmorphic space group of the…

The lattice dynamics of coesite has been studied by a combination of diffuse x-ray scattering, inelastic x-ray scattering and an ab initio lattice dynamics calculation. The combined technique gives access to the full lattice dynamics in…

The phonon renormalization across the semiconductor-to-metal crossover in FeSi is investigated by inelastic neutron scattering combined with \textit{ab-initio} lattice dynamical calculations. A significant part of reciprocal space with a…

Materials Science · Physics 2022-05-03 Nazir Khan , Sven Krannich , Dominic Boll , Rolf Heid , Daniel Lamago , A. Ivanov , David Voneshen , Frank Weber

We report neutron inelastic scattering experiments on single crystal PbMg$_{1/3}$Nb$_{2/3}$O$_{3}$ doped with 32\% PbTiO$_{3}$, a relaxor ferroelectric that lies close to the morphotropic phase boundary. When cooled under an electric field…

Materials Science · Physics 2016-01-06 John A. Schneeloch , Zhijun Xu , B. Winn , C. Stock , P. M. Gehring , R. J. Birgeneau , Guangyong Xu
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