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Here we present theoretical studies of the effect of vibronic coupling on nonlinear transport characteristics (current-voltage and conductance-voltage) in molecular electronic devices. Considered device is composed of molecular quantum dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

Vibronic coupling effects usually manifest themselves in molecules and crystals rather than in an unbound atoms. We theoretically demonstrate the existence of vibronic states in a moving two-level atom exposed to a strong electromagnetic…

Quantum Physics · Physics 2020-10-28 Andrei Ivanov , Evgeniy Perlin

We consider the nonequilibrium quantum vibrations of a molecule clamped between two macroscopic leads in a current-carrying state at finite voltages. Our approach is based on the nonequilibrium Green function technique and the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 D. A. Ryndyk , M. Hartung , G. Cuniberti

We describe how to treat the interaction of travelling electrons with localised vibrational modes in nanojunctions. We present a multichannel scattering technique which can be applied to calculate the transport properties for realistic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 H. Ness , A. J. Fisher

We present a microscopic model, describing current-driven switching in metallic atomic-size contacts. Applying a high current through an atomic-size contact, creates a strong electronic nonequilibrium that excites vibrational modes by…

Mesoscale and Nanoscale Physics · Physics 2024-05-03 Markus Ring , Fabian Pauly , Peter Nielaba , Elke Scheer

Recent progress in the field of molecular electronics has revealed the fundamental importance of the coupling between the electronic degrees of freedom and specific vibrational modes. Considering the examples of a molecular dimer and a…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We investigate the distribution of the electron density and the potential in a quantum wire coupled to reservoirs, treating this structure as a unified quantum system and taking into account the Coulomb interaction of electrons. The…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 V. A. Sablikov , S. V. Polyakov , M. Buttiker

We theoretically analyze correlation effects on the transport properties of a benzene molecule that are mediated by interactions between the motion of the nuclei and the transmitted charge. We focus on the lowest-lying molecular vibrational…

Mesoscale and Nanoscale Physics · Physics 2013-08-09 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

The dynamics of an electron in a strong laser field can be significantly altered by radiation reaction. This usually results in a strongly damped motion, with the electron losing a large fraction of its initial energy. Here we show that the…

Plasma Physics · Physics 2014-02-12 Matteo Tamburini , Christoph H. Keitel , Antonino Di Piazza

We present a technique to calculate the transport properties through one-dimensional models of molecular wires. The calculations include inelastic electron scattering due to electron-lattice interaction. The coupling between the electron…

Condensed Matter · Physics 2009-10-31 H. Ness , S. A. Shevlin , A. J. Fisher

We provide analytical results for the perturbative correction to the current-voltage relation through a vibrating molecule for weak electron-phonon coupling. The nonlinear conductance exhibits a step-like feature at $eV=\hbar \omega_0$,…

Mesoscale and Nanoscale Physics · Physics 2008-03-14 R. Egger , A. O. Gogolin

Molecular spintronics is made possible by the coupling between electronic configuration and magnetic po- larization of the molecules. For control and application of the individual molecular states it is necessary to both read and write…

Mesoscale and Nanoscale Physics · Physics 2016-04-27 T. Saygun , J. Bylin , H. Hammar , J. Fransson

A molecular wire coupled to two electron reservoirs is investigated within a tight-binding approach including spin and Coulomb interaction. Under the assumption of weak coupling to the electron reservoirs a quantum master equation can be…

Mesoscale and Nanoscale Physics · Physics 2007-08-28 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

Mesoscale and Nanoscale Physics · Physics 2011-03-15 R. Härtle , M. Thoss

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

We investigate the influence of external laser excitations on the average current through bridged molecules. For the computation of the current, we use a numerically very efficient formalism that is based on the Floquet solutions of the…

Chemical Physics · Physics 2007-05-23 Sigmund Kohler , Jörg Lehmann , Sébastien Camalet , Peter Hänggi

We explore theoretically how the coupling to cavity vacuum fields affects the electron transport in quantum conductors due to the counter-rotating-wave terms of light-matter interaction. We determine the quantum conductance in terms of the…

Mesoscale and Nanoscale Physics · Physics 2023-01-31 Geva Arwas , Cristiano Ciuti

The physics of vibrational kinetics in nitrogen-containing plasma produced by collisions with electrons is studied on the basis of recently derived cross sections and rate coefficients for the resonant vibrational-excitation by…

Chemical Physics · Physics 2013-04-17 V. Laporta , D. Bruno

Quantum electrodynamics in a laser is formulated, in which the electron-laser interaction is exactly considered, while the interaction of an electron and a single photon is considered by perturbation. The formulation is applied to the…

Quantum Physics · Physics 2014-08-11 Qi-Ren Zhang