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Motivated by the magnetism of pyrochlore oxides, we consider the effect of quantum fluctuations in the most general symmetry-allowed nearest-neighbor Kramers exchange Hamiltonian on the pyrochlore lattice. At the classical level, this…

Strongly Correlated Electrons · Physics 2025-08-12 Lasse Gresista , Daniel Lozano-Gómez , Matthias Vojta , Simon Trebst , Yasir Iqbal

The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions,…

Strongly Correlated Electrons · Physics 2017-03-29 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We study the ground-state and low-energy properties of classical vector spin models with nearest-neighbour antiferromagnetic interactions on a class of geometrically frustrated lattices which includes the kagome and pyrochlore lattices. We…

Statistical Mechanics · Physics 2009-10-31 R. Moessner , J. T. Chalker

We study the low-temperature behaviour of the classical Heisenberg antiferromagnet with nearest neighbour interactions on the pyrochlore lattice. Because of geometrical frustration, the ground state of this model has an extensive number of…

Statistical Mechanics · Physics 2009-10-30 R. Moessner , J. T. Chalker

The effective quantum pseudospin-1/2 model for interacting rare-earth magnetic moments, which are locally described with atomic doublets, is studied theoretically for magnetic pyrochlore oxides. It is derived microscopically for localized…

Strongly Correlated Electrons · Physics 2015-03-17 Shigeki Onoda , Yoichi Tanaka

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised…

Strongly Correlated Electrons · Physics 2024-08-06 S. Nallamuthu , Andrea Dzubinska , K. Arun , Vimaljith A. R , Marian Reiffers , R. Nagalakshmi , Ivan Curlik , Sergej Ilkovic

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Two geometrically frustrated pyrochlore stannates, undergoing long range magnetic order below 1K, were investigated at very low temperature. Anomalies in the behaviour of hyperfine quantities are found, by 155Gd Mossbauer spectroscopy in…

Strongly Correlated Electrons · Physics 2009-11-13 P. Bonville , I. Mirebeau , J. P. Sanchez

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

MuSR experiments have been performed on powder sample of the "ordered spin ice" Tb$_2$Sn$_2$O$_7$ pyrochlore compound. At base temperature (T=35mK) the muon relaxation is found to be of dynamical nature which demonstrates that strong…

Strongly Correlated Electrons · Physics 2009-11-11 F. Bert , P. Mendels , A. Olariu , N. Blanchard , G. Collin , A. Amato , C. Baines , A. D. Hillier
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