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We investigate the phase behavior of a single-component system in 3 dimensions with spherically-symmetric, pairwise-additive, soft-core interactions with an attractive well at a long distance, a repulsive soft-core shoulder at an…

Soft Condensed Matter · Physics 2009-11-07 G. Franzese , G. Malescio , A. Skibinsky , S. V. Buldyrev , H. E. Stanley

Thermodynamics tells us to expect underwater contact between two hydrophobic surfaces to result in stronger adhesion compared to two hydrophilic surfaces. However, presence of water changes not only energetics, but also the dynamic process…

Soft Condensed Matter · Physics 2022-11-22 Mengyue Sun1 , Nityanshu Kumar1 , Ali Dhinojwala , Hunter King

In a recent paper [PRL 91, 138103 (2003)] a new mechanism to explain the cold denaturation of proteins, based on the loss of local low-density water structure, has been proposed. In the present paper this mechanism is tested by means of…

Other Condensed Matter · Physics 2009-11-11 Manuel I. Marques

We study the evolution of rotational response of a hydrodynamic model of a two-component superfluid with a non-dissipative drag interaction, as the system undergoes a transition into a paired phase at finite temperature. The transition…

Statistical Mechanics · Physics 2008-10-21 E. K. Dahl , E. Babaev , A. Sudbo

The phase diagram of water harbours many mysteries: some of the phase boundaries are fuzzy, and the set of known stable phases may not be complete. Starting from liquid water and a comprehensive set of 50 ice structures, we compute the…

Statistical Mechanics · Physics 2021-01-27 Aleks Reinhardt , Bingqing Cheng

A two-dimensional system of 10000 hard disks with square periodic boundary conditions, at a density in the middle of the 2-phase region predicted from equation-of-state data, when subjected to a weak external uniform force, is seen to phase…

Statistical Mechanics · Physics 2008-06-09 Leslie V Woodcock

We determine the phase diagram of liquid supercooled water by extensive computer simulations using the TIP5P-E model [J. Chem. Phys. {\bf 120}, 6085 (2004)]. We find that the transformation of water into a low density liquid in the…

Statistical Mechanics · Physics 2007-05-23 Dietmar Paschek

We report the first observation of homogeneous crystallization in simulated high-dimensional ($d > 3$) liquids that follow physically realistic dynamics and have system sizes that are large enough to eliminate the possibility that…

Soft Condensed Matter · Physics 2023-11-08 Robert S. Hoy

Molecular dynamics results on water confined in a silica pore in the low hydration regime are presented. Strong layering effects are found due to the hydrophilic character of the substrate. The local properties of water are studied as…

Soft Condensed Matter · Physics 2009-11-07 P. Gallo , M. Rapinesi , M. Rovere

We investigate the implications of integrability for the existence of quantum disentangled liquid (QDL) states in the half-filled one-dimensional Hubbard model. We argue that there exist finite energy-density eigenstates that exhibit QDL…

Strongly Correlated Electrons · Physics 2017-11-09 Thomas Veness , Fabian H. L. Essler , Matthew P. A. Fisher

Solid CS$_{2}$ is superficially similar to CO$_{2}$, with the same $Cmca$ molecular crystal structure at low pressures, which has suggested similar phases also at high pressures. We carried out an extensive first principles evolutionary…

Materials Science · Physics 2015-06-23 S. Shahab Naghavi , Yanier Crespo , Roman Martonak , Erio Tosatti

\textit{Ab initio} random structure searching based on density functional theory is used to determine the ground-state structures of ice at high pressures. Including estimates of lattice zero-point energies, ice is found to adopt three…

Other Condensed Matter · Physics 2013-05-29 Jeffrey M. McMahon

We present diffusion Monte Carlo (DMC) results on a new metastable, superfluid phase above the crystal ground state in two-dimensional 4He at densities > 0.065 1/A^2. The state is anisotropic with hexatic orbital order. This implies that…

Other Condensed Matter · Physics 2009-11-13 V. Apaja , M. Saarela

In this work the high pressure region of the phase diagram of water has been studied by computer simulation by using the TIP4P/2005 model of water. Free energy calculations were performed for ices VII and VIII and for the fluid phase to…

Materials Science · Physics 2009-01-14 J. L. Aragones , M. M. Conde , E. G. Noya , C. Vega

Within the framework of density functional theory, the inclusion of exact exchange and non-local van der Waals/dispersion (vdW) interactions is crucial for predicting a microscopic structure of ambient liquid water that quantitatively…

Soft Condensed Matter · Physics 2015-10-12 Biswajit Santra , Robert A. DiStasio , Fausto Martelli , Roberto Car

A fluid in a pore can form diverse heterogeneous structures. We combine a capillary description with the cubic-plus-association equation of state to study the thermodynamic stability of droplets, bubbles and films of water at 358 K in a…

Computational Physics · Physics 2019-09-04 Magnus Aa. Gjennestad , Øivind Wilhelmsen

The most accepted origin for the water anomalous behavior is the phase transition between two liquids (LLPT) in the supercooled regime connected to the glassy first order phase transition at lower temperatures. Two length scales potentials…

Soft Condensed Matter · Physics 2023-04-19 José Rafael Bordin , Leandro B. Krott

The transitions in disordered substances are discussed briefly: liquid--liquid phase transitions, liquid--glass transition and the transformations of one amorphous form to another amorphous form of the same substances. A description of…

Disordered Systems and Neural Networks · Physics 2007-05-23 V. N. Ryzhov , E. E. Tareyeva

Motivated by experimental and numerical studies revealing that discoidal high-density lipoprotein (HDL) particles may adopt flat elliptical and nonplanar saddle-like configurations, it is hypothesized that these might represent stabilized…

Soft Condensed Matter · Physics 2013-07-23 Mohsen Maleki , Eliot Fried

Liquid water exhibits anomalous behavior in the supercooled region. A popular hypothesis to explain supercooled water's anomalies is the existence of a metastable liquid-liquid transition terminating at a critical point. The hypothesized…

Chemical Physics · Physics 2020-01-08 V. P. Voronov , V. E. Podnek , M. A. Anisimov