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Based on ab initio calculations we determine the features and relative stability of different models proposed to describe the $(2 \times 2)$-FeO(111) reconstruction. Our results suggest that both wurtzite and spinel-like environments are…

Strongly Correlated Electrons · Physics 2016-09-21 Ivan Bernal-Villamil , Silvia Gallego

The two-dimensional electron gas found at the surface of SrTiO$_3$ and related interfaces has attracted significant attention as a promising basis for oxide electronics. In order to utilize its full potential, the response of this 2DEG to…

We present a combined experimental-theoretical study demonstrating the role of site disorder, off-stoichiometry and strain on the optical behavior of magnetoelectric gallium ferrite. Optical properties such as band-gap, refractive indices…

Surface magnetic properties of the pseudomorphic Fe(110) monolayer on a W(110) substrate are investigated from first principles as a function of the substrate thickness (up to eight layers). Analyzing the magnetocrystalline anisotropy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Torsten Andersen , Wolfgang Hübner

In the majority of magnetic systems the surface is required to order at the same temperature as the bulk. In the present study, we report a distinct and unexpected surface magnetic phase transition, uniquely at a lower temperature than the…

A large challenge in determining the physics of helimagnetic SrFeO3 is in stabilizing the stoichiometric chemical phase over long enough time scales to conduct extensive measurements. Degradation in SrFeO3 manifests mainly as a crossover…

Iron oxides play an increasingly prominent role in heterogeneous catalysis, hydrogen production, spintronics and drug delivery. The surface or material interface can be performance limiting in these applications, so it is vital to determine…

Controlling the surface structure on the atomic scale is a major difficulty for most transition metal oxides; this is especially true for the ternary perovskites. The influence of surface stoichiometry on the atomic structure of the…

Materials Science · Physics 2018-04-13 Stefan Gerhold , Zhiming Wang , Michael Schmid , Ulrike Diebold

LaAlO3 and SrTiO3 are insulating, nonmagnetic oxides, yet the interface between them exhibits a two-dimensional electron system with high electron mobility,1 superconductivity at low temperatures,2-6 and electric-field-tuned metal-insulator…

Superconductivity · Physics 2015-05-30 J. A. Bert , B. Kalisky , C. Bell , M. Kim , Y. Hikita , H. Y. Hwang , K. A. Moler

Controlling magnetism by using electric fields is a goal of research towards novel spintronic devices and future nano-electronics. For this reason, multiferroic heterostructures attract much interest. Here we provide experimental evidence,…

The oxygen stoichiometry has a large influence on the physical and chemical properties of complex oxides. Most of the functionality in e.g. catalysis and electrochemistry depends in particular on control of the oxygen stoichiometry. In…

Crystal surfaces are sensitive to the surrounding environment, where atoms left with broken bonds reconstruct to minimize surface energy. In many cases, the surface can exhibit chemical properties unique from the bulk. These differences are…

Materials Science · Physics 2016-12-21 Weizong Xu , Preston C. Bowes , Everett D. Grimley , Douglas L. Irving , James M. LeBeau

The (111) facet of magnetite (Fe$_3$O$_4$) has been studied extensively by experimental and theoretical methods, but controversy remains regarding the structure of its low-energy surface terminations. Using density functional theory (DFT)…

Oxide based ferromagnet/semiconductor heterostructures offer substantial advantages for spin electronics. We have grown (111) oriented Fe3O4 thin films and Fe3O4/ZnO heterostructures on ZnO(0001) and Al2O3(0001) substrates by pulsed laser…

Materials Science · Physics 2008-12-30 A. Nielsen , A. Brandlmaier , M. Althammer , W. Kaiser , M. Opel , J. Simon , W. Mader , S. T. B. Goennenwein , R. Gross

Layered ruthenates are a unique class of systems which manifests a variety of electronic and magnetic features emerged from competing energy scales. At the heart of such features lies the multi-orbital physics, especially, the…

Strongly Correlated Electrons · Physics 2022-11-08 Minjae Kim , Chang-Jong Kang , Jae-Ho Han , Kyoo Kim , Bongjae Kim

Changes of the magnetic and crystal structure on the microscopic scale in 40 nm FeRh thin films have been applied to investigate the phenomena of a disorder induced ferromagnetism at room temperature initiated through light ion-irradiation…

Effect of oxygen off-stoichiometry on the structural and magnetic properties of La0.15Sr0.85MnO3-d (d = 0.02,0.14) has been studied employing low-temperature x-ray diffraction, calorimetry, electrical-transport and magnetization. The nearly…

Materials Science · Physics 2014-02-27 Aga Shahee , R. J. Chaudhari , R. Rawat , A. M. Awasthi , N. P. Lalla

We employ spin-polarized (SP) STM to study the spin-dependent tunneling between a magnetite (111) sample and an antiferromagnetic tip through a vacuum barrier at room temperature. Atomic scale STM images show significant magnetic contrast…

Materials Science · Physics 2007-05-23 N. Berdunov , S. Murphy , G. Mariotto , I. V. Shvets

Digital image correlation of laser-ablated platinum nanoparticles on the surface of a polycrystalline metal (nickel-based superalloy Rene 88DT) was used to obtain the local strain behavior from an in situ scanning electron microscope…

Materials Science · Physics 2013-09-02 M. A. Tschopp , B. B. Bartha , W. J. Porter , P. T. Murray , S. B. Fairchild

Strontium titanate (SrTiO$_3$) is a foundational material in the emerging field of complex oxide electronics. While its electronic and optical properties have been studied for decades, SrTiO$_3$ has recently become a renewed materials…

Mesoscale and Nanoscale Physics · Physics 2014-07-11 W. D. Rice , P. Ambwani , M. Bombeck , J. D. Thompson , C. Leighton , S. A. Crooker