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Except for ortho- and para-H2, very little is known about nuclear spin isomers (or spin modifications) of molecules. The main reason is the lack of practical enrichment techniques. Recently a few enrichment methods were developed, which…

Chemical Physics · Physics 2007-05-23 P. L. Chapovsky , L. J. F. Hermans

In this article, we study control of electron-nuclear spin dynamics at magnetic field strengths where the Larmor frequency of the nucleus is comparable to the hyperfine coupling strength. The quantization axis for the nuclear spin differs…

Quantum Physics · Physics 2009-11-13 Navin Khaneja

We investigate the influence of nuclear spins on the resistance of helical edge states of two-dimensional topological insulators (2DTIs). Via the hyperfine interaction, nuclear spins allow electron backscattering, otherwise forbidden by…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Chen-Hsuan Hsu , Peter Stano , Jelena Klinovaja , Daniel Loss

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

The mesoscopic spin system formed by the 10E4-10E6 nuclear spins in a semiconductor quantum dot offers a unique setting for the study of many-body spin physics in the condensed matter. The dynamics of this system and its coupling to…

Mesoscale and Nanoscale Physics · Physics 2013-01-11 Bernhard Urbaszek , Xavier Marie , Thierry Amand , Olivier Krebs , Paul Voisin , Patrick Maletinsky , Alexander Hogele , Atac Imamoglu

Within the scheme of quantum rate equations, we investigate the spin-resolved transport through a double quantum dot system with four ferromagnetic terminals. It is found that the injection efficiency of spin-polarized electrons can be…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Ling Qin , Hai-Feng Lu , Yong Guo

Electron spin qubits in silicon, whether in quantum dots or in donor atoms, have long been considered attractive qubits for the implementation of a quantum computer due to the semiconductor vacuum character of silicon and its compatibility…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 M. Urdampilleta , A. Chatterjee , C. C. Lo , T. Kobayashi , J. Mansir , S. Barraud , A. C. Betz , S. Rogge , M. F. Gonzalez-Zalba , J. J. L. Morton

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

We study repeated (noncontinuous) measurements on the electron spin in a quantum dot and find that the measurement technique may lead to a different met$ or mechanism to realize nuclear spin polarization. While it may be used in any case,…

Quantum Physics · Physics 2011-07-28 Lian-Ao Wu

We theoretically investigate the influence of the fluctuating Overhauser field on the spin of an electron confined to a quantum dot (QD). The fluctuations arise from nuclear angular momentum being exchanged between different nuclei via the…

Mesoscale and Nanoscale Physics · Physics 2014-05-07 Erik Welander , Evgeny Chekhovich , Alexander Tartakovskii , Guido Burkard

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic…

The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and…

Quantum Physics · Physics 2018-10-02 J. E. Lang , J. -P. Tetienne , T. S. Monteiro

We study theoretically the formation of the nuclear-spin polaron state in semiconductor nanosystems within the Lindblad equation approach. To this end, we derive a general Lindblad equation for the density operator that complies with the…

Mesoscale and Nanoscale Physics · Physics 2022-06-01 Iris Kleinjohann , Andreas Fischer , Mikhail M. Glazov , Frithjof B. Anders

We observe dynamic nuclear polarization in a GaAs double dot system using two electrons that are never exchanged with the reservoir. By periodically bringing the system to the mixing point where the singlet and the triplet T+ states are…

Mesoscale and Nanoscale Physics · Physics 2008-01-24 S. Foletti , J. Martin , M. Dolev , D. Mahalu , V. Umansky , A. Yacoby

Dynamic nuclear polarization is widely used to enhance the sensitivity of nuclear magnetic resonance. It is presently the method of choice for enhancing the sensitivity of high-field solid state NMR experiments performed under cryogenic…

Chemical Physics · Physics 2022-02-02 Maria Grazia Concilio , Ilya Kuprov , Lucio Frydman

It is well known that non-central nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear…

Nuclear Theory · Physics 2015-11-17 Jun Xu , Bao-An Li , Wen-Qing Shen , Yin Xia

We study the effect of contact hyperfine interaction on the nuclear spin diffusion coefficients in semiconductor quantum dots. The diffusion coefficients are calculated with both the method of moment and density matrix. We show that nuclear…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Changxue Deng , Xuedong Hu

We propose a new mechanism for polarizing nuclear spins in quantum dots, based on periodic modulation of the hyperfine coupling by electric driving at the electron spin resonance frequency. Dynamical nuclear polarization results from…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 M. S. Rudner , L. S. Levitov

An all-optical scheme to polarize nuclear spins in a single quantum dot is analyzed. The hyperfine interaction with randomly oriented nuclear spins presents a fundamental limit for electron spin coherence in a quantum dot; by cooling the…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. Imamoglu , E. Knill , L. Tian , P. Zoller

We find that detuning an optical pulse train from electronic transitions in quantum dots controls the direction of nuclear spin flips. The optical pulse train generates electron spins that precess about an applied magnetic field, with a…

Quantum Physics · Physics 2015-05-13 S. G. Carter , A. Shabaev , Sophia E. Economou , T. A. Kennedy , A. S. Bracker , T. L. Reinecke
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