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While the vibrational thermodynamics of materials with small anharmonicity at low temperatures has been understood well based on the harmonic phonons approximation; at high temperatures, this understanding must accommodate how phonons…

Materials Science · Physics 2015-10-20 Tian Lan

Anharmonic lattice vibrations govern the thermal dynamics in materials and present how the atoms interact and how they conduct heat. An indepth understanding of the microscopic mechanism of phonon anharmonicity in condensed systems is…

Materials Science · Physics 2021-12-30 Bin Wei , Qiyang Sun , Chen Li , Jiawang Hong

The anharmonic lattice dynamics of rock-salt thermoelectric compounds SnTe and PbTe are investigated with inelastic neutron scattering (INS) and first-principles calculations. The experiments show that, surprisingly, although SnTe is closer…

Materials Science · Physics 2015-06-18 C. W. Li , O. Hellman , J. Ma , A. F. May , H. B. Cao , X. Chen , A. D. Christianson , G. Ehlers , D. J. Singh , B. C. Sales , O. Delaire

We present a microscopic theory for ultrafast control of solids with high-intensity terahertz frequency optical pulses. When resonant with selected infrared-active vibrations, these pulses transiently modify the crystal structure and lead…

Strongly Correlated Electrons · Physics 2014-07-15 Alaska Subedi , Andrea Cavalleri , Antoine Georges

Anharmonic lattice vibrations play a key role in many physical phenomena. They govern the heat conductivity of solids, strongly affect the phonon spectra, play a prominent role in soft mode phase transitions, allow ultrafast engineering of…

Materials Science · Physics 2026-02-12 Gili Scharf , Tomer Hasharoni , Lara Donval , Leah Ben Gur , Alon Ron

We study the impact of phonon anharmonicity on the electronic dynamics of soft materials using a nonperturbative quantum-classical approach. The method is applied to a one-dimensional model of doped organic semiconductors with low-frequency…

Materials Science · Physics 2025-09-24 Jonathan H. Fetherolf , Petra Shih , Timothy C. Berkelbach

This Chapter contains an overview of the effects of nonlinear interactions in selected problems of non-equilibrium statistical mechanics. Most of the emphasis is put on open setups, where energy is exchanged with the environment. With…

Pattern Formation and Solitons · Physics 2020-06-23 Stefano Iubini , Stefano Lepri , Roberto Livi , Antonio Politi , Paolo Politi

The lattice dynamics of TiO$_2$ in the rutile crystal structure was studied by a combination of thermal diffuse scattering, inelastic x-ray scattering and density functional perturbation theory. We experimentally confirm the existence of an…

Materials Science · Physics 2016-01-13 Björn Wehinger , Alexeï Bosak , Paweł T. Jochym

Dynamics of an array of line defects interacting with a background elastic medium is studied in the linear regime. It is shown that the inertial coupling between the defects and the ambient phonons leads to an anomalous response behavior…

Statistical Mechanics · Physics 2009-11-07 Ali Najafi , Ramin Golestanian

With the use of theory developed earlier, bulk effects in ultracold neutron coherent inelastic scattering are considered both for solid and liquid target samples related to energy and momentum exchange with phonon and diffusion-like modes.…

Nuclear Theory · Physics 2009-11-10 A. L. Barabanov , S. T. Belyaev

The energy spectrum of the extended attractive potential of a crystallographic row for negatively charged particles has quasi-bound states. It follows that a negatively charged particle with small transversal momentum component ($p_{\bot} R…

Mesoscale and Nanoscale Physics · Physics 2015-01-12 Gennady V. Kovalev

The phonon dispersion relations of crystal lattices can often be well-described with the harmonic approximation. However, when the potential energy landscape exhibits more anharmonicity, for instance, in case of a weakly bonded crystal or…

Materials Science · Physics 2022-01-19 Jonathan Lahnsteiner , Menno Bokdam

The effect of "anomalous" scattering of neutrons and electrons from protons in the electron-volt energy-transfer range is considered, and related experimental results are mentioned. A recent independent confirmation of this effect with a…

Quantum Physics · Physics 2007-05-23 C. Aris Chatzidimitriou-Dreismann

Phonon hydrodynamics is an exotic phonon transport phenomenon that challenges the conventional understanding of diffusive phonon scattering in crystalline solids. It features a peculiar collective motion of phonons with various…

Materials Science · Physics 2022-05-24 Kanka Ghosh , Andrzej Kusiak , Jean-Luc Battaglia

Anharmonic effects in an atomic monolayer thin crystal with honeycomb lattice structure are investigated by analytical and numerical lattice dynamical methods. Starting from a semi-empirical model for anharmonic couplings of third and…

Materials Science · Physics 2015-05-20 K. H. Michel , S. Costamagna , F. M. Peeters

We investigated the lattice dynamics of the unconventional superconductor LiFeAs using inelastic neutron scattering experiments and density-functional theory (DFT) calculations. By comparing the neutron scattering intensities with…

The anharmonic lattice dynamics of oxide and halide perovskites play a crucial role in their mechanical and optical properties. Raman spectroscopy is one of the key methods used to study these structural dynamics. However, despite decades…

The lattice dynamics in substitutional disordered alloys with constituents having large size differences is driven by strong disorder in masses, inter-atomic force constants and local environments. In this letter, a new first-principles…

Materials Science · Physics 2016-08-14 Oscar Grånäs , Biswanath Dutta , Subhradip Ghosh , Biplab Sanyal

Detailed understanding of vibrational heat transfer mechanisms between solids is essential for the efficient thermal engineering and control of nanomaterials. We investigate the frequency dependence of anharmonic scattering and interfacial…

Materials Science · Physics 2014-10-31 K. Sääskilahti , J. Oksanen , J. Tulkki , S. Volz

Knowledge of lattice anharmonicity is essential to elucidate distinctive thermal properties in crystalline solids. Yet, accurate \textit{ab initio} investigations of lattice anharmonicity encounter difficulties owing to the cumbersome…

Materials Science · Physics 2022-04-13 Zhen Zhang , Dong-Bo Zhang , Tao Sun , Renata M. Wentzcovitch
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