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We investigated the photoexcited carrier dynamics in Si by using optical pump and terahertz probe spectroscopy in an energy range between 2 meV and 25 meV. The formation dynamics of excitons from unbound e-h pairs was studied through the…

Materials Science · Physics 2015-05-27 Takeshi Suzuki , Ryo Shimano

Understanding heat transport in organic semiconductors is of fundamental and practical relevance. Therefore, we study the lattice thermal conductivities of a series of (oligo)acenes, where an increasing number of rings per molecule leads to…

Materials Science · Physics 2024-12-09 Lukas Legenstein , Lukas Reicht , Sandro Wieser , Michele Simoncelli , Egbert Zojer

As a newly emergent type-II Dirac semimetal, Platinum Telluride (PtTe2) stands out from other 2D noble-transition-metal dichalcogenides for the unique structure and novel physical properties, such as high carrier mobility, strong…

We report an optical study of charge transport in graphene. Diffusion of hot carriers in epitaxial graphene and reduced graphene oxide samples are studied using an ultrafast pump-probe technique with a high spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Brian A. Ruzicka , Shuai Wang , Lalani K. Werake , Ben Weintrub , Kian Ping Loh , Hui Zhao

Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

Due to its high electrical conductivity and excellent transmittance at terahertz frequencies, graphene is a promising candidate as transparent electrodes for terahertz devices. We demonstrate a liquid crystal based terahertz phase shifter…

Cubic boron arsenide (BAs) is promising for microelectronics thermal management due to its high thermal conductivity. Recently, its potential as an optoelectronic material is also being explored. However, it remains challenging to measure…

In order to determine the role of non-thermal transport of hot carriers which is decisive for the dissipation of energy in condensed matter we performed time-resolved broadband femtosecond transient reflectivity measurements on $7-197…

Funtionalized pentacene, 6,13-bis(triisopropylsilylethynyl)pentacene (TIPS-pentacene), field-effect transistors(FET's) were made by thermal evaporation or solution deposition method and the mobility was measured as a function of temperature…

Strongly Correlated Electrons · Physics 2007-05-23 Jin Gyu Park , Relja Vasic , James S. Brooks , John E. Anthony

We report the effect of air exposure on the electronic properties of pentacene single crystals. Air can diffuse reversibly in and out of the crystals and controls the physical properties. We discern two competing mechanisms that modulate…

Materials Science · Physics 2009-11-11 Oana D. Jurchescu , Jacob Baas , Thomas T. M. Palstra

Atomic-scale disorder shapes the potential energy landscape traversed by photoexcited charge carriers, while the carriers themselves also dynamically reshape this landscape. However, resolving ultrafast photocarrier motion at atomic length…

Mesoscale and Nanoscale Physics · Physics 2026-04-29 Vedran Jelic , Kaedon Cleland-Host , Stefanie Adams , Mohamed Hassan , Austin Hayes , Tyler L. Cocker

We present a novel optical transient absorption and reflection microscope based on a diffraction-limited pump pulse in combination with a wide-field probe pulse, for the spatio-temporal investigation of ultrafast population transport in…

The perturbation of a semiconductor from the thermodynamic equilibrium often leads to the display of nonlinear dynamics and formation of spatiotemporal patterns due to the spontaneous generation of competing processes. Here, we describe the…

Materials Science · Physics 2019-09-16 Ebrahim Najafi , Amir Jafari , Bolin Liao , Ahmed Zewail

THz Time-Resolved Photoconductivity is used to probe carrier dynamics in the dilute III-V nitride GaP0.49As0.47N0.036. In these measurements a femtosecond optical pump-pulse excites electron-hole pairs, and a delayed THz pulse measures the…

Materials Science · Physics 2018-11-14 J. N. Heyman , E. M. Weiss , J. R. Rollag , K. M. Yu , O. D. Dubon , Y. J. Kuang , C. W. Tu , W. Walukiewicz

W. Chr. Germs, K. Guo, R. A. J. Janssen, and M. Kemerink [1] recently measured the temperature and concentration dependent seebeck coefficient in organic thin film transistor and found the seebeck coefficient increases with carrier…

Disordered Systems and Neural Networks · Physics 2012-12-04 Ling Li , Nianduan Lu , Ming Liu

We propose the use of a frequency-dependent photothermal measurement as a complement to light-flash, i.e. time-dependent, measurements to determine the through-plane thermal diffusivity of small, thin samples, e.g. semiconducting polymers…

Materials Science · Physics 2018-11-14 Maryam Shahi , J. W. Brill

A semi-classical Monte Carlo model for studying three-dimensional carrier dynamics in photoconductive switches is presented. The model was used to simulate the process of photoexcitation in GaAs-based photoconductive antennas illuminated…

Other Condensed Matter · Physics 2016-08-31 E. Castro-Camus , J. Lloyd-Hughes , M. B. Johnston

Even though the terahertz spectrum is well suited for chemical identification, material characterization, biological sensing and medical imaging, practical development of these applications has been hindered by the attributes of terahertz…

Topological crystalline insulators -- topological insulators whose properties are guaranteed by crystalline symmetry -- can potentially provide a promising platform for terahertz optoelectronic devices, as their properties can be tuned on…

Optics · Physics 2021-11-08 Zhenyang Xiao , Jiashu Wang , Xinyu Liu , Badih Assaf , David Burghoff

Terahertz (THz) radiation has uses from security to medicine; however, sensitive room-temperature detection of THz is notoriously difficult. The hot-electron photothermoelectric effect in graphene is a promising detection mechanism:…