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Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

The electronic structure of the vanadium dioxide VO_2 in the tetragonal R and two monocinic M_1 and M_2 structural modifications was calculated in frames of the local-density functional (LDA) approach and the LSDA + U formalism of…

Strongly Correlated Electrons · Physics 2007-05-23 M. A. Korotin , N. A. Skorikov , V. I. Anisimov

Different types of order are discussed in the context of strongly correlated transition metal oxides, involving pure compounds and $3d^{3}-4d^{4}$ and $3d^{2}-4d^{4}$ hybrids. Apart from standard, long-range spin and orbital orders we…

Strongly Correlated Electrons · Physics 2019-10-24 Wojciech Brzezicki

To compare the metal-insulator transitions (MITs) of VO2 and V2O3 we analyze the relations between the structural and electronic properties of the vanadium Magneli phases. These materials set up the homologous series VnO(2n-1) (3 <= n <= 9)…

Strongly Correlated Electrons · Physics 2009-11-10 Udo Schwingenschloegl , Volker Eyert

The common phase diagrams of superconducting iron pnictides show interesting material specificities in the structural and magnetic phase transitions. In some cases the two transitions are separate and second order, while in others they…

Strongly Correlated Electrons · Physics 2012-02-14 Ryan Applegate , Rajiv R. P. Singh , Cheng-Chien Chen , Thomas P. Devereaux

Evolution of composite spin-orbital order and coupled spin-orbital excitations is studied in a variety of $d^4$ systems with $n$=$4$ electrons in the $t_{2g}$ orbital sector using the generalised self-consistent + fluctuations approach for…

Strongly Correlated Electrons · Physics 2025-04-30 Shahid Ahmad , Harshvardhan Parmar , Shubhajyoti Mohapatra , Avinash Singh

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

Vanadium Sesquioxide (V$_2$O$_3$) is an antiferromagnetic insulator below $T_{\mathrm N}\approx$ 155 K. The magnetic order is not of C- or G-type as one would infer from the bipartite character of the hexagonal basal plane in the…

Materials Science · Physics 2015-08-19 Daniel Grieger , Michele Fabrizio

We show that 1:1 ordering of A$'$ and A$''$ cations in A$'_{1/2}$A$''_{1/2}$B$_2$X$_4$ magnetic spinels results in appearance of magnetoelectric properties. Possible value of magnetically induced electric polarization is calculated using…

Strongly Correlated Electrons · Physics 2014-05-15 N. V. Ter-Oganessian

The lacunar spinel GaV4S8 exhibits orbital ordering at 44 K and shows a complex magnetic phase diagram below 12.7 K, which includes ferromagnetic and cycloidal spin order. At low but finite external magnetic fields, N\'eel-type skyrmions…

Strongly Correlated Electrons · Physics 2017-12-14 S. Widmann , E. Ruff , A. Günther , H. -A. Krug von Nidda , P. Lunkenheimer , V. Tsurkan , S. Bordács , I. Kézsmárki , A. Loidl

Using realistic low-energy model with parameters derived from the first-principles electronic structure calculation, we address the origin of the quasi-one-dimensional behavior in orthorhombic NaV$_2$O$_4$, consisting of the double chains…

Materials Science · Physics 2012-09-11 Z. V. Pchelkina , I. V. Solovyev , R. Arita

Insulating spinel materials, with the chemical formula $AB_2X_4$, behave as diamond lattice antiferromagnets when only the A-site atom is magnetic. Many exhibit classic signatures of frustration, induced not geometrically but by competing…

Strongly Correlated Electrons · Physics 2011-11-15 SungBin Lee , Leon Balents

The ferrimagnetic spinel $\mathrm{CoV_2O_4}$ has been a topic of intense recent interest, both as a frustrated insulator with unquenched orbital degeneracy and as a near-itinerant magnet which can be driven metallic with moderate applied…

Strongly Correlated Electrons · Physics 2016-02-03 D. Reig-i-Plessis , D. Casavant , V. O. Garlea , A. A. Aczel , M. Feygenson , J. Neuefeind , H. D. Zhou , S. E. Nagler , G. J. MacDougall

We report the magnetic properties of $A$-site spinel compound MnSc$_2$Se$_4$. The macroscopic magnetic measurements uncovers successive magnetic transitions at $T_{\rm{N1}}$= 2.04 K, followed by two further transitions at $T_{\rm{N2}}$=1.8…

Strongly Correlated Electrons · Physics 2022-06-01 K. Guratinder , V. Tsurkan , L. Prodan , L. Keller , J. P. Embs , F. Juranyi , M. Medarde , Ch. Rüegg , O. Zaharko

Evidence has been found for a change in the ordered occupation of the vanadium d-orbitals at the 77K phase transition in YVO3, manifested by a change in the type of Jahn-Teller distortion. The orbital ordering above 77K is not destroyed at…

Strongly Correlated Electrons · Physics 2009-11-07 G. R. Blake , T. T. M. Palstra , Y. Ren , A. A. Nugroho , A. A. Menovsky

The puzzling nature of magnetic and lattice phase transitions of iron pnictides is investigated via a first-principles Wannier function analysis of representative parent compound LaOFeAs. A rare ferro-orbital ordering is found to give rise…

Superconductivity · Physics 2010-01-07 Chi-Cheng Lee , Wei-Guo Yin , Wei Ku

The single layered manganite Pr$_{0.22}$Sr$_{1.78}$MnO$_4$ undergoes structural transition from high temperature tetragonal phase to low temperature orthorhombic phase below room temperature. The orthorhombic phase was reported to have two…

Strongly Correlated Electrons · Physics 2012-04-25 S. Chattopadhyay , S. Giri , S. Majumdar

We report a systematic enhancement of the pressure dependence of TN in A2+[V2]O4 spinels as the V-V separation approaches the critical separation for a transition to itinerant-electron behavior. An intermediate phase between localized and…

Using density-functional theory calculations and experimental investigations on structural, magnetic and dielectric properties, we have elucidated a unique tetragonal ground state for MnTi2O4, a Ti^{3+} (3d^1)-ion containing spinel-oxide.…

Strongly Correlated Electrons · Physics 2019-10-09 A. Rahaman , M. Chakraborty , T. Paramanik , R. K. Maurya , S. Mahana , R. Bindu , D. Topwal , P. Mahadevan , D. Choudhury

We attribute the structural phase transition (SPT) in the parent compounds of the iron pnictides to orbital ordering. Due to the anisotropy of the $d_{xz}$ and $d_{yz}$ orbitals in the $xy$ plane, a ferro-orbital ordering makes the…

Strongly Correlated Electrons · Physics 2013-05-29 Weicheng Lv , Jiansheng Wu , Philip Phillips