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A structural model of hydrogenated amorphous silicon containing an isolated dangling bond is used to investigate the effects of electron interactions on the electronic level splittings, localization of charge and spin, and fluctuations in…

Materials Science · Physics 2009-11-07 R. G. Hennig , P. A. Fedders , A. E. Carlsson

From density functional calculations, we show that localized states stemming from defects or topological disorder exhibit an anomalously large electron-phonon coupling. We provide a simple analysis to explain the observation and perform a…

Disordered Systems and Neural Networks · Physics 2009-11-10 Raymond Atta-Fynn , Parthapratim Biswas , D. A. Drabold

We present a computational study of the electronic properties of amorphous SiO2. The ionic configurations used are the ones generated by an earlier molecular dynamics simulations in which the system was cooled with different cooling rates…

Disordered Systems and Neural Networks · Physics 2009-10-30 Thorsten Koslowski , Walter Kob , Katharina Vollmayr

Electron localization is the tendency of an electron in a many-body system to exclude other electrons from its vicinity. Using a new natural measure of localization based on the exact manyelectron wavefunction, we find that localization can…

Mesoscale and Nanoscale Physics · Physics 2021-01-15 T. R. Durrant , M. J. P. Hodgson , J. D. Ramsden , R. W. Godby

We study the spatial structure of wave functions with exceptionally high local amplitudes in the Anderson model of localisation. By means of exact diagonalisations of finite systems, we obtain and analyse images of these wave functions: we…

Disordered Systems and Neural Networks · Physics 2009-11-07 V. Uski , B. Mehlig , M. Schreiber

The study of defect centers in silicon has been recently reinvigorated by their potential applications in optical quantum information processing. A number of silicon defect centers emit single photons in the telecommunication $O$-band,…

Many-electron systems confined to a quasi-1D geometry by a cylindrical distribution of positive charge have been investigated by density functional computations in the unrestricted local spin density approximation. Our investigations have…

Mesoscale and Nanoscale Physics · Physics 2010-08-27 R. Cortes-Huerto M. Paternostro P. Ballone

We investigated the effect of spin polarization on the structural properties and gradient of electric field (EFG) on Sn, In, and Cd impurity in RSn$_3$ (R=Sm, Eu, Gd) and RIn$_3$ (R=Tm, Yb, Lu) compounds. The calculations were performed…

Strongly Correlated Electrons · Physics 2009-11-13 S. Jalali Asadabadi , H. Akbarzadeh

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray

Highly accurate experimental structure factors of silicon are available in the literature, and these provide the ideal test for any \emph{ab initio} method for the construction of the all-electron charge density. In a recent paper [J. R.…

Materials Science · Physics 2015-05-14 J. R. Trail , D. M. Bird

The many-body wave-function of an interacting one-dimensional electron system is probed, focusing on the low-density, strong interaction regime. The properties of the wave-function are determined using tunneling between two long, clean,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 H. Steinberg , O. M. Auslaender , A. Yacoby , J. Qian , G. A. Fiete , Y. Tserkovnyak , B. I. Halperin , K. W. Baldwin , L. N. Pfeiffer , K. W. West

The structural and electronic properties of amorphous silicon ($a$-Si) are investigated by first-principles calculations based on the density-functional theory (DFT), focusing on the intrinsic structural defects. By simulated melting and…

Materials Science · Physics 2017-10-11 Yoritaka Furukawa , Yu-ichiro Matsushita

We present a theoretical study of the structure-property correlation in gallium ferrite, based on the first principles calculations followed by a subsequent comparison with the experiments. Local spin density approximation (LSDA+U) of the…

Materials Science · Physics 2011-07-27 Amritendu Roy , Somdutta Mukherjee , Rajeev Gupta , Rajendra Prasad , Sushil Auluck , Ashish Garg

First-principles density functional theory (DFT) codes which employ a localized basis offer advantages over those which use plane-wave bases, such as better scaling with system size and better suitability to low-dimensional systems. The…

Materials Science · Physics 2024-11-25 Daniel Bennett , Michele Pizzochero , Javier Junquera , Efthimios Kaxiras

We propose a computational method that simplifies drastically the inclusion of spin-orbit interaction in density functional theory implemented on localised atomic orbital basis sets. Our method is based on a well-known procedure for…

Materials Science · Physics 2009-11-11 Lucas Fernandez-Seivane , Miguel A. Oliveira , Stefano Sanvito , Jaime Ferrer

The spin-polarization at the V(001) surface has been studied by using different local (LSDA) and semilocal (GGA) approximations to the exchange-correlation potential of DFT within two ab initio methods: the all-electron TB-LMTO-ASA and the…

Strongly Correlated Electrons · Physics 2009-10-31 R. Robles , J. Izquierdo , A. Vega , L. C. Balbas

Graphene antidot lattices have recently been proposed as a new breed of graphene-based superlattice structures. We study electronic properties of triangular antidot lattices, with emphasis on the occurrence of dispersionless (flat) bands…

Mesoscale and Nanoscale Physics · Physics 2009-07-16 Mihajlo Vanevic , Vladimir M. Stojanovic , Markus Kindermann

Electronic properties of III-V semiconductor alloys are examined using first principles with the focus on the spatial localization of electronic states. We compare localization at the band edges due to various isovalent impurities in a host…

Materials Science · Physics 2017-06-15 C. Pashartis , O. Rubel

Linear scaling density functional theory approaches to electronic structure are often based on the tendency of electrons to localize even in large atomic and molecular systems. However, in many cases of actual interest, for example in…

Chemical Physics · Physics 2022-03-25 Marcel David Fabian , Ben Shpiro , Roi Baer

Numerical studies of amorphous silicon in harmonic approximation show that the highest 3.5% of vibrational normal modes are localized. As vibrational frequency increases through the boundary separating localized from delocalized modes, near…

Disordered Systems and Neural Networks · Physics 2007-05-23 William Garber , Folkert M. Tangerman , Philip B. Allen , Joseph L. Feldman
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