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We analyze electronically excited nuclear wave functions and their coherence when subjecting a molecule to the action of natural, pulsed incoherent solar-like light, and to that of ultrashort coherent light assumed to have the same center…

Quantum Physics · Physics 2015-06-12 Alex C. Han , Moshe Shapiro , Paul Brumer

Recent experiments claimed that the enhancement of catalytic reaction rates occurs via the reduction of activation barriers driven by non-equilibrium (``hot'') electrons in plasmonic metal nanoparticles. These experiments place plasmonic…

Chemical Physics · Physics 2020-04-22 Yonatan Sivan , Ieng Wai Un , Yonatan Dubi

The electronic and nuclear dynamics in methanol, following 156~nm photoexcitation, are investigated by combining a detailed analysis of time-resolved photoelectron spectroscopy experiments with electronic structure calculations. The…

We present experimental and modeling studies of UV nanosecond pulsed laser desorption and ablation of (111) bulk silicon. The results involve a new approach to the analysis of plume formation dynamics under high-energy photon irradiation of…

Materials Science · Physics 2007-05-23 Wladimir Marine , Nadezhda M. Bulgakova , Lionel Patrone , Igor Ozerov

Absorption and scattering of electromagnetic waves by dielectric media are of fundamental importance in many branches of physics. In this Letter we analytically derived the ultimate upper limits for the absorbed and scattered powers by any…

Optics · Physics 2015-06-02 Jean-Paul Hugonin , Mondher Besbes , Philippe Ben-Abdallah

We present a novel analytical model for analysing the spectral photoluminescence quantum yield of non-planar semiconductor thin films. This model considers the escape probability of luminescence and is applied to triple-cation perovskite…

The local field approach and kinetic equation method is applied to calculate the surface plasmon radiative damping in a spheroidal metal nanoparticle embedded in any dielectric media. The radiative damping of the surface plasmon resonance…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Nicolas I. Grigorchuk

We report plasmon-enhanced Raman scattering in graphene coupled to a single plasmonic hotspot measured as a function of laser energy. The enhancement profiles of the G peak show strong enhancement (up to $10^5$) and narrow resonances (30…

Controlling macroscopic properties of quantum materials requires the ability to induce and manipulate excited states. The set of collective excitations of a solid is encoded in its dispersion relations. We find that the spectra of the…

For the development and optimization of novel light emitting materials, such as fluorescent proteins, dyes and semiconductor quantum dots (QDs), a reliable and robust analysis of the emission efficiency is crucial. The emission efficiency…

Epitaxially-grown quantum well and quantum dot solar cells suffer from weak light absorption, strongly limiting their performance. Light trapping based on optical resonances is particularly relevant for such devices to increase light…

Applied Physics · Physics 2023-11-10 Maxime Giteau , Yusuke Oteki , Kento Kitahara , Naoya Miyashita , Ryo Tamaki , Yoshitaka Okada

We ask whether soft photons, defined by asymptotic charges, can have consequences for the outcome of localised quantum processes. We consider a spatially localised two-state system, at rest in flat spacetime, coupled to a $U(1)$ gauge…

High Energy Physics - Theory · Physics 2021-08-11 Sanved Kolekar , Jorma Louko

Hybrid pumping appears as a promising compromise in order to reach the much coveted goal of an electrically pumped organic laser. In such configuration the organic material is optically pumped by an electrically pumped inorganic device on…

Motivated by Pierre Auger Observatory results favoring a heavy nuclear composition for ultrahigh-energy (UHE) cosmic rays, we investigate implications for the cumulative neutrino background. The requirement that nuclei not be…

High Energy Astrophysical Phenomena · Physics 2016-03-14 Kohta Murase , John F. Beacom

We present a description of a strongly driven multimode optomechanical system that shows the emergence of cooperative effects usually known from systems of atom-light interaction. Our calculations show that under application of a coherent…

Quantum Physics · Physics 2014-11-11 T. Kipf , G. S. Agarwal

The interplay of the non-equivalent corners in the Brillouin zone of transition metal dichalcogenides have been investigated extensively. While experimental and theoretical works contributed to a detailed understanding of the relaxation of…

Mesoscale and Nanoscale Physics · Physics 2023-10-13 Malte Selig , Dominik Christiansen , Manuel Katzer , Mariana V. Ballottin , Peter C. M. Christianen , Andreas Knorr

An important determinant of crop yields is the regulation of photosystem II (PSII) light harvesting by energy-dependent quenching (qE). However, the molecular details of excitation quenching have not been quantitatively connected to the…

Biological Physics · Physics 2022-06-08 Doran I. G. Bennett , Graham R. Fleming , Kapil Amarnath

Assuming a spherical symmetry, the extreme UV emitted by a very hot source ionizes low pressure molecular hydrogen making a transparent bubble of H II (Protons and electrons). For an increase of radius, intensity of extreme UV and…

General Physics · Physics 2007-07-23 Jacques Moret-Bailly

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…

Optics · Physics 2024-02-27 Zhiyuan Wang , Jianwei Tang , Jiahao Han , Juan Xia , Tianzi Ma , Xue-Wen Chen

The spontaneous emission rate of a radiating atom reaches its time-independent equilibrium value after an initial transient regime. In this paper we consider the associated relaxation effects of the spontaneous decay rate of atoms in…

Quantum Physics · Physics 2007-10-31 Martijn Wubs , L. G. Suttorp
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