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We investigate the distribution of the number of photons emitted by a single molecule undergoing a spectral diffusion process and interacting with a continuous wave laser field. The spectral diffusion is modeled based on a stochastic…

Statistical Mechanics · Physics 2009-11-10 Yong He , Eli Barkai

We present a general relation between Mandel's $Q$ parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing.…

Statistical Mechanics · Physics 2007-05-23 Eli Barkai , YounJoon Jung , Robert Silbey

A theory is formulated for time dependent fluctuations of the spectrum of a single molecule in a dynamic environment. In particular, we investigate the photon counting statistics of a single molecule undergoing a spectral diffusion process.…

Statistical Mechanics · Physics 2007-05-23 YounJoon Jung , Eli Barkai , Robert J. Silbey

We derive the moment generating function for photon emissions from a single molecule driven by laser excitation. The frequencies of the fluoresced photons are explicitly considered. Calculations are performed for the case of a two level dye…

Statistical Mechanics · Physics 2009-08-14 Golan Bel , Frank L. Brown

A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…

Chemical Physics · Physics 2009-11-13 F. Shikerman , E. Barkai

We consider the theory of the non-linear spectroscopy for a single molecule undergoing stochastic dynamics and interacting with a sequence of two laser pulses. General expressions for photon counting statistics are obtained, and an exact…

Optics · Physics 2008-01-13 F. Shikerman , E. Barkai

Mandel Q-parameter, which is determined from single event photon statistics, provides an alternative to differentiate single-molecule with fluorescence detection. In this work, by using the Q-parameter of the sample fluorescence compared to…

Quantum Physics · Physics 2009-11-13 Shuangli Dong , Tao Huang , Yuan Liu , Jun Wang , Guofeng Zhang , Liantuan Xiao+ , Suotang Jia

We follow the trajectories of phase singularities at nulls of intensity in the speckle pattern of waves transmitted through random media as the frequency of the incident radiation is scanned in microwave experiments and numerical…

Disordered Systems and Neural Networks · Physics 2015-06-19 Xiaojun Cheng , Yitzchak Lockerman , Azriel Z. Genack

The exact analytical solution of Maxwell equations for a Bessel light beam scattered by a sphere is found. Scattered power, stored energy and a generalized Q factor as a function of frequency, the sphere radius, permittivity, and the Bessel…

Optics · Physics 2020-08-26 Vasily Klimov

Quantum networks require flying qubits that transfer information between the nodes. This may be implemented by means of single atoms (the nodes) that emit and absorb single photons (the flying qubits) and requires full control of photon…

Quantum Physics · Physics 2017-09-20 Philipp Müller , Tristan Tentrup , Marc Bienert , Giovanna Morigi , Jürgen Eschner

We studied intensity fluctuations of a single photon source relying on the pulsed excitation of the fluorescence of a single molecule at room temperature. We directly measured the Mandel parameter Q(T) over 4 orders of magnitude of…

Quantum Physics · Physics 2009-11-07 F. Treussart , R. Alleaume , V. Le Floc'h , L. T. Xiao , J. -M Courty , J. -F. Roch

In the solid state, a large variety of single-photon emitters present high quality photophysical properties together with a potential for integration. However, in many cases, the host matrix induces fluctuations of the emission wavelength…

Optics · Physics 2026-02-05 Aymeric Delteil , Stéphanie Buil , Jean-Pierre Hermier

The optical spectrum of a quantum system is jointly determined by the properties of the emitter and the driving field. All-optical spectral control can hence be a promising method to engineer the properties of single photon emitters for…

The small cross section of Raman scattering poses a great challenge for its direct study at the single-molecule level. By exploiting the high Franck-Condon factor of a common-mode resonance, choosing a large vibrational frequency difference…

The propagation of light in a resonant atomic vapor can \textit{a priori} be thought of as a multiple scattering process, in which each scattering event redistributes both the direction and the frequency of the photons. Particularly, the…

We investigate theoretically a scheme for spectroscopy of electrons emitted by an on-demand single particle source. The total system, with an electron turnstile source and a single level quantum dot spectrometer, is implemented with edge…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 F. Battista , P. Samuelsson

In this paper, we design and analyze a novel spectral method for the subdiffusion equation. As it has been known, the solutions of this equation are usually singular near the initial time. Consequently, direct application of the traditional…

Numerical Analysis · Mathematics 2022-04-06 Chuanju Xu , Wei Zeng

The analysis of single-mode photon fluctuations and their counting statistics at the superradiant phase transition is presented. The study concerns the equilibrium Dicke model in a regime where the Rabi frequency, related to a coupling of…

Mesoscale and Nanoscale Physics · Physics 2019-06-26 D. S. Shapiro , A. N. Rubtsov , S. V. Remizov , W. V. Pogosov , Yu. E. Lozovik

We calculate spectra of radiation produced by a relativistic particle in the presence of one-dimensional Langmuir turbulence which might be generated by a streaming instability in the plasma, in particular, in the shock front or at the…

Astrophysics · Physics 2009-06-23 Gregory D. Fleishman , Igor N. Toptygin

We investigate spontaneous photon emission processes of two-level atoms in parabolic and ellipsoidal cavities thereby taking into account the full multimode scenario. In particular, we calculate the excitation probabilities of the atoms and…

Quantum Physics · Physics 2014-12-05 Gernot Alber , Nils Trautmann
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