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We discuss the transition strength between the disordered ground state and the basic low-lying triplet excitation for the Heisenberg chain with alternating exchange based on series expansions in the interdimer interaction up to tenth order.…

Strongly Correlated Electrons · Physics 2007-05-23 M. Mueller , H. -J. Mikeska

We have studied dimerized spin systems by realizing the cluster expansion to high order. We have extended our previous dimer expansion for one-dimensional systems to cover weakly interacting chains for a quantitative description of three…

Strongly Correlated Electrons · Physics 2009-11-07 H. -J. Mikeska , M. Mueller

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

The dynamical spin structure factor and the Raman response are calculated for structurally dimerized and spin-Peierls chains in a magnetic field, using exact diagonalization techniques. In both cases there is a spin liquid phase composed of…

Strongly Correlated Electrons · Physics 2009-10-31 Weiqiang Yu , Stephan Haas

We have performed an {\it ab initio} study of the electronic structure of two isostructural quantum spin systems, KCuCl$_{3}$ and TlCuCl$_{3}$, which have recently attracted much attention due to their unconventional magnetic properties.…

Materials Science · Physics 2009-11-07 T. Saha-Dasgupta , R. Valenti

The compound TlCuCl3 represents a model system of dimerized quantum spins with strong interdimer interactions. We investigate the triplet dispersion as a function of temperature by inelastic neutron scattering experiments on single…

Strongly Correlated Electrons · Physics 2009-11-11 Ch. Rüegg , B. Normand , M. Matsumoto , Ch. Niedermayer , A. Furrer , K. W. Krämer , H. U. Güdel , Ph. Bourges , Y. Sidis , H. Mutka

A study is presented of a two-dimensional frustrated and dimerized quantum spin-system which models the effect of inter-chain coupling in a spin-Peierls compound. Employing a bond-boson method to account for quantum disorder in the ground…

Strongly Correlated Electrons · Physics 2009-10-30 Wolfram Brenig

The minerals A2Cu3O(SO4)3 (A2=Na2, NaK, K2) constitute quantum spin systems with copper hexamers as basic structural units. Strong intra-hexamer spin couplings give rise to an effective triplet ground-state. Weak inter-hexamer spin…

Strongly Correlated Electrons · Physics 2021-12-06 A. Furrer , A. Podlesnyak , E. Pomjakushina , V. Pomjakushin

The mineral malachite, Cu2(OD)2CO3, has a quantum spin-liquid ground state and no long-range magnetic order down to at least T=0.4 K. Inelastic neutron scattering measurements show that the excitation spectrum consists of dispersive gapped…

Strongly Correlated Electrons · Physics 2015-03-05 E. Canevet , B. Fak , R. K. Kremer , J. H. Chun , M. Enderle , E. E. Gordon , J. L. Bettis , M. -H. Whangbo , J. W. Taylor , D. T. Adroja

The magnetic field--driven transition in the spin-Peierls system CuGeO_3 associated with the closing of the spin gap is investigated numerically. The field dependence of the spin dynamical structure factor (seen by inelastic neutron…

Strongly Correlated Electrons · Physics 2009-10-30 D. Poilblanc , J. Riera , C. A. Hayward , C. Berthier , M. Horvatic

Dimethylammonium copper (II) chloride (also known as DMACuCl3 or MCCL) is a low dimensional S=1/2 quantum spin system proposed to be an alternating ferro-antiferromagnetic chain with similar magnitude ferromagnetic (FM) and…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , W. Tian , G. E. Granroth , M. D. Lumsdena , J-H. Chung , D. G. Mandrusa , S. E. Nagler

We study the phase transition in a system composed of dimers interacting with each other via a nearest-neighbor (NN) exchange $J$ and competing interactions taken from a truncated dipolar coupling. Each dimer occupies a link between two…

Statistical Mechanics · Physics 2013-09-06 Danh-Tai Hoang , Hung T. Diep

TlCuCl$_3$ has a singlet ground state with the excitation gap $\Delta =0.65$ meV. The magnetic excitations in TlCuCl$_3$ have been investigated by means of neutron inelastic scattering experiments. The constant-$\it{\pmb Q}$ energy scan…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Kato , H. Tanaka , K. Kakurai , M. Mueller , H. -J. Mikeska

We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…

Strongly Correlated Electrons · Physics 2009-11-10 N. Johannsen , A. Vasiliev , A. Oosawa , H. Tanaka , T. Lorenz

Below about 150 K, the spin arrangement in the chain arrays of Sr14Cu24O41 is shown to develop in two dimensions (2D). Both the correlations and the dispersion of the observed elementary excitations agree well with a model of interacting…

Strongly Correlated Electrons · Physics 2009-10-31 L. P. Regnault , J. P. Boucher , H. Moudden , J. E. Lorenzo , A. Hiess , U. Ammerahl , G. Dhalenne , A. Revcolevschi

Recently measured high-field ESR spectra of the spin dimer material TlCuCl3 are described within the framework of an effective field theory. A good agreement between the theory and experiment is achieved, for all geometries and in a wide…

Strongly Correlated Electrons · Physics 2009-11-10 A. K. Kolezhuk , V. N. Glazkov , H. Tanaka , A. Oosawa

Single-crystal neutron inelastic scattering was performed in order to investigate the magnetic excitations in the spin gap system TlCuCl$_3$. The constant-${\bf Q}$ energy scan profiles were collected in the $a^*-c^*$ plane. Three…

Condensed Matter · Physics 2007-05-23 A. Oosawa , T. Kato , H. Tanaka , H. Uekusa , Y. Ohashi , K. Nakajima , M. Nishi , K. Kakurai

We have analyzed the experimental susceptibility data of KCuCl$_3$ and found that the data are well-explained by the double-spin-chain models with strong antiferromagnetic dimerization. Large quantum Monte Carlo calculations were performed…

Condensed Matter · Physics 2009-10-30 Tota Nakamura , Kiyomi Okamoto

We treat the ground state, elementary excitations, and neutron scattering cross section for a system of trimers consisting of three tightly bound spins 1/2 on a distorted Kagom\'e lattice, subject to isotropic nearest neighbor (usually…

Strongly Correlated Electrons · Physics 2015-06-15 A. B. Harris , T. Yildirim

The ground state of the spin-Peierls system TiOCl was probed using synchrotron x-ray diffraction on a single-crystal sample at T = 6 K. We tracked the evolution of the structural superlattice peaks associated with the dimerized ground state…

Strongly Correlated Electrons · Physics 2012-08-23 A. Prodi , J. S. Helton , Yejun Feng , Y. S. Lee
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