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Motivated to understand the phonon spectrum renormalization in the ground state of the half-filled SSH model, we use the Born-Oppenheimer approximation together with the harmonic approximation to evaluate the all-to-all real-space ionic…

Strongly Correlated Electrons · Physics 2021-10-04 Stepan Fomichev , Mona Berciu

We reformulate and extend porous electrode theory for non-ideal active materials, including those capable of phase transformations. Using principles of non-equilibrium thermodynamics, we relate the cell voltage, ionic fluxes, and Faradaic…

Chemical Physics · Physics 2012-08-24 Todd R. Ferguson , Martin Z. Bazant

The exciton on a single polydiacetylene chain is considered in a Wannier approach, taking into account the surrounding polarizable medium. The electron-hole Coulomb interaction potential is explictly obtained for a quantum wire of circular…

Strongly Correlated Electrons · Physics 2007-05-23 Francois Dubin , Michel Schott

We study the electrostatic potential of a molecular wire bridging two metallic electrodes in the limit of weak contacts. With the use of a tight-binding model including a fully three-dimensional treatment of the electrostatics of the…

Chemical Physics · Physics 2007-05-23 Stéphane Pleutin , Hermann Grabert , Gert-Ludwig Ingold , Abraham Nitzan

We investigate the transport behavior of polyene molecules sandwiched between two metallic contacts using the non-equilibrium Green's function formalism. We calculate both current and noise power as a function of applied voltage and show…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 S. Dallakyan , S. Mazumdar

Conduction in pristine conjugated polymers (other than polyacetylene) is by polaron hopping between sites corresponding to conjugation lengths. The strong increase of current $I$ with voltage $V$ observed for both emission-limited and ohmic…

Soft Condensed Matter · Physics 2015-06-25 E. M. Conwell , M. W. Wu

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking exciton effects into…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

When the energy of a pump wave is in resonance with the exciton creation energy, the electric susceptibility of a conjugated polymer in response to the probe wave is altered by the exciton gas. In this paper, we calculate the dependence of…

Condensed Matter · Physics 2009-10-30 Ming-Che Chang , Hsin-Fei Meng

Nonlinear behavior of electro-osmosis in dilute non-adsorbing polymer solutions with low salinity is investigated with Brownian dynamics simulations and a kinetic theory. In the Brownian simulations, the hydrodynamic interaction between the…

Soft Condensed Matter · Physics 2015-06-19 Yuki Uematsu

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking into account of the…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

The excited state electronic structure of $\pi$ conjugated phenylene-acetylene oligomers is calculated using time-dependent density functional theory (TD-DFT) approaches. The theoretical fluorescence spectra are analyzed in terms of…

Chemical Physics · Physics 2015-06-26 R. J. Magyar , S. Tretiak , Y. Gao , H. L. Wang , A. P. Shreve

We have studied the feasibility of electron conduction in azulene molecule and compared with that in its isomer naphthalene. We have used non-equilibrium Green's function formalism to measure the current in our systems as a response of the…

Materials Science · Physics 2008-07-23 Sudipta Dutta , S. Lakshmi , Swapan K. Pati

A method for the study of the electronic transport in strongly coupled electron-phonon systems is formalized and applied to a model of polyyne chains biased through metallic Au leads. We derive a stationary non equilibrium polaronic theory…

Mesoscale and Nanoscale Physics · Physics 2009-09-09 A. La Magna , I. Deretzis , V. Privitera

We calculate non-perturbatively the inelastic effects on the conductance through a conjugated molecular wire-metal heterojunction, including realistic electron-phonon coupling. We show that at sub-band-gap energies the current is dominated…

Materials Science · Physics 2009-10-31 H. Ness , A. J. Fisher

We study collective plasmon excitations and screening of disordered single- and bilayer black phosphorus beyond the low energy continuum approximation. The dynamical polarizability of phosphorene is computed using a tight-binding model that…

Mesoscale and Nanoscale Physics · Physics 2015-09-30 Fengping Jin , Rafael Roldán , Mikhail I. Katsnelson , Shengjun Yuan

We study theoretically the current-voltage characteristics, shot noise, and full counting statistics of a quantum wire double barrier structure. We model each wire segment by a spinless Luttinger liquid. Within the sequential tunneling…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Jaeuk U. Kim , Mahn-Soo Choi , Ilya V. Krive , Jari M. Kinaret

We develop a bosonization technique for one-dimensional fermions out of equilibrium. The approach is used to study a quantum wire attached to two electrodes with arbitrary energy distributions. The non-equilibrium electron Green function is…

Mesoscale and Nanoscale Physics · Physics 2010-06-08 D. B. Gutman , Yuval Gefen , A. D. Mirlin

The effect of electron-optical phonon interaction on the hydrogenic impurity binding energy in a cylindrical quantum wire is studied. By using Landau and Pekar variational method, the hamiltonian is separated into two parts which contain…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yueh-Nan Chen , Der-San Chuu , Yuh-Kae Lin

We develop a theory of tunneling spectroscopy of interacting electrons in a non-equilibrium quantum wire coupled to reservoirs. The problem is modelled as an out-of-equilibrium Luttinger liquid with spatially dependent interaction. The…

Mesoscale and Nanoscale Physics · Physics 2009-07-09 D. B. Gutman , Yuval Gefen , A. D. Mirlin

Computationally inexpensive approximations describing electron-phonon scattering in molecular-scale conductors are derived from the non-equilibrium Green's function method. The accuracy is demonstrated with a first principles calculation on…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Magnus Paulsson , Thomas Frederiksen , Mads Brandbyge
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