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Related papers: Bulk and interfacial properties of binary hard-pla…

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The effect of thermal fluctuations near a contact line of a liquid interface partially wetting an impenetrable substrate is studied analytically and numerically. Promoting both the interface profile and the contact line position to random…

Soft Condensed Matter · Physics 2016-11-15 D. Belardinelli , M. Sbragaglia , M. Gross , B. Andreotti

Chemically driven fluids can demix to form condensed droplets that exhibit phase behaviors not observed at equilibrium. In particular, nonequilibrium interfacial properties can emerge when the chemical reactions are driven differentially…

Soft Condensed Matter · Physics 2023-11-20 Yongick Cho , William M. Jacobs

We present a versatile density functional approach (DFT) for calculating the depletion potential in general fluid mixtures. In contrast to brute force DFT, our approach requires only the equilibrium density profile of the small particles…

Soft Condensed Matter · Physics 2009-10-31 R. Roth , R. Evans , S. Dietrich

Boundary conditions for the solid-liquid interface of the solidifying pure melt have been derived. In the derivation the model of Gibbs interface is used. The boundary conditions include both the state quantities of bulk phases are taken at…

Materials Science · Physics 2016-11-02 Gennady Buchbinder , Peter Galenko

We consider the evolution of interfaces in binary mixtures permeating strongly heterogeneous systems such as porous media. To this end, we first review available thermodynamic formulations for binary mixtures based on \emph{general…

Computational Physics · Physics 2018-04-26 M. Schmuck , G. A. Pavliotis , S. Kalliadasis

The theory of interface localization in near-critical planar systems at phase coexistence is formulated from first principles. We show that mutual delocalization of two interfaces, amounting to interfacial wetting, occurs when the bulk…

Statistical Mechanics · Physics 2016-05-13 Gesualdo Delfino

The description of fluid mixtures molecular behavior is significant for various industry fields due to the complex composition of fluid found in nature. Statistical mechanics approaches use intermolecular interaction potential to predict…

Chemical Physics · Physics 2022-01-19 Irina Nesterova , Yuriy Kanygin , Pavel Lomovitskiy , Aleksey Khlyupin

Although density functional theory provides reliable predictions for the static properties of simple fluids under confinement, a theory of comparative accuracy for the transport coefficients has yet to emerge. Nonetheless, there is evidence…

We investigate the equilibrium of a fluid in contact with a solid boundary through a density-functional theory. Depending on the conditions, the fluid can be in one phase, gas or liquid, or two phases, while the wall induces an external…

Fluid Dynamics · Physics 2012-02-06 Antonio Pereira , Serafim Kalliadasis

The statistical-mechanical study of the equilibrium properties of fluids, starting from the knowledge of the interparticle interaction potential, is essential to understand the role that microscopic interaction between individual particles…

Soft Condensed Matter · Physics 2025-10-07 Ana M. Montero

We investigate bulk structural properties of tetravalent associating particles within the framework of classical density functional theory, building upon Wertheim's thermodynamic perturbation theory. To this end, we calculate density…

Soft Condensed Matter · Physics 2021-12-08 Daniel Stopper , Frank Hirschmann , Martin Oettel , Roland Roth

The structural properties of additive binary hard-sphere mixtures are addressed as a follow-up of a previous paper [S. Pieprzyk et al., Phys. Rev. E 101, 012117 (2020)]. The so-called rational-function approximation method and an approach…

This work focuses on the interfacial dynamics with interfacial mass flux in the presence of acceleration and surface tension. We employ the general matrix method to find the fundamental solutions for the linearized boundary value problem…

Fluid Dynamics · Physics 2021-07-07 D. V. Ilyin , S. I. Abarzhi

It is shown that the density of two {\it initially independent} condensates which are allowed to expand and overlap can show interferences as a function of time due to interparticle interaction. Using many-body theory, explicit expressions…

Other Condensed Matter · Physics 2007-05-23 L. S. Cederbaum , A. I. Streltsov , Y. B. Band , O. E. Alon

Using classical density functional theory (DFT) in a modified mean-field approximation we investigate the fluid phase behavior of quasi-two dimensional dipolar fluids confined to a plane. The particles carry three-dimensional dipole moments…

Statistical Mechanics · Physics 2013-06-18 R. Geiger , S. H. Klapp

Within a recently developed mode-coupling theory for fluids confined to a slit we elaborate numerical results for the long-time limits of suitably generalized intermediate scattering functions. The theory requires as input the density…

Soft Condensed Matter · Physics 2021-10-29 Suvendu Mandal , Simon Lang , Vitalie Boţan , Thomas Franosch

The free energetics of water density fluctuations near a surface, and the rare low-density fluctuations in particular, serve as reliable indicators of surface hydrophobicity; the easier it is to displace the interfacial waters, the more…

Statistical Mechanics · Physics 2016-05-19 Erte Xi , Richard C. Remsing , Amish J. Patel

Soft particles can be better emulsifiers than hard particles because they stretch at fluid interfaces. This deformation can increase adsorption energies by orders of magnitude relative to rigid particles. The deformation of a particle at an…

Soft Condensed Matter · Physics 2015-07-15 Robert W. Style , Lucio Isa , Eric R. Dufresne

We extend the Cahn-Landau-de Gennes mean field theory of binary mixtures to understand the wetting thermodynamics of a three phase system, that is in contact with an external surface which prefers one of the phases. We model the system…

Soft Condensed Matter · Physics 2020-12-01 Biswaroop Mukherjee , Buddhapriya Chakrabarti

The molecular density functional theory of fluids provides an exact theory for computing solvation free energies in implicit solvents. One of the reasons it has not received nearly as much attention as quantum density functional theory for…

Statistical Mechanics · Physics 2019-02-04 David M. Rogers