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A simple and highly reproducible technique is demonstrated for the fabrication of metallic electrodes with nanometer separation. Commercially available bare gold colloidal nanoparticles are first trapped between prefabricated…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Saiful I. Khondaker , Zhen Yao

We form single-electron transistors from individual chemically-synthesized gold nanoparticles, 5-15 nm in diameter, with monolayers of organic molecules serving as tunnel barriers. These devices allow us to measure the discrete electronic…

Mesoscale and Nanoscale Physics · Physics 2008-12-17 F. Kuemmeth , K. I. Bolotin , S. -F. Shi , D. C. Ralph

Nanomechanical shuttles transferring small groups of electrons or even individual electrons from one electrode to another offer a novel approach to the problem of controlled charge transport. Here, we report the fabrication of…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 A. V. Moskalenko , S. N. Gordeev , O. F. Koentjoro , P. R. Raithby , R. W. French , F. Marken , S. E. Savel'ev

We report a simple and reproducible method to fabricate two metallic electrodes made of different metals with a nanometer-sized gap. These electrodes are fabricated by defining a pair of gold electrodes lithographically and…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Mandar M. Deshmukh , Amy L. Prieto , Qian Gu , Hongkun Park

Three terminal single-electron transistor devices utilizing Al/Al2O3 gate electrodes were developed for the study of electron transport through individual single-molecule magnets. The devices were patterned via multiple layers of optical…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. J. Henderson , C. M. Ramsey , E. del Barco , A. Mishra , G. Christou

We present a microscopic study of single-electron tunneling in nanomechanical double-barrier tunneling junctions formed using a vibrating scanning nanoprobe and a metallic nanoparticle connected to a metallic substrate through a molecular…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark A. Ratner

Transistors, regardless of their size, rely on electrical gates to control the conductance between source and drain contacts. In atomic-scale transistors, this conductance is exquisitely sensitive to single electrons hopping via individual…

We present a microscopic theory of single-electron tunneling through metallic nanoparticles connected to the electrodes through molecular bridges. It combines the theory of electron transport through molecular junctions with the description…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark A. Ratner

Pairs of electrodes with nanometer separation (nano-gap) are achieved through an electromigration-induced break-junction (EIBJ) technique at room temperature. Lithographically defined gold (Au) wires are formed by e-beam evaporation over…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ajit K. Mahapatro , Subhasis Ghosh , David B. Janes

Applying ac voltages, we trapped gold nanoparticles between microfabricated electrodes under well-defined conditions. We demonstrate that the nanoparticles can be controllably fused together to form homogeneous gold nanowires with…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 L. Bernard , M. Calame , S. J. van der Molen , J. Liao , C. Schoenenberger

Single-electron transistors would represent an approach for less power consuming microelectronic devices if room-temperature operation and industry-compatible fabrication were possible. We present a concept based on stripes of small,…

Materials Science · Physics 2017-07-18 Svenja Willing , Hauke Lehmann , Mirjam Volkmann , Christian Klinke

We demonstrate a device geometry for single-molecule electronics experiments that combines both the ability to adjust the spacing between the electrodes mechanically and the ability to shift the energy levels in the molecule using a gate…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 A. R. Champagne , A. N. Pasupathy , D. C. Ralph

We have developed a controlled and highly reproducible method of making nanometer-spaced electrodes using electromigration in ambient lab conditions. This advance will make feasible single molecule measurements of macromolecules with…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 D. R. Strachan , D. E. Smith , D. E. Johnston , T. -H. Park , M. J. Therien , D. A. Bonnell , A. T. Johnson

We report on the electric measurements of an individual Au nanoparticle with an ultra-high contact resistance of about $10^{19} \Omega$. The high-impedance measurements have been carried out by counting the electrons that are transferred…

Mesoscale and Nanoscale Physics · Physics 2008-03-12 An. Gruneis , M. J. Esplandiu , D. Garcia-Sanchez , A. Bachtold

We have developed a fast, yet highly reproducible method to fabricate metallic electrodes with nanometer separation using electromigration (EM). We employ four-terminal instead of two-terminal devices in combination with an analog feedback…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Zheng-Ming Wu , Michael Steinacher , Roman Huber , Michel Calame , Sense Jan van der Molen , Christian Schonenberger

We have investigated the spectrum of discrete electronic states in single, nm-scale Al particles incorporated into new tunneling transistors, complete with a gate electrode. The addition of the gate has allowed (a) measurements of the…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 D. C. Ralph , C. T. Black , M. Tinkham

Myoglobin single-electron transistors were investigated using nanometer- gap platinum electrodes fabricated by electromigration at cryogenic temperatures. Apomyoglobin (myoglobin without heme group) was used as a reference. The results…

Mesoscale and Nanoscale Physics · Physics 2013-12-16 Debin Li , Peter M. Gannet , David Lederman

The realization of single-molecule electronic devices, in which a nanometer-scale molecule is connected to macroscopic leads, requires the reproducible production of highly ordered nanoscale gaps in which a molecule of interest is…

Mesoscale and Nanoscale Physics · Physics 2009-05-08 Sujit S. Datta , Douglas R. Strachan , A. T. Charlie Johnson

We have developed a technology to reproducibly make gaps with distance control on the single atom scale. The gold contacts are flat on the nanometre scale and are fabricated on an oxidized aluminium film that serves as a gate. We show that…

Materials Science · Physics 2009-11-10 Y. V. Kervennic , D. Vanmaekelbergh , L. P Kouwenhoven , H. S. J Van der Zant

To date, endeavors in nanoscale spintronics are dominated by the use of single-electron or single-spin transistors having at their heart a semiconductor, metallic or molecular quantum dot who's localized states are non-spin-degenerate and…

Mesoscale and Nanoscale Physics · Physics 2017-12-12 Ilia N. Sivkov , Oleg O. Brovko , Ivan Rungger , Valeri S. Stepanyuk
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