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Related papers: Polymer Dynamics in Repton Model at Large Fields

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Polydispersity is inevitable in industrially produced polymers. Established theories of polymer dynamics and rheology, however, were mostly built on monodisperse linear polymers. Dynamics of polydisperse polymers is yet to be fully explored…

Soft Condensed Matter · Physics 2021-06-29 Oluseye Adeyemi , Shiping Zhu , Li Xi

We report a numerical study of the diffusiophoresis of short polymers using non-equilibrium molecular dynamics simulations. More precisely, we consider polymer chains in a fluid containing a solute which has a concentration gradient, and…

Soft Condensed Matter · Physics 2020-05-20 Simón Ramírez-Hinestrosa , Hiroaki Yoshida , Lydéric Bocquet , Daan Frenkel

We study asymptotic properties of diffusion and other transport processes (including self-avoiding walks and electrical conduction) on large randomly branched polymers using renormalized dynamical field theory. We focus on the swollen phase…

Statistical Mechanics · Physics 2015-06-04 Hans-Karl Janssen , Olaf Stenull

We study the segmental dynamics of poly(ethylene oxide) (PEO) from microscopic simulations in the neat polymer and a polymer electrolyte (PEO/LiBF$_4$) by analyzing the normal modes. We verify the applicability of the Rouse theory,…

Soft Condensed Matter · Physics 2008-04-15 Arijit Maitra , Andreas Heuer

The Rouse model can be regarded as the standard model to describe the dynamics of a short polymer chain under melt conditions. In this contribution, we explicitly check one of the fundamental assumptions of this model, namely that of a…

Soft Condensed Matter · Physics 2014-10-14 Diddo Diddens , Andreas Heuer

We study the dynamics of a polymer or a D-dimensional elastic manifold diffusing and convected in a non-potential static random flow (the ``randomly driven polymer model''). We find that short-range (SR) disorder is relevant for d < 4 for…

Condensed Matter · Physics 2009-07-10 Kay Joerg Wiese , Pierre Le Doussal

While the dynamics of dimers and polymer chains in a viscous solvent is well understood within the celebrated Rouse model, the effect of an external magnetic field on the dynamics of a charged chain is much less understood. Here we…

Statistical Mechanics · Physics 2022-07-01 Rushikesh Shinde , Jens Uwe Sommer , Hartmut Löwen , Abhinav Sharma

Synthetic polymers have a distribution of chain lengths which can be characterized by dispersity, D. Macroscopic properties of polymers are influenced by chain mobility in the melt and manipulating D can significantly impact these…

Chemical Physics · Physics 2024-09-30 Taofeek Tejuosho , Sohil Kollipara , Sumant Patankar , Janani Sampath

We study the propulsion of a one-dimensional (1D) polymer chain under sinusoidal external forces in the overdamped (low Reynolds number) regime. We show that, when hydrodynamical interactions are included, the polymer presents directional…

Soft Condensed Matter · Physics 2012-09-25 Daniel Santos-Oliván , Alessandro Fiasconaro , Fernando Falo

The research is important for a molecular theory of liquid and has a wide interest as an example solving the problem when dynamic parameters of systems can be indirectly connected with their equilibrium properties. In frameworks of the…

Statistical Mechanics · Physics 2007-05-23 Andrei N. Yakunin

Structure and dynamics of an active polymer on a smooth cylindrical surface are studied by Brownian dynamics simulations. The effect of active force on the polymer adsorption behavior and the combined effect of chain mobility, length N,…

Soft Condensed Matter · Physics 2024-08-21 Chen Shen , Chao-ran Qin , Tian-liang Xu , Kang Chen , Wen-de Tian

A lattice model is presented for the simulation of dynamics in polymeric systems. Each polymer is represented as a chain of monomers, residing on a sequence of nearest-neighbor sites of a face-centered-cubic lattice. The polymers are self-…

Soft Condensed Matter · Physics 2009-11-10 Alexander van Heukelum , G. T. Barkema

Fundamental understanding of the effect of microscopic parameters on the dynamics of probe particles in different complex environments has wide implications. Examples include diffusion of proteins in the biological hydrogels, porous media,…

Soft Condensed Matter · Physics 2019-09-11 Praveen Kumar , Ligesh Theeyancheri , Subhasish Chaki , Rajarshi Chakrabarti

Using extensive computer simulations, the behavior of the structural modes --- more precisely, the eigenmodes of a phantom Rouse polymer --- are characterized for a polymer in the three-dimensional repton model, and are used to study the…

Soft Condensed Matter · Physics 2015-03-18 Gerard T. Barkema , Debabrata Panja , J. M. J. van Leeuwen

We use direct numerical simulations to study homogeneous, and isotropic turbulent flows of dilute polymer solutions at high Reynolds and Deborah numbers. We find that for small wavenumbers $k$, the kinetic energy spectrum shows…

Fluid Dynamics · Physics 2023-02-14 Marco E Rosti , Prasad Perlekar , Dhrubaditya Mitra

The tumbling dynamics of individual polymers in semidilute solution is studied by large-scale non-equilibrium mesoscale hydrodynamic simulations. We find that the tumbling time is equal to the non-equilibrium relaxation time of the polymer…

Soft Condensed Matter · Physics 2011-03-21 C. -C. Huang , G. Sutmann , G. Gompper , R. G. Winkler

We study of the dynamics of ring polymers confined to diffuse in a background gel at low concentrations. We do this in order to probe the inter-play between topology and dynamics in ring polymers. We develop an algorithm that takes into…

Soft Condensed Matter · Physics 2014-08-22 Davide Michieletto , Davide Marenduzzo , Enzo Orlandini , Gareth P. Alexander , Matthew S. Turner

Polymer stretching in random smooth flows is investigated within the framework of the FENE dumbbell model. The advecting flow is Gaussian and short-correlated in time. The stationary probability density function of polymer extension is…

Chaotic Dynamics · Physics 2007-05-23 M. Martins Afonso , D. Vincenzi

Similarly-charged polyelectrolytes are known to attract each other and aggregate into bundles when the charge density of the polymers exceeds a critical value that depends on the valency of the counterions. The dynamics of aggregation of…

Soft Condensed Matter · Physics 2016-09-22 Anvy Moly Tom , R. Rajesh , Satyavani Vemparala

The statistics of polymers advected by a turbulent flow are investigated. To limit the polymer lengths above to coil-stretch transition, a FENE-P type relaxation law is used. The turbulence is modeled by a random strain, delta-correlated in…

Chaotic Dynamics · Physics 2009-11-07 Jean-Luc Thiffeault