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Related papers: Orbital ordering in undoped manganites using Jahn-…

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We study the ground state orbital ordering of $LaMnO_3$, at weak electron-phonon coupling, when the spin state is A-type antiferromagnet. We determine the orbital ordering by extending to our Jahn-Teller system a recently developed Peierls…

Strongly Correlated Electrons · Physics 2015-05-13 S. Yarlagadda , P. B. Littlewood , M. Mitra , R. K. Monu

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

Strongly Correlated Electrons · Physics 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

It is shown that the layered antiferromagnetic order in stoechiometric LaMnO_3 cannot be understood purely from electronic interactions. On the contrary, it mainly results from strong cooperative Jahn-Teller deformations. Those involve a…

Strongly Correlated Electrons · Physics 2009-10-31 M. Capone , D. Feinberg , M. Grilli

We present evidence that the insulator to metal transition in (La,Ca)MnO3 near x~0.2 is driven by the suppression of coherent Jahn-Teller distortions, originating from d type orbital ordering. The orbital ordered state is characterised by…

Materials Science · Physics 2009-11-07 Bas B. Van Aken , Auke Meetsma , Y. Tomioka , Y. Tokura , Thomas T. M. Palstra

We introduce an effective model for $e_g$ electrons to describe three-dimensional perovskite (La$_{1-x}$Sr$_{x}$MnO$_3$ and La$_{1-x}$Ca$_{x}$MnO$_3$) manganites and study the magnetic and orbital order on $4\times 4\times 4$ cluster using…

Strongly Correlated Electrons · Physics 2010-10-26 Krzysztof Rościszewski , Andrzej M. Oleś

We report on first principles Self-Interaction Corrected LSD (SIC-LSD) calculations of electronic structure of LaMnO$_{3}$ in the cubic phase. We found a strong tendency to localisation of the Mn $e_{g}$ electron and to orbital ordering. We…

Strongly Correlated Electrons · Physics 2009-11-11 H. Zenia , G. A. Gehring , W. M. Temmerman

The standard way to find the orbital occupation of Jahn-Teller (JT) ions is to use structural data, with the assumption of a one-to-one correspondence between the orbital occupation and the associated JT distortion, e.g. in O6 octahedron.…

Strongly Correlated Electrons · Physics 2011-10-19 Hua Wu , C. F. Chang , O. Schumann , Z. Hu , J. C. Cezar , T. Burnus , N. Hollmann , N. B. Brookes , A. Tanaka , M. Braden , L. H. Tjeng , D. I. Khomskii

The effect of uniaxial strain on electronic structure and magnetism in LaMnO$_3$ is studied from a model Hamiltonian that illustrates the competition between the Jahn-Teller, super exchange, and double exchange interactions. We retain in…

Materials Science · Physics 2010-12-07 B. R. K. Nanda , S. Satpathy

Resonant soft x-ray diffraction has been used to probe the temperature dependent orbital and magnetic structure of $\mathrm{LaSr_{2}Mn_{2}O_7}$. Previous crystallographic studies have shown that this material has almost no MnO$_{6}$ oxygen…

Strongly Correlated Electrons · Physics 2007-05-23 S. B. Wilkins , N. Stojic , T. A. W. Beale , N. Binggeli , P. Bencok , S. Stanescu , J. F. Mitchell , P. Abbamonte , P. D. Hatton , M. Altarelli

The origin of the cooperative Jahn-Teller distortion and orbital-order in LaMnO3 is central to the physics of the manganites. The question is complicated by the simultaneous presence of tetragonal and GdFeO3-type distortions and the strong…

Strongly Correlated Electrons · Physics 2013-05-29 Eva Pavarini , Erik Koch

We present a mean-field theory of charge, orbital, and spin ordering in manganites at 50% and 0% dopings by considering Jahn-Teller interaction, nearest-neighbor repulsion, and no single-site double occupancy. For spinless fermions, we show…

Strongly Correlated Electrons · Physics 2009-10-31 Sudhakar Yarlagadda , C. S. Ting

We report on high-temperature electron spin resonance studies of a detwinned LaMnO$_3$ single crystal across the Jahn-Teller transition at $T_{\rm JT}$ = 750 K. The anisotropy of the linewidth and g-factor reflects the local Jahn-Teller…

Strongly Correlated Electrons · Physics 2015-06-22 S. Schaile , H. -A. Krug von Nidda , J. Deisenhofer , M. V. Eremin , Y. Tokura , A. Loidl

The first-principles SIC-LSD theory is utilized to study electronic, magnetic and orbital phenomena in LaMnO$_{3}$. The correct ground state is found, which is antiferro orbitally ordered with the spin magnetic moments antiferromagnetically…

Strongly Correlated Electrons · Physics 2009-11-10 R. Tyer , W. M. Temmerman , Z. Szotek , G. Banach , A. Svane , L. Petit , G. A. Gehring

Using the multiband $d-p$ model and unrestricted Hartree-Fock approximation we investigate the electronic structure and spin-orbital order in three-dimensional MnO$_3$ lattice such as realized in LaMnO$_3$. The orbital order is induced and…

Strongly Correlated Electrons · Physics 2019-04-04 Krzysztof Rościszewski , Andrzej M. Oleś

We have studied the interplay between orbital ordering, Jahn-Teller and GdFeO3-type lattice distortions in perovskite-type transition-metal oxides using model Hartree-Fock calculations. It has been found that the covalency between A-site…

Strongly Correlated Electrons · Physics 2009-10-31 T. Mizokawa , D. I. Khomskii , G. A. Sawatzky

Based on the magnetoresistance, magnetization, ultrasound, and crystallographic data, we studied the role of the cooperative Jahn-Teller effect in the charge ordered (CO) state for La1-xCaxMnO3. We found that, with increasing the fraction…

Strongly Correlated Electrons · Physics 2009-11-10 R. K. Zheng , G. Li , A. N. Tang , Y. Yang , W. Wang , X. G. Li , Z. D. Wang , H. C. Ku

The functional properties of transition metal perovskite oxides are known to result from a complex interplay of magnetism, polarization, strain, and stoichiometry. Here, we show that for materials with a cooperative Jahn-Teller distortion,…

Materials Science · Physics 2021-01-04 Chiara Ricca , Nicolas Niederhauser , Ulrich Aschauer

The interactions between $e_g$ orbitals in neighboring sites are investigated in LaMnO$_3$ by taking into account virtual exchange of electrons and phonons. The spin and orbital ordering temperatures and the spin wave dispersion relation…

Strongly Correlated Electrons · Physics 2009-11-07 Satoshi Okamoto , Sumio Ishihara , Sadamichi Maekawa

We use the temperature of the structural phase transition to determine the Jahn-Teller (JT) coupling constant in the model derived for LaMnO$_3$ which includes both the superexchange between S=2 spins and the JT effect. We also investigate…

Strongly Correlated Electrons · Physics 2022-01-27 Olga Sikora , Andrzej M. Oles

LaMnO$_3$ is considered as a prototypical Jahn-Teller perovskite compound, exhibiting a metal to insulator transition at $T_{JT} = 750K$ related to the joint appearance of an electronic orbital ordering and a large lattice Jahn-Teller…

Strongly Correlated Electrons · Physics 2020-07-01 Michael Marcus Schmitt , Yajun Zhang , Alain Mercy , Philippe Ghosez
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