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The spin-flip rate that couples dark and bright excitons in self-assembled quantum dots is obtained from time-resolved spontaneous emission measurements in a modified local density of optical states. Employing this technique, we can…

Other Condensed Matter · Physics 2010-03-18 Jeppe Johansen , Brian Julsgaard , Søren Stobbe , Jørn M. Hvam , Peter Lodahl

The population dynamics of dark and bright excitons in (In,Ga)As/GaAs quantum dots is studied by two-color pump-probe spectroscopy in an external magnetic field. With the field applied in Faraday geometry and at T<20 K, the dark excitons…

Mesoscale and Nanoscale Physics · Physics 2012-05-08 H. Kurtze , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer

Silicon nanocrystals are studied by time-resolved fluorescence spectroscopy. After laser excitation the bright and dark exciton ground state levels are populated at random, but subsequently the decay curves reveal a thermalization between…

Mesoscale and Nanoscale Physics · Physics 2009-09-11 Brian Julsgaard , Ying-Wei Lu , Peter Balling , Arne Nylandsted Larsen

Electron-hole exchange interactions split the exciton ground state into "dark" and "bright" states. The dynamics of those states depends on the internal relaxation time between bright and dark states (spin-flip time), and on the radiative…

Materials Science · Physics 2009-11-11 Gustavo A. Narvaez , Gabriel Bester , Alberto Franceschetti , Alex Zunger

The dephasing time of the lowest bright exciton in CdSe/ZnS wurtzite quantum dots is measured from 5 K to 170 K and compared with density dynamics within the exciton fine structure using a sensitive three-beam four-wave-mixing technique…

Mesoscale and Nanoscale Physics · Physics 2012-02-23 Francesco Masia , Nicolò Accanto , Wolfgang Langbein , Paola Borri

The temperature-dependent electron spin relaxation of positively charged excitons in a single InAs quantum dot (QD) was measured by time-resolved photoluminescence spectroscopy at zero applied magnetic fields. The experimental results show…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

Exciton spin relaxation is investigated in single epitaxially grown semiconductor quantum dots in order to test the expected spin relaxation quenching in this system. We study the polarization anisotropy of the photoluminescence signal…

We calculate the acoustic phonon-assisted exciton spin relaxation in single self-assembled In$_{1-x}$Ga$_x$As/GaAs quantum dots using an atomic empirical pseudopotential method. We show that the transition from bright to dark exciton states…

Materials Science · Physics 2015-06-17 Hai Wei , Guang-can Guo , Lixin He

Photoluminescence of a single CdSe quantum dot embedded in a ZnSe nanowire has been investigated. It has been found that the dark exciton has a strong influence on the optical properties. The most visible influence is the strongly reduced…

We perform a theoretical study of radiative decay of dark intravalley excitons in transition metal dichalcogenide monolayers. This decay necessarily involves an electronic spin flip. The intrinsic decay mechanism due to interband spin-flip…

Mesoscale and Nanoscale Physics · Physics 2019-03-19 A. O. Slobodeniuk , D. M. Basko

Spin relaxation in undoped quasi-spherical CdS quantum dots at zero magnetic fields is investigated using time- and polarization-resolved transient absorption measurements. Unlike in previous studies of these systems, the measured signals…

Mesoscale and Nanoscale Physics · Physics 2007-09-27 P. Nahálková , D. Sprinzl , P. Malý , P. Němec , V. N. Gladilin , J. T. Devreese

Spin relaxation of electrons doped in InP quantum dots was studied by means of luminescence pump-probe and Hanle measurements. Optical pumping makes spins of doped electrons to be oriented in parallel to the helicity of the circularly…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Y. Masumoto , B. Pal , S. Oguchi , M. Ikezawa

The dark exciton state in semiconductor quantum dots constitutes a long-lived solid-state qubit which has the potential to play an important role in implementations of solid-state based quantum information architectures. In this work, we…

We demonstrate a new method of measuring the exciton spin relaxation time in semiconductor nanostructures by continuous-wave photoluminescence. We find that for self-assembled CdTe quantum dots the degree of circular polarization of…

Materials Science · Physics 2009-11-10 S. Mackowski , T. A. Nguyen , H. E. Jackson , L. M. Smith , J. Kossut , G. Karczewski

We show that a Bose-Einstein condensate consisting of dark excitons forms in GaAs coupled quantum wells at low temperatures. We find that the condensate extends over hundreds of micrometers, well beyond the optical excitation region, and is…

Mesoscale and Nanoscale Physics · Physics 2022-08-18 Subhradeep Misra , Michael Stern , Vladimir Umansky , Israel Bar Joseph

Exciton luminescence of a CdSe quantum dot (QD) inserted in a ZnSe nanowire is strongly influenced by the dark exciton states. Because of the small size of these QDs (2-5nm), exchange interaction between hole and electron is highly enhanced…

The fine structure of the exciton spectrum, containing optically allowed (bright) and forbidden (dark) exciton states, determines the radiation efficiency in nanostructures. We study time-resolved micro-photoluminescence in MoS$_2$…

We use one single, few-picosecond-long, variably polarized laser pulse to deterministically write any selected spin state of a quantum dot confined dark exciton whose life and coherence time are six and five orders of magnitude longer than…

Quantum Physics · Physics 2015-11-18 I. Schwartz , D. Cogan , E. R. Schmidgall , L. Gantz , Y. Don , M. Zielinski , D. Gershoni

We investigate theoretically the spin splitting of the exciton states in semiconductor coupled quantum dots (CQDs) containing a single magnetic ion. We find that the spin splitting can be switched on/off in the CQDs \textit{via} the…

Materials Science · Physics 2009-11-13 Xiaojing Li , Kai Chang

Current implementations of quantum bits (qubits) continue to undergo too many errors to be scaled into useful quantum machines. An emerging strategy is to encode quantum information in the two meta-stable pointer states of an oscillator…

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