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Dynamical density functional theory (DDFT) is a powerful variational framework to study the nonequilibrium properties of colloids by only considering a time-dependent one-body number density. Despite the large number of recent successes,…

Soft Condensed Matter · Physics 2021-01-13 René Wittmann , Hartmut Löwen , Joseph M. Brader

We present the exact adiabatic theory for the dynamics of the inhomogeneous density distribution of a classical fluid. Erroneous particle number fluctuations of dynamical density functional theory are absent, both for canonical and grand…

Soft Condensed Matter · Physics 2016-05-25 Daniel de las Heras , Joseph M. Brader , Andrea Fortini , Matthias Schmidt

We employ Reactive Dynamical Density Functional Theory (R-DDFT) and Reactive Brownian Dynamics (R-BD) simulations to investigate the dynamics of a suspension of active soft Gaussian colloids with binary interaction switching, i.e., a…

Soft Condensed Matter · Physics 2022-07-29 Michael Bley , Pablo I. Hurtado , Joachim Dzubiella , Arturo Moncho-Jordá

The dynamics of star polymers has been investigated via extensive Molecular- and Brownian Dynamics simulations for a large range of functionality $f$ and packing fraction $\eta$. The calculated isodiffusivity curves display both minima and…

Soft Condensed Matter · Physics 2009-11-10 G. Foffi , F. Sciortino , P. Tartaglia , E. Zaccarelli , F. Lo Verso , L. Reatto , K . A. Dawson , C. N. Likos

Based on Brownian Dynamics (BD) simulations, we study the dynamical self-assembly of active Brownian particles with dipole-dipole interactions, stemming from a permanent point dipole at the particle center. The propulsion direction of each…

Soft Condensed Matter · Physics 2021-06-09 Guo-Jun Liao , Carol K. Hall , Sabine H. L. Klapp

Simulation and experimental studies have demonstrated non-equilibrium ordering in driven colloidal suspensions: with increasing driving force, a uniform colloidal mixture transforms into a locally demixed state characterized by the lane…

Soft Condensed Matter · Physics 2024-07-16 Hiroshi Frusawa

Understanding the dynamic behavior of polar fluids is essential for modeling complex systems such as electrolytes and biological media. In this work, we develop and apply a Stochastic Density Functional Theory (SDFT) framework to describe…

Soft Condensed Matter · Physics 2025-07-23 Sleeba Varghese , Pierre Illien , Benjamin Rotenberg

Based on Dynamical Density Functional Theory (DDFT) we investigate a binary mixture of interacting Brownian particles driven over a substrate via a one-dimensional ratchet potential. The particles are modeled as soft spheres where one…

Soft Condensed Matter · Physics 2015-06-19 Ken Lichtner , Sabine H. L. Klapp

We perform detailed computational and experimental measurements of the driven dynamics of a dense, uniform suspension of sedimented microrollers driven by a magnetic field rotating around an axis parallel to the floor. We develop a…

Soft Condensed Matter · Physics 2020-07-03 Brennan Sprinkle , Ernest B. van der Wee , Yixiang Luo , Michelle Driscoll , Aleksandar Donev

Two-dimensional mixtures of dipolar colloidal particles with different dipole moments exhibit extremely rich self-assembly behaviour and are relevant to a wide range of experimental systems, including charged and super-paramagnetic colloids…

Soft Condensed Matter · Physics 2019-04-16 W. R. C. Somerville , J. L. Stokes , A. M. Adawi , T. S. Horozov , A. J. Archer , D. M. A. Buzza

The phoretic Brownian dynamics method is shown here to be an effective approach to simulate the properties of colloidal chemophoretic based systems. The method is then optimized to allow for the comparison with results from multiparticle…

Soft Condensed Matter · Physics 2024-06-17 Surabhi Jaiswal , Marisol Ripoll , Snigdha Thakur

We have developed a lab work module where we teach undergraduate students how to quantify the dynamics of a suspension of microscopic particles, measuring and analyzing the motion of those particles at the individual level or as a group.…

Soft Condensed Matter · Physics 2016-02-23 David Germain , Mathieu Leocmach , Thomas Gibaud

Equilibrium polyethylene crystal structure, cohesive energy, and elastic constants are calculated by density-functional theory applied with a recently proposed density functional (vdW-DF) for general geometries [Phys. Rev. Lett. 92, 246401…

Materials Science · Physics 2009-11-11 Jesper Kleis , Bengt I. Lundqvist , David C. Langreth , Elsebeth Schroder

The motion of a particle under the influence of a dynamical disorder is described by the DLD model. One motivation is to understand the motion of an electron inside a metal; Another is to understand quantal Brownian motion. The overview is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Doron Cohen

We present dynamical density functional theory results for the time evolution of the density distribution of a sedimenting model two-dimensional binary mixture of colloids. The interplay between the bulk phase behaviour of the mixture, its…

Soft Condensed Matter · Physics 2015-06-17 Alexandr Malijevsky , Andrew J. Archer

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

Dynamic force spectroscopy (DFS) is an experimental technique that is commonly used to assess information of the strength, energy landscape, and lifetime of noncovalent bio-molecular interactions. DFS traditionally requires an applied force…

Biological Physics · Physics 2016-07-04 Oscar Björnham , Magnus Andersson

Odd diffusion breaks time-reversal symmetry in overdamped systems through transverse probability currents while preserving equilibrium steady states. In this work, we develop a dynamical density functional theory (DDFT) for dense…

Soft Condensed Matter · Physics 2026-02-02 Iman Abdoli , René Wittmann , Hartmut Löwen

Density-dependent diffusion is a widespread phenomenon in nature. We have examined the density-dependent diffusion behavior of some biological processes such as tumor growth and invasion [23]. Here, we extend our previous work by developing…

Statistical Mechanics · Physics 2022-02-14 Ahmed M. Fouad , Marwa M. Fouad

The connection between fundamental interactions acting in molecules in a fluid and macroscopically measured properties, such as the viscosity between colloidal particles coated with polymers, is studied here. The role that hydrodynamic and…

Soft Condensed Matter · Physics 2015-09-02 A. Gama Goicochea , M. A. Balderas Altamirano , R. Lopez-Esparza , M. A. Waldo , E. Perez