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We have shown that the observed large reduction of the effective moment in Na2V3O7 may be caused by conventional crystal-field interactions and the intra-atomic spin-orbit coupling of the V4+ ion. The fine discrete electronic structure of…

Strongly Correlated Electrons · Physics 2015-06-24 Z. Ropka , R. J. Radwanski

We have shown that the observed drastic violation of the Curie-Weiss law in Na2V3O7, reported in Phys. Rev. Lett. 90 (2003) 167202, is caused by conventional crystal-field interactions and the intra-atomic spin-orbit coupling of the V4+…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

We contest the interpretation by Gavilano et al. (Phys.Rev.Lett. 90 (2003) 167202) of violation of the Curie law behavior of the paramagnetic susceptibility at low temperatures by means of the quenching of the V4+-ion moment. These results…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

The orbital and spin moment of the Ni2+ ion in NiO has been calculated at 0 K to be 0.54mB and 1.99 mB respectively. Such large orbital moment, more than 20% of the total moment of 2.53 mB, proves the need for the ''unquenching'' of the…

Strongly Correlated Electrons · Physics 2023-06-21 R. J. Radwanski , Z. Ropka

We consider spin-orbit coupling effects in Na$_4$Ir$_3$O$_8$, a material in which Ir$^{4+}$ spins form an hyper-kagom\'{e} lattice, a three-dimensional network of corner-sharing triangles. We argue that both low temperature thermodynamic…

Strongly Correlated Electrons · Physics 2008-10-03 Gang Chen , Leon Balents

It has recently been proposed that Na4Ir3O8 is a weak Mott insulator at ambient pressure, supporting a three-dimensional spin liquid phase with a spinon Fermi surface. This proposal is consistent with recent experimental findings that the…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Yong Baek Kim

The superconducting pyrochlore oxide Cd2Re2O7 shows a structural transition with inversion symmetry breaking (ISB) at Ts1 = 200 K. A recent theory [L. Fu, Phys. Rev. Lett. 115, 026401 (2015)] suggests that the origin is an electronic…

BaRuO3 having five different crystal structures has been synthesized by varying the pressure while sintering. Contrary to the other phases being nonmagnetic, the cubic perovskite phase synthesized recently shows an itinerant ferromagnetic…

Materials Science · Physics 2014-05-20 Young-Joon Song , K. -W. Lee

We have described properties of LiCoO_2 within the Quantum Atomistic Solid State (QUASST) theory taking into account very strong electron correlations, predominantly of the intra-atomic origin, spin-orbit coupling and the detailed local…

Strongly Correlated Electrons · Physics 2008-10-08 R. J. Radwanski , Z. Ropka

It has been shown that for the highly-correlated d4 electronic system the spin-orbit interactions produce, even in case of the cubic crystal-field interactions, a singlet ground state. Its magnetic moment grows rapidly with the applied…

Strongly Correlated Electrons · Physics 2008-10-08 R. J. Radwanski , Z. Ropka

Spin-orbit coupling in crystals is known to lead to unusual direction dependent exchange interactions, however understanding of the consequeces of such effects in molecular crystals is incomplete. Here we perform four component relativistic…

Strongly Correlated Electrons · Physics 2017-04-19 A. C. Jacko , A. L. Khosla , J. Merino , B. J. Powell

Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se)…

In FeSc2S4 spin-orbital exchange competes with strong spin-orbit coupling, suppressing long-range spin and orbital order and, hence, this material represents one of the rare examples of a spin-orbital liquid ground state. Moreover, it is…

Strongly Correlated Electrons · Physics 2015-06-22 L. Mittelstädt , M. Schmidt , Zhe Wang , F. Mayr , V. Tsurkan , P. Lunkenheimer , D. Ish , L. Balents , J. Deisenhofer , A. Loidl

The spin-orbit interaction lies at the heart of quantum computation with spin qubits, research on topologically non-trivial states, and various applications in spintronics. Hole spins in Ge/Si core/shell nanowires experience a spin-orbit…

The orbital and spin moment of the Co2+ ion in CoO has been calculated within the quasi-atomic approach with taking into account the intra-atomic spin-orbit coupling and crystal field interactions. The orbital moment of 1.38 m_B amounts at…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

A pronounced Curie-like upturn of the magnetic susceptibility chi(T) of the quasi one-dimensional spin chain compound Ba2V3O9 has been found recently. Frequently this is taken as a signature for a staggered field mechanism due to the…

Strongly Correlated Electrons · Physics 2009-11-07 B. Schmidt , V. Yushankhai , L. Siurakshina , P. Thalmeier

Contrary to the well known spin qubits, rare-earth qubits are characterized by a strong influence of crystal field due to large spin-orbit coupling. At low temperature and in the presence of resonance microwaves, it is the magnetic moment…

Strongly Correlated Electrons · Physics 2009-11-26 Sylvain Bertaina , J. H. Shim , S. Gambarelli , B. Z. Malkin , B. Barbara

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

Spin-orbit coupling links a particle's velocity to its quantum mechanical spin, and is essential in numerous condensed matter phenomena, including topological insulators and Majorana fermions. In solid-state materials, spin-orbit coupling…

Quantum Gases · Physics 2013-12-12 Victor Galitski , Ian B. Spielman

We review recent theoretical developments about the role of spins, electron-electron interactions, and spin-orbit coupling in metal nanoparticles and semiconductor quantum dots. For a closed system, in the absence of spin-orbit coupling or…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yuval Oreg , P. W. Brouwer , X. Waintal , Bertrand I. Halperin
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