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By means of a molecular model, we examine hybrid nematic films with antagonistic anchoring angles where one of the surfaces is in the strong anchoring regime. If anchoring at the other surface is weak, and in the absence of wetting by the…

Soft Condensed Matter · Physics 2010-12-17 D. de las Heras , L. Mederos , E. Velasco

Using a generalisation of an Onsager type approach, we are able to predict a dielectric permittivity profile of an inhomogeneous dipolar fluid in the presence of a dielectric interface. The reaction and cavity fields are calculated…

Soft Condensed Matter · Physics 2009-11-10 Reimar Finken , Vincent Ballenegger , Jean-Pierre Hansen

The celebrated work of Onsager on hard particle systems, based on the truncated second order virial expansion, is valid at relatively low volume fractions for large aspect ratio particles. While it predicts the isotropic-nematic phase…

Soft Condensed Matter · Physics 2017-08-16 Eduardo S. Nascimento , Peter Palffy-Muhoray , Jamie M. Taylor , Epifanio G. Virga , Xiaoyu Zheng

Excess contributions to the free energy due to interfaces occur for many problems encountered in the statistical physics of condensed matter when coexistence between different phases is possible (e.g. wetting phenomena, nucleation, crystal…

Statistical Mechanics · Physics 2015-05-27 Kurt Binder , Benjamin Block , Subir K. Das , Peter Virnau , David Winter

Thermally excited capillary waves at fluid interfaces in binary liquid mixtures exhibit simultaneously both density and composition fluctuations. Based on a density functional theory for inhomogeneous binary liquid mixtures we derive an…

Soft Condensed Matter · Physics 2009-11-11 Thorsten Hiester , S. Dietrich , Klaus Mecke

We present a large-scale molecular dynamics study of nematic-paranematic interfaces under shear. We use a model of soft repulsive ellipsoidal particles with well-known equilibrium properties, and consider interfaces which are oriented…

Soft Condensed Matter · Physics 2013-03-19 Guido Germano , Friederike Schmid

We investigate fluids of dipolar hard particles by a certain variant of density-functional theory. The proper treatment of the long range of the dipolar interactions yields a contribution to the free energy which favors ferromagnetic order.…

Condensed Matter · Physics 2009-10-28 B. Groh , S. Dietrich

Binary fluid mixtures are examples of complex fluids whose microstructure and flow are strongly coupled. For pairs of simple fluids, the microstructure consists of droplets or bicontinuous demixed domains and the physics is controlled by…

Soft Condensed Matter · Physics 2018-06-05 Michael E. Cates , Elsen Tjhung

We examine the ordering properties of rectangular hard rods with length L and diameter D at a single planar wall and between two parallel hard walls using the second-virial density functional theory. The theory is implemented in the…

Soft Condensed Matter · Physics 2016-02-17 R. Aliabadi , M. Moradi , S. Varga

In the framework of a field theoretical approach we study Maier-Saupe nematogenic fluid in contact with a hard wall. The pair interaction potential of the considered model consists of an isotropic and an anisotropic Yukawa terms. In the…

Soft Condensed Matter · Physics 2013-03-25 M. Holovko , I. Kravtsiv , D. di Caprio

We revisit the classic problem of the structure of the isotropic-nematic interface within Ginzburg-Landau-de Gennes theory, refining previous analytic treatments of biaxiality at the interface. We compare our analysis with numerical results…

Soft Condensed Matter · Physics 2015-05-13 S. M. Kamil , A. K. Bhattacharjee , R. Adhikari , Gautam I. Menon

We apply a modified mean-field density functional theory to determine the phase behavior of binary mixtures of Stockmayer fluids whose spherical constituents interact according to Lennard-Jones (LJ) pair potentials with embedded pointlike…

Soft Condensed Matter · Physics 2009-11-11 I. Szalai , S. Dietrich

Polyhedral nematics are examples of exotic orientational phases that possess a complex internal symmetry, representing highly non-trivial ways of rotational symmetry breaking, and are subject to current experimental pursuits in colloidal…

Statistical Mechanics · Physics 2018-01-29 Ke Liu , Jonas Greitemann , Lode Pollet

We study a diffuse interface model describing the complex rheology and the interfacial dynamics during phase separation in a polar liquid-crystalline emulsion. More precisely, the physical systems comprises a two-phase mixture consisting in…

Analysis of PDEs · Mathematics 2024-06-27 Giulia Bevilacqua , Andrea Giorgini

We show that surface interactions can vectorially structure the three-dimensional polariza-tion field of a ferroelectric fluid. The contact between a ferroelectric nematic liquid crystal and a surface with in-plane polarity generates a…

Soft Condensed Matter · Physics 2024-01-19 Xi Chen , Eva Korblova , Matthew A. Glaser , Joseph E. Maclennan , David M. Walba , Noel A. Clark

We consider the phase separation of binary fluids in contact with a surface which is preferentially wetted by one of the components of the mixture. We review the results available for this problem and present new numerical results obtained…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea , Sanjay Puri , Joel L. Lebowitz

We analyze the interplay between wetting and anchoring of nematic liquid crystals on disordering, e.g., rough substrates in the framework of the Landau-de Gennes theory, in situations of competing homeotropic and planar easy axes on the…

Soft Condensed Matter · Physics 2010-02-23 Friederike Schmid , David L. Cheung

We present an experimental study of the isotropic-nematic phase transition in an aqueous mixture of charged semi-flexible rods (fd virus) and neutral polymer (Dextran). A complete phase diagram is measured as a function of ionic strength…

Soft Condensed Matter · Physics 2009-11-10 Zvonimir Dogic , Kirstin Purdy , Eric Grelet , Marie Adams , Seth Fraden

The phase behavior of rodlike molecules with polydisperse length and solvent-mediated attraction and repulsion is described by an extension of the Onsager theory for rigid rods. A phenomenological square-well potential is used to model…

Soft Condensed Matter · Physics 2015-05-13 Micah J. Green , A. Nicholas G. Parra-Vasquez , Natnael Behabtu , Matteo Pasquali

Barrier planes described by the Ionic Hubbard model and sandwiched between metallic planes on both sides are studied using unrestricted Hartree Fock. For zero onsite correlation, the presence of the metallic interface generates an…

Strongly Correlated Electrons · Physics 2011-04-20 Tribikram Gupta , Sanjay Gupta