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The electronic properties of quarter-filled organic materials showing spin-Peierls transition are investigated theoretically. By studying the one-dimensional extended Peierls-Hubbard model analytically as well as numerically, we find that…

Strongly Correlated Electrons · Physics 2007-05-23 Makoto Kuwabara , Hitoshi Seo , Masao Ogata

A charge density wave (CDW) ground state is observed in polycrystalline Cu$_2$Se below 125 K, which corresponds to an energy gap of 40.9 meV and an electron-phonon coupling constant of 0.6. Due to the polycrystalline structure, the Peierls…

Materials Science · Physics 2014-11-06 Mengliang Yao , Weishu Liu , Xiang Chen , Zhensong Ren , Stephen Wilson , Zhifeng Ren , Cyril P. Opeil

We have investigated the charge dynamics and the nature of many-body interactions in La- and Pr- doped CaFe2As2. From the infrared part of the optical conductivity, we discover that the scattering rate of mobile carriers above 200 K…

Using a combination of resistance fluctuation (noise) and dielectric spectroscopy we investigate the nature of relaxor-type electronic ferroelectricity in the organic conductor $\kappa$-(BETS)$_2$Mn[N(CN)$_2$]$_3$, a system representative…

Titanyl-phthalocyanines catalytic ability towards oxygen reduction is demonstrated in experimental literature. Our recent theoretical simulations revealed electronic structure origin of catalytic ability in peripherally and axially…

Materials Science · Physics 2016-11-01 Jeffrey R. De Lile , Su Zhou

The behavior of three-dimensional (3D) semimetals under strong magnetic fields is a topic of recurring interest in condensed matter physics. Recently, the advent of Weyl and Dirac semimetals has brought about an interesting platform for…

Strongly Correlated Electrons · Physics 2022-05-11 Sarbajaya Kundu , Claude Bourbonnais , Ion Garate

We study theoretically the shift of the superconducting transition temperature (Tc) under uniaxial compression in beta-type organic superconductors, beta-(BEDT-TTF)2I3 and beta-(BDA-TTP)2X[X=SbF6,AsF6], in order to clarify the electron…

Superconductivity · Physics 2015-05-19 Takeo Suzuki , Seiichiro Onari , Hiroshi Ito , Yukio Tanaka

In one-dimensional quantum materials, conducting electrons and the underlying lattices can undergo a spontaneous translational symmetry breaking, known as Peierls transition. For nearly a century, the Peierls transition has been understood…

Fluctuating-charge models are computationally efficient methods of treating polarization and charge-transfer phenomena in molecular mechanics and classical molecular dynamics simulations. They are also theoretically appealing as they are…

Chemical Physics · Physics 2010-04-02 Jiahao Chen

The multiband nature of iron pnictides gives rise to a rich temperature-doping phase diagram of competing orders and a plethora of collective phenomena. At low dopings, the tetragonal-to-orthorhombic structural transition is closely…

Superconductivity · Physics 2016-02-18 V. K. Thorsmølle , M. Khodas , Z. P. Yin , Chenglin Zhang , S. V. Carr , Pengcheng Dai , G. Blumberg

We investigate a series of liquid-crystalline phthalocyanines (metal-free and Cu, Zn, Ni, Co complexes) by correlating their vibrational signatures with their electronic performance in organic thin-film transistors (OTFTs). Raman…

We address the question of the origin of the recently discovered chiral property of the charge-density-wave phase in 1$T$-TiSe$_2$ which so far lacks a microscopic understanding. We argue that the lattice degrees of freedom seems to be…

Strongly Correlated Electrons · Physics 2015-06-15 B. Zenker , H. Fehske , H. Beck , C. Monney , A. R. Bishop

To elucidate different photoinduced melting dynamics of charge orders observed in quasi-two-dimensional organic conductors $ \theta $-(BEDT-TTF)$_2$RbZn(SCN)$_4$ and $ \alpha $-(BEDT-TTF)$_2$I$_3$…

Strongly Correlated Electrons · Physics 2010-03-11 Satoshi Miyashita , Yasuhiro Tanaka , Shinichiro Iwai , Kenji Yonemitsu

In strongly correlated organic materials it has been pointed out that charge-ordering could also achieve electronic ferroelectricity at the same critical temperature $T_{co}$. A prototype of such phenomenon are the quasi-one dimensional…

Strongly Correlated Electrons · Physics 2018-01-18 Mariano de Souza , Lucas Squillante , Cesar Sônego , Paulo Menegasso , Pascale Foury-Leylekian , Jean-Paul Pouget

Phase competition and excitations in the one-dimensional neutral-ionic transition systems are theoretically studied comprehensively. From the semiclassical treatment of the bosonized Hamiltonian, we examine the competition among the neutral…

Strongly Correlated Electrons · Physics 2016-09-12 Masahisa Tsuchiizu , Hideo Yoshioka , Hitoshi Seo

Photoinduced phase transitions and charge dynamics in the interacting Dirac-electron system with a charge-ordered ground state are theoretically studied by taking an organic salt $\alpha$-(BEDT-TTF)$_2$I$_3$. By analysing the extended…

Strongly Correlated Electrons · Physics 2022-07-21 Yasuhiro Tanaka , Masahito Mochizuki

The family of molecular conductors TMTTF/TMTSF-X demonstrates almost all known electronic phases in parallel with a set of weak structural modifications of anion ordering and mysterious structureless transitions. Only in early 2000's their…

Strongly Correlated Electrons · Physics 2007-05-23 Serguei Brazovskii

The ultrafast dynamics of charge carriers in organic donor-acceptor interfaces are of primary importance to understanding the fundamental properties of these systems. In this work, we focus on a charge-transfer complex formed by…

Materials Science · Physics 2023-10-23 Matheus Jacobs , Jannis Krumland , Ana M. Valencia , Caterina Cocchi

Among the mechanisms for lattice structural deformation, the electron-phonon interaction mediated Peierls charge-density-wave (CDW) instability in single band low-dimensional systems is perhaps the most ubiquitous. The standard mean-field…

Strongly Correlated Electrons · Physics 2009-11-11 Sanjoy Datta , Sudhakar Yarlagadda

We discuss the properties of fluctuations of the electric charge in the vicinity of the chiral crossover transition within effective chiral models at finite temperature and vanishing net baryon density. The calculation includes…

High Energy Physics - Phenomenology · Physics 2015-05-30 V. Skokov , B. Friman , K. Redlich