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We report momentum resolved charge excitations in a one dimensional (1-D) Mott insulator studied using high resolution (~ 325 meV) inelastic x-ray scattering over the entire Brillouin zone for the first time. Excitations at the insulating…

Strongly Correlated Electrons · Physics 2007-05-23 M. Z. Hasan , P. A. Montano , E. D. Isaacs , Z-X. Shen , H. Eisaki , S. K. Sinha , Z. Islam , N. Motoyama , S. Uchida

Using high-resolution resonant inelastic x-ray scattering (RIXS), we performed a momentum-resolved study of magnetic excitations in the model spin-1/2 2D antiferromagnetic insulator Sr_2CuCl_2O_2. We identify both a single-spin-wave feature…

We report a resonant inelastic x-ray scattering study of the dispersion relations of charge transfer excitations in insulating La$_2$CuO$_4$. These data reveal two peaks, both of which show two-dimensional characteristics. The lowest energy…

Strongly Correlated Electrons · Physics 2009-11-07 Y. J. Kim , J. P. Hill , C. A. Burns , S. Wakimoto , R. J. Birgeneau , D. Casa , T. Gog , C. T. Venkataraman

The electronic structure of Mott insulators continues to be a major unsolved problem in physics despite more than half-century of intense research efforts. Well-developed momentum-resolved spectroscopies such as photoemission or neutron…

Strongly Correlated Electrons · Physics 2009-11-07 M. Z. Hasan , E. D. Isaacs , Z-X. Shen , L. L. Miller , K. Tsutsui , T. Tohyama , S. Maekawa

We have measured the magnetic excitation spectrum of the model square-lattice spin-1/2 antiferromagnet $\rm Sr_2CuO_2Cl_2$ over a broad range of energy and momentum using high-resolution inelastic neutron scattering (INS). The magnon…

Strongly Correlated Electrons · Physics 2015-06-18 K. W. Plumb , A. T. Savici , G. E. Granroth , F. C. Chou , Young-June Kim

We report a Cu K-edge resonant inelastic x-ray scattering (RIXS) study of high-Tc cuprates. Momentum-resolved charge excitations in the CuO2 plane are examined from parent Mott insulators to carrier-doped superconductors. The Mott gap…

We calculate the resonant inelastic X-ray scattering (RIXS) response in a Mott insulator which is described by the Falicov-Kimball model. The model can be solved exactly within the single site dynamical mean-field theory (DMFT)…

Strongly Correlated Electrons · Physics 2015-03-31 Nandan Pakhira , J. K. Freericks , A. M. Shvaika

We report particle-hole pair excitations in a cuprate insulator in the intermediate regimes of momentum-transfers using high energy inelastic x-ray scattering. The excitation spectra show dispersive features near the Mott edge which shed…

Strongly Correlated Electrons · Physics 2009-11-07 M. Z. Hasan , E. D. Isaacs , Z-X. Shen , L. L. Miller

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

Strongly Correlated Electrons · Physics 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

We report the first observation of soft-x-ray scattering from spin fluctuations in a high-Tc parent compound. An antiferromagnetic charge transfer insulator, CaCuO2, was irradiated by Cu M-edge soft x-rays. Ultra-high resolution…

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

Core hole resonance is used in X-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic X-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators…

Strongly Correlated Electrons · Physics 2016-12-14 L. Andrew Wray , Shih-Wen Huang , Yuqi Xia , M. Zahid Hasan , Charles Mathy , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We investigate the dynamical spin and charge structure factors and the one-particle spectral function of the one-dimensional extended Hubbard model at half band-filling using the dynamical density-matrix renormalization group method. The…

Strongly Correlated Electrons · Physics 2009-11-11 H. Benthien , E. Jeckelmann

Quantum fluctuations in low-dimensional systems and near quantum phase transitions have significant influences on material properties. Yet, it is difficult to experimentally gauge the strength and importance of quantum fluctuations. Here we…

We investigate the resonant two-magnon Raman scattering in two-dimensional (2D) Mott insulators by using a half-filled 2D Hubbard model in the strong coupling limit. By performing numerical diagonalization calculations for small clusters,…

Strongly Correlated Electrons · Physics 2007-05-23 T. Tohyama , H. Onodera , K. Tsutsui , S. Maekawa

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

Superconductivity · Physics 2015-06-15 S. Wakimoto , K. Ishii , H. Kimura , K. Ikeuchi , M. Yoshida , T. Adachi , D. Casa , M. Fujita , Y. Fukunaga , T. Gog , Y. Koike , J. Mizuki , K. Yamada

We establish the spectral line shape of orbital excitations created by resonant inelastic X-ray scattering for the model Mott insulator CoO. Improved experimental energy resolution reveals that the line shapes are strikingly different from…

Strongly Correlated Electrons · Physics 2015-06-18 L. Andrew Wray , J. Li , Z. Q. Qiu , Jinsheng Wen , Zhijun Xu , Genda Gu , Shih-Wen Huang , Elke Arenholz , Wanli Yang , Zahid Hussain , Yi-De Chuang

We report on the study of the magnetic excitations of Mott insulator La2CuO4 by using resonant inelastic x-ray scattering (RIXS) and cluster calculations within the framework of exact diagonalization. Our results demonstrate experimentally…

Strongly Correlated Electrons · Physics 2025-10-06 A. Singh , H. Y. Huang , K. Tsutsui , T. Tohyama , S. Komiya , J. Okamoto , C. T. Chen , A. Fujimori , D. J. Huang

Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen, but can be activated by photodoping. The energy-momentum distribution of…

Strongly Correlated Electrons · Physics 2020-04-23 Yao Wang , Yuan Chen , Chunjing Jia , Brian Moritz , Thomas P. Devereaux
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