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It has been demonstrated recently that supercooled liquids sharing simple structural features (e.g. pair distribution functions) may exhibit strikingly distinct dynamical behavior. Here we show that a more subtle structural feature…

Statistical Mechanics · Physics 2012-06-04 Glen M. Hocky , Thomas E. Markland , David R. Reichman

The structural relaxation, potential energy states, and mechanical properties of a model glass subjected to thermal cycling are investigated using molecular dynamics simulations. We study a non-additive binary mixture which is annealed with…

Soft Condensed Matter · Physics 2018-12-05 Nikolai V. Priezjev

Puzzling observations of both thermal and dielectric responses in multi-silicate glasses at low temperatures $T$ to static magnetic fields $B$ have been reported in the last decade and call for an extension of the standard two-level systems…

Disordered Systems and Neural Networks · Physics 2015-05-13 Giancarlo Jug

A broad fundamental understanding of the mechanisms underlying the phenomenology of supercooled liquids has remained elusive, despite decades of intense exploration. When supercooled beneath its characteristic melting temperature, a liquid…

Soft Condensed Matter · Physics 2016-11-10 Nicholas B. Weingartner , Chris Pueblo , Flavio S. Nogueira , K. F. Kelton , Zohar Nussinov

We define the heat capacity for steady periodically driven systems and as an example we compute it for dissipative two-level systems where the energy gap is time-modulated. There, as a function of ambient temperature, the Schottky peak…

Statistical Mechanics · Physics 2024-08-27 Elena Rufeil Fiori , Christian Maes

The heat flow between a quantum system and its reservoir is analyzed when initially both are in a separable thermal state and asymptotically approach a correlated equilibrium. General findings are illustrated for specific systems and…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Joachim Ankerhold , Jukka P. Pekola

We performed parallel study of calorimetric and high-frequency shear modulus behavior of Zr-based metallic glasses after deep relaxation just below the glass transition. It is shown that deep relaxation results in the appearance of a strong…

Disordered Systems and Neural Networks · Physics 2025-03-07 A. S. Makarov , G. V. Afonin , R. A. Konchakov , J. C. Qiao , N. P. Kobelev , V. A. Khonik

The Mpemba effect denotes an anomalous relaxation phenomenon where a system initially at a hot temperature cools faster than a system that starts at a less elevated temperature. We introduce an isothermal analog of this effect for a system…

Statistical Mechanics · Physics 2022-09-02 Julius Degünther , Udo Seifert

In this paper the phenomenon of dynamic heterogeneity in supercooled liquid systems is considered in terms of the recently proposed gauge theory of glass transition. The physical interpretation of the dynamic scaling is considered. It is…

Statistical Mechanics · Physics 2015-06-23 Mikhail Vasin

The standard model of glasses is an ensemble of two-level systems interacting with a thermal bath. The general origin of memory effects in this model is a quasi-stationary but non-equilibrium state of a single two-level system, which is…

Disordered Systems and Neural Networks · Physics 2009-11-13 Gerardo Aquino , Armen Allahverdyan , Theo M. Nieuwenhuizen

We develop a theory of the effective disorder temperature in glass-forming materials driven away from thermodynamic equilibrium by external forces. Our basic premise is that the slow configurational degrees of freedom of such materials are…

Materials Science · Physics 2015-05-13 Eran Bouchbinder , J. S. Langer

Liquid water exhibits anomalous behavior in the supercooled region. A popular hypothesis to explain supercooled water's anomalies is the existence of a metastable liquid-liquid transition terminating at a critical point. The hypothesized…

Chemical Physics · Physics 2020-01-08 V. P. Voronov , V. E. Podnek , M. A. Anisimov

Dielectric relaxation spectroscopy (1 Hz - 20 GHz) has been performed on supercooled glass-formers from the temperature of glass transition (T_g) up to that of melting. Precise measurements particularly in the frequencies of MHz-order have…

Disordered Systems and Neural Networks · Physics 2009-11-07 Takuya Fujima , Hiroshi Frusawa , Kohzo Ito

Given the vast differences in interaction details, describing the dynamics of structurally disordered materials in a unified theoretical framework presents a fundamental challenge to condensed-matter physics and materials science. Here, we…

Soft Condensed Matter · Physics 2025-08-12 Liang Gao , Hai-Bin Yu , Thomas B. Schrøder , Jeppe C. Dyre

Tackling the low-temperature fate of supercooled liquids is challenging due to the immense timescales involved, which prevent equilibration and lead to the operational glass transition. Relating glassy behaviour to an underlying,…

Statistical Mechanics · Physics 2017-08-16 Francesco Turci , C. Patrick Royall , Thomas Speck

In order to understand the mechanisms for glassy dynamics in biological tissues and shed light on those in non-biological materials, we study the low-temperature disordered phase of 2D vertex-like models. Recently it has been noted that…

Soft Condensed Matter · Physics 2018-05-09 Daniel M. Sussman , M. Paoluzzi , M. Cristina Marchetti , M. Lisa Manning

Soft glassy materials are out of thermodynamic equilibrium and show time dependent slowing down of the relaxation dynamics. Under such situation these materials follow Boltzmann superposition principle only in the effective time domain,…

Soft Condensed Matter · Physics 2012-03-27 Rahul Gupta , Bharat Baldewa , Yogesh M. Joshi

Glasses and disordered materials are known to display anomalous features in the density of states, in the specific heat and in thermal transport. Nevertheless, in recent years, the question whether these properties are really anomalous (and…

Disordered Systems and Neural Networks · Physics 2021-03-26 Matteo Baggioli , Alessio Zaccone

It has been shown that the dependence of thermal expansion coefficient and of the isobaric heat capacity of supercooled water on the temperature contradicts to an important thermodynamic relation. Keywords: Supercooled water, Negative…

General Physics · Physics 2009-09-29 I. A. Stepanov

Studying the primary {\alpha}- and secondary {\beta}-relaxation process has contributed significantly to the understanding of the structure and rheology of metallic glasses. In this letter, we report on a third relaxation mechanism…

Materials Science · Physics 2017-03-28 Stefan Küchemann , Robert Maaß
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