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Related papers: Unrestricted Hartree-Fock for Quantum Dots

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We perform unrestricted Hartree-Fock (HF) calculations for electrons in a parabolic quantum dot at zero magnetic field. The crossover from Fermi liquid to Wigner molecule behavior is studied for up to eight electrons and various spin…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Boris Reusch , Wolfgang Häusler , Hermann Grabert

Wigner molecules formed at high magnetic fields in circular and elliptic quantum dots are studied by exact diagonalization (ED) and unrestricted Hartree-Fock (UHF) methods with multicenter basis of displaced lowest Landau level wave…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 B. Szafran , F. M. Peeters , S. Bednarek , J. Adamowski

The stretching of closed-shell molecules is a qualitative problem for restricted Hartree-Fock that is usually circumvented by the use of unrestricted Hartree-Fock (UHF). UHF is well known to break the spin symmetry at the Coulson-Fischer…

Chemical Physics · Physics 2015-06-23 Paula Mori-Sánchez , Aron J. Cohen

Few-electron systems confined in two-dimensional parabolic quantum dots at high magnetic fields are studied by the Hartree-Fock (HF) and exact diagonalization methods. A generalized multicenter Gaussian basis is proposed in the HF method. A…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 B. Szafran , S. Bednarek , J. Adamowski , M. B. Tavernier , E. Anisimovas , F. M. Peeters

Restricted open-shell Hartree-Fock (ROHF) theory is formulated as a projected self-consistent unrestricted HF (UHF) model by mathematically constraining spin density eigenvalues. The resulting constrained UHF (CUHF) wave function is…

Strongly Correlated Electrons · Physics 2015-05-19 Takashi Tsuchimochi , Gustavo E. Scuseria

The ground states of the two-dimensional repulsive Hubbard model are studied within the unrestricted Hartree-Fock (UHF) theory. Magnetic and charge properties are determined by systematic, large-scale, exact numerical calculations, and…

Strongly Correlated Electrons · Physics 2013-09-20 Jie Xu , Chia-Chen Chang , Eric J. Walter , Shiwei Zhang

The ground-state Hartree-Fock (HF) wavefunction of the Hooke's atom is not known in closed form, contrary to the exact solution. The single HF orbital involved has thus far been studied using expansion techniques only, leading to slightly…

Atomic Physics · Physics 2008-05-05 Ragot Sebastien

We present unrestricted Hartree Fock method coupled with configuration interaction (CI) method (URHF-CI) suitable for the calculation of ground and excited states of large number of electrons localized by complex gate potentials in…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Ramin M. Abolfath , Pawel Hawrylak

Ground state energies are obtained using the unrestricted Hartree Fock method for up to four interacting electrons parabolically confined in a quantum dot subject to a magnetic field. Restoring spin and rotational symmetries we recover Hund…

Mesoscale and Nanoscale Physics · Physics 2011-10-10 U. De Giovannini , F. Cavaliere , R. Cenni , M. Sassetti , B. Kramer

We use different types of determinantal Hartree-Fock (HF) wave functions to calculate variational bounds for the ground state energy of spin-half fermions in volume V_0, with mass m, electric charge zero, and magnetic moment mu, which are…

Strongly Correlated Electrons · Physics 2008-11-26 Sudhanshu S. Jha , S. D. Mahanti

L\"owdin's symmetry dilemma is an ubiquitous issue in approximate quantum chemistry. In the context of Hartree-Fock (HF) theory, the use of Slater determinants with some imposed constraints to preserve symmetries of the exact problem may…

Chemical Physics · Physics 2021-07-22 Leonardo A. Cunha , Joonho Lee , Diptarka Hait , C. William McCurdy , Martin Head-Gordon

We demonstrate that unrestricted Hartree-Fock theory applied to electrons in a uniform potential has stable Wigner crystal solutions for $r_s \geq 1.44$ in two dimensions and $r_s \geq 4.5$ in three dimensions. The correlation energies of…

Materials Science · Physics 2009-10-01 J. R. Trail , M. D. Towler , R. J. Needs

We report results for the ground state energies and wave functions obtained by projecting spatially unrestricted Hartree Fock states to eigenstates of the total spin and the angular momentum for harmonic quantum dots with $N\leq 12$…

Mesoscale and Nanoscale Physics · Physics 2011-10-10 U. De Giovannini , F. Cavaliere , R. Cenni , M. Sassetti , B. Kramer

We study $N$ interacting massless Dirac fermions confined in a two-dimensional quantum dot. Physical realizations of this problem include a graphene monolayer and the surface state of a strong topological insulator. We consider both a…

Mesoscale and Nanoscale Physics · Physics 2011-02-15 Tomi Paananen , Reinhold Egger , Heinz Siedentop

We calculate ground state energies in the Brueckner-Hartree-Fock theory for $N$ electrons (with $N\le 20$) confined to a circular quantum dot and in presence of a static magnetic field. Comparison with the predictions of Hartree-Fock,…

Strongly Correlated Electrons · Physics 2007-05-23 A. Emperador , E. Lipparini , Ll. Serra

The Hartree-Fock (HF) wave function, commonly used for approximating molecular ground states, becomes nonideal in open shell systems due to the inherent multi-configurational nature of the wave function, limiting accuracy in Quantum…

Chemical Physics · Physics 2026-02-23 Pawan Sharma Poudel , Kenji Sugisaki , Michal Hajdušek , Rodney Van Meter

We consider circular and elliptic quantum dots with parabolic external confinement, containing 0 - 22 electrons and with values of r_s in the range 0 < r_s < 3. We perform restricted and unrestricted Hartree-Fock calculations, and further…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Clare Sloggett , Oleg Sushkov

We present a group theoretical study of the symmetry-broken unrestricted Hartree-Fock orbitals and electron densities in the case of a two-dimensional N-electron single quantum dot (with and without an external magnetic field). The breaking…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Constantine Yannouleas , Uzi Landman

We assess the utility of Hartree-Fock (HF) trial wavefunctions in performing phaseless auxiliary-field quantum Monte Carlo (ph-AFQMC) on the uniform electron gas (UEG) model. The combination of ph-AFQMC with spin-restricted HF…

Chemical Physics · Physics 2019-08-20 Joonho Lee , Fionn D. Malone , Miguel A. Morales

Our previously developed Constrained-Pairing Mean-Field Theory (CPMFT) is shown to map onto an Unrestricted Hartree-Fock (UHF) type method if one imposes a corresponding pair constraint to the correlation problem that forces occupation…

Strongly Correlated Electrons · Physics 2015-05-19 Takashi Tsuchimochi , Thomas M. Henderson , Gustavo E. Scuseria , Andreas Savin
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