Related papers: Linear and Second-order Optical Response from Firs…
Super- and subradiance are usually described in the framework of Dicke collective states, which is an ``atomic picture'' in which the electromagnetic field only provides an effective interaction between the atoms. Here, we discuss a…
We present in detail the formulation of the ab initio theory we have developed for the calculation of the macroscopic second-order susceptibility $\chi^{(2)}$. We find a general expression for $\chi^{(2)}$ valid for any fields, containing…
We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…
Classical optical frameworks such as the discrete dipole approximation (DDA) assume that the linear spectrum of coupled quantum emitters can be computed solely from the linear susceptibilities of individual constituents. However, recent…
Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a…
The structure of the electronic nonlinear optical conductivity is elucidated in a detailed study of the time-reversal symmetric two-band model. The nonlinear conductivity is decomposed as a sum of contributions related with different…
The family of 2D layered semiconductors, including transition metal chalcogenides (TMCs) of the form MX (M=Ga, In; X=S, Se, Te) exhibit exceptional nonlinear optical properties. The energetically most favorable crystal ordering for…
We develop a theory of the nonlinear optical responses in superconducting systems in the presence of a dc supercurrent. The optical transitions between particle-hole pair bands across the superconducting gap are allowed in clean…
In this technical review we give an introduction to optical spectroscopy for layered materials as a powerful, non-invasive tool to access details of the electronic band structure and crystal quality. Potential applications in photonics and…
We adapted a recently proposed framework to characterize the optical response of interacting electrons in solids in order to expedite its computation without compromise in accuracy at the microscopic level. Our formulation is based on…
We demonstrate first- and second-order spatial differentiation of an optical beam transverse profile using thin suspended subwavelength gratings. Highly reflective one-dimensional gratings are patterned on suspended 200 nm-thick silicon…
Second-order nonlinear optical materials enable frequency doubling of light (second-harmonic generation, SHG), which is essential for optoelectronic applications ranging from materials characterization to quantum technologies. However,…
The second order optical response of centrosymmetric materials manifests itself mostly at their surface, being strongly suppressed in their bulk. However, the overall surface response is also suppressed in nanoparticles with a…
The second-order nonlinear optical susceptibility ($\chi_{abc}^{(2)}$) and linear electro-optical coefficient ($r_{abc}$) of a large number of single-walled zigzag, armchair and chiral SiC nanotubes (SiC-NTs) as well as bulk SiC polytypes…
First-principles calculations with the full-potential linearized augmented plane-wave (FP-LAPW) method have been performed to investigate detailed electronic and linear optical properties of Sr$_{2}$CuO$_{2}$Cl$_{2}$, which is a classical…
Calculations of the opacity of hot, dense matter require models for plasma line broadening. However, the most general theories are too complex to calculate directly and some approximation is inevitably required. The most widely-used…
We consider optical response in multi-band, multi-layer two-dimensional superconductors. Within a simple model, we show that linear response to AC gating can detect collective modes of the condensate, such as Leggett and clapping modes. We…
We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in…
In this work, three InAs/InAs$_{0.65}$Sb$_{0.35}$ superlattices with different periods were investigated using photoluminescence and photoreflectance measurements and their band structure was simulated using a 14 bulk-band kp model. The…
A review of the main phenomena related with the linear optical properties of isolated and supported metal nanoparticles is presented. The extinction, absorption and scattering efficiencies are calculated using the Mie theory and the…