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Related papers: Ab-initio density functional study of O on the Ag(…

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The oxidation of {\alpha}-Ti(0001) surface was studied using density functional theory. In order to enhance the oxidation resistance, we substituted Ti atoms with Si atoms in Ti(0001) surface. We observe that Si prefers to segregate at the…

Our ab initio calculations of CO adsorption energies on low miller index (111), (100), stepped (211), and kinked (532) gold surfaces show a strong dependence on local coordination with a reduction in Au atom coordination leading to higher…

Materials Science · Physics 2009-11-13 F. Mehmood , A. Kara , T. S. Rahman , C. R. Henry

Only recently, the activation of oxygen molecules on clean defect-free transition metal oxide surfaces has been reported, for example on the CaO-terminated surface of the Ruddelsden-Popper perovskite \crosurf. In this work we show that…

Materials Science · Physics 2018-10-10 Wernfried Mayr-Schmölzer , Florian Mittendorfer , Josef Redinger

Theoretical calculations based on density functional theory have made significant contributions to our understanding of metal oxides, their surfaces, and the binding of molecules at these surfaces. In this paper we investigate the binding…

Materials Science · Physics 2007-05-23 Oyvind Borck , Elsebeth Schroder

In this paper we investigate by means of first-principles density functional theory calculations the (111) surface of the Ag-Cu alloy under varying conditions of pressure of the surrounding oxygen atmosphere and temperature. This alloy has…

Materials Science · Physics 2009-11-13 Simone Piccinin , Catherine Stampfl , Matthias Scheffler

The Work function (f)is fundamental for chemistry and electronics. Additionally, f can be used to examine the validity of the theoretical surfaces by comparing it with experimental f, even in the absence of long-range orders. In the…

Materials Science · Physics 2025-07-10 Yukio Watanabe , S. Miyauchi , S. Kaku , T. Yamada , A. Horiguchi

Nowadays, electrochemical reduction of CO$_2$ has been considered as an effective method to solve the problem of global warming. The primary challenge in studying the mechanism is to determine the adsorption states of CO$_2$, since…

Chemical Physics · Physics 2020-07-03 Shuai Guo , Yao Li , Lei Liu , Xiangping Zhang , Suojiang Zhang

Atom controlled sub-nanometer MoS$_2$ pores have been recently fabricated. Oxidative environments are of particular interest for MoS$_2$ applications in electronics, sensing and energy storage. In this work we carried out first-principles…

Materials Science · Physics 2023-01-31 Murilo Kendjy Onita , Flavio Bento de Oliveira , Andreia Luisa da Rosa

Knowledge of the atomic geometry of a surface is a prerequisite for any detailed understanding of the surface's electronic structure and chemical properties. Previous studies have convincingly demonstrated that density functional theory…

Materials Science · Physics 2007-05-23 C. Stampfl , M. Scheffler

The adsorption of hydrogen on the polar Zn-ended ZnO(0001) surface has been investigated by density functional {\it ab-initio} calculations. An on top H(1x1) ordered overlayer with genuine H-Zn chemical bonds is shown to be energetically…

Materials Science · Physics 2015-05-13 N. Sanchez , S. Gallego , J. Cerdá , M. C. Muñoz

Several dissociated and two non-dissociated adsorption structures of the phenol molecule on the Si(001)-(2 \times 1) surface are studied using density functional theory with various exchange and correlation functionals. The relaxed…

Computational Physics · Physics 2015-05-19 Karen Johnston , Andris Gulans , Tuukka Verho , Martti J. Puska

Using first-principles calculations, we systematically study the adsorption behaviors of molecular CO on the Be (0001) surface. By calculating the potential energy surfaces, we find that CO molecularly adsorbs on the Be surface with small…

Materials Science · Physics 2015-05-13 Shuang-Xi Wang , Yu Yang , Bo Sun , Rong-Wu Li , Shao-Jun Liu , Ping Zhang

We report on a computational study of the clean and oxygen-covered Rh(110) surface, based on density-functional theory within the local-density approximation. We have used plane-wave basis sets and Vanderbilt ultra-soft pseudopotentials.…

Condensed Matter · Physics 2009-10-28 Kurt Stokbro , Stefano Baroni

We have studied the chemisorption processes of O2 on the (100) surface of uranium using generalized gradient approximation to density functional theory. Dissociative adsorptions of O2 are significantly favored compared to molecular…

Strongly Correlated Electrons · Physics 2015-06-24 M. N. Huda , A. K. Ray

The results of DFT supercell calculations of oxygen behavior upon the UN (001) and (110) surfaces as well as at the tilt grain boundary are presented. Oxygen adsorption, migration, incorporation into the surface N vacancies on (001) and…

Materials Science · Physics 2015-06-12 D. Bocharov , D. Gryaznov , Yu. F. Zhukovskii , E. A. Kotomin

Solar water splitting has attracted much attention as a clean and renewable route to produce hydrogen fuel. Since the oxygen evolution half-reaction (OER) requires high overpotentials, much research has focused on finding catalyst materials…

Materials Science · Physics 2019-06-03 Maria Bouri , Ulrich Aschauer

To help understand the high activity of silver as an oxidation catalyst, e.g., for the oxidation of ethylene to epoxide and the dehydrogenation of methanol to formaldehyde, the interaction and stability of oxygen species at the Ag(111)…

Materials Science · Physics 2009-11-10 Wei-Xue Li , Catherine Stampfl , Matthias Scheffler

The adsorption and dissociation of isolated water molecule on Zr(0001) surface are theoretically investigated for the first time by using density-functional theory calculations. Two kinds of adsorption configurations with almost the same…

Materials Science · Physics 2015-05-27 Shuang-Xi Wang , Ping Zhang , Peng Zhang , Jian Zhao , Shu-Shen Li

The adsorption of CO molecules at the Ca3Ru2O7(001) surface was studied using low-temperature scanning tunneling microscopy (STM) and density functional theory (DFT). Ca3Ru2O7 can be easily cleaved along the (001) plane, yielding a smooth,…

We study adsorption sites of a single Xe adatom on Nb(110) surface using a density functional theory approach: The on-top site is the most favorable position for the adsorption. We compare the binding features of the present study to…

Materials Science · Physics 2015-06-03 S. Dag , M. Shaughnessy , C. Y. Fong , X. D. Zhu , L. H. Yang