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Two single-molecule magnets are coupled antiferromagnetically to form a supramolecule dimer. We study the coupling effect and tunneling process by means of the numerical exact diagonalization method, and apply them to the recently…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. M. Hu , Z. D. Chen , S. Q. Shen

A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Tiron , W. Wernsdorfer , D. Foguet-Albiol , N. Aliaga-Alcalde , G. Christou

It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 María José Santander , Alvaro S. Nunez , A. Roldán-Molina , Roberto E. Troncoso

A Mn4 single-molecule magnet (SMM) is used to show that quantum tunneling of magnetization (QTM) is not suppressed by moderate three dimensional exchange coupling between molecules. Instead, it leads to an exchange bias of the quantum…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Tiron , W. Wernsdorfer , N. Aliaga-Alcalde , D. N. Hendrickson , G. Christou

The resonant tunneling phenomenon is well understood in quantum mechanics. We argue why a similar phenomenon must be present in quantum field theory. We then use the functional Schr\"odinger method to show how resonant tunneling through…

High Energy Physics - Theory · Physics 2009-10-08 S. -H. Henry Tye , Daniel Wohns

Quantum (step-like) magnetization curves are studies for a spin pair with antiferromagnetic coupling in the presence of a magnetic field parallel to the easy axis of the magnetic anisotropy. The consideration is done both analytically and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 B. A. Ivanov , V. E. Kireev

Two antiferromagnetically coupled tunneling systems is a minimal model exhibiting the effect of quantum-mechanical phase in the Landau-Zener effect. It is shown that the averaged staying probability oscillates vs resonance shift between the…

Statistical Mechanics · Physics 2007-05-23 D. A. Garanin

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

The role of spin polarized reservoirs in quantum tunneling of magnetization and relaxation processes in a single molecular magnet (SMM) is investigated theoretically. The SMM is exchange-coupled to the reservoirs and also subjected to a…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 Maciej Misiorny , Józef Barnas

We study macroscopic quantum tunneling of the magnetic moment in a single-domain particle placed above the surface of a superconductor. Such a setup allows one to manipulate the height of the energy barrier, preserving the degeneracy of the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Eugene M. Chudnovsky , Jonathan R. Friedman

Using the simplest two-subband Stoner model, it is shown that the variation of the Fermi energy under applied magnetic field is inverse proportional to the spontaneous magnetization and hence most pronounced close to the critical Stoner…

Strongly Correlated Electrons · Physics 2007-05-23 Yu. G. Pogorelov , J. B. Sousa , J. -P. Araujo

The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model. On the basis of instanton technique…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Hui Hu , Rong Lü , Jia-Ling Zhu , Jia-Jiong Xiong

We study the Schwinger effect, in which the external field having a spatiotemporal profile creates electron-positron pairs via multidimensional quantum tunneling. Our treatment is based on the trace formula for the QED effective action,…

High Energy Physics - Theory · Physics 2016-04-13 Cesim K. Dumlu

We present a formalism based on the functional Schr\"odinger equation to analyse time-dependent tunneling in quantum field theory at the semi-classical level. The full problem is reduced step by step to a finite dimensional quantum…

High Energy Physics - Theory · Physics 2019-11-27 Luc Darmé , Joerg Jaeckel , Marek Lewicki

We investigate a system of three tunnel-coupled semiconductor quantum dots in a triangular geometry, one of which is connected to a metallic lead, in the regime where each dot is essentially singly occupied. Both ferro- and…

Strongly Correlated Electrons · Physics 2015-12-22 Andrew K. Mitchell , Thomas F. Jarrold , David E. Logan

We study macroscopic quantum coherence in antiferromagnetic molecular magnets in the presence of magnetic fields. Such fields generate artificial tunnel barriers with externally tunable strength. We give detailed semi-classical predictions…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Alain Chiolero , Daniel Loss

The quantum tunneling of the magnetization vector are studied theoretically in single-domain ferromagnetic nanoparticles placed in an external magnetic field at an arbitrarily directed angle in the $ZX$ plane. We consider the…

Statistical Mechanics · Physics 2009-10-31 Rong Lu , Jia-Lin Zhu , Zhi-Rong Liu , Lee Chang , Bing-Lin Gu

High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…

Mesoscale and Nanoscale Physics · Physics 2022-02-17 Sascha Brinker , Felix Küster , Stuart S. P. Parkin , Paolo Sessi , Samir Lounis

We consider an effect of a strong magnetic field on the ground state and macroscopic coherent tunneling in small antiferromagnetic particles with uniaxial and biaxial single-ion anisotropy. We find several tunneling regimes that depend on…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 B. A. Ivanov , V. E. Kireev

The quantum tunneling of the magnetization vector between excited levels are studied theoretically in single-domain ferromagnetic nanoparticles with biaxial crystal symmetry placed in an external magnetic field at an arbitarily directed…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Rong Lu , Su-Peng Kou , Jia-Lin Zhu , Lee Chang , Bing-Lin Gu
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