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An accurate analytical parametrization for the exchange-correlation free energy of the homogeneous electron gas, including interpolation for partial spin-polarization, is derived via thermodynamic analysis of recent restricted path integral…

Chemical Physics · Physics 2015-06-17 Valentin V. Karasiev , Travis Sjostrom , James Dufty , S. B. Trickey

By propagating the many-body Schr\"odinger equation, we determine the exact time-dependent Kohn-Sham potential for a system of strongly correlated electrons which undergo field-induced tunneling. Numerous features are entirely absent from…

Strongly Correlated Electrons · Physics 2021-01-15 Matthew J. P. Hodgson , James D. Ramsden , Jacob B. J. Chapman , Piers Lillystone , Rex W Godby

A combination of density functional theory in its local density approximation (LDA) with k- and $\omega $ dependent self-energy found from fluctuational-exchange-type random phase approximation (FLEX-RPA) is utilized here to study…

Superconductivity · Physics 2024-03-12 Griffin Heier , Sergey Y. Savrasov

We develop an automated procedure to select the local potential of a separable pseudopotential that minimizes transferability errors for the isolated atom, and we show that this optimization leads to significant improvements in the accuracy…

Chemical Physics · Physics 2018-11-05 Casey O. Barkan , Andrew M. Rappe

Density functional theory offers a very accurate way of computing materials properties from first principles. However, it is too expensive for modelling large-scale molecular systems whose properties are, in contrast, computed using…

Computational Physics · Physics 2016-12-12 Alexander V. Shapeev

Self-interactions (SIs) are a major problem in density functional approximations and the source of serious divergence from experimental results. Here, we propose to optimize density functional total energies in terms of the effective local…

Other Condensed Matter · Physics 2012-06-20 Nikitas I. Gidopoulos , Nektarios N. Lathiotakis

We present one inherent shortcoming of the LDA+U method in respect of its self-interaction correction of the LDA. By reexamining the mean-field approximation on the Hubbard energy in the Hartree-Fock form, we have derived a new expression…

Strongly Correlated Electrons · Physics 2007-07-19 Dong-Kyun Seo

In approximate density functional theory (DFT), the self-interaction error is an electron delocalization anomaly associated with underestimated insulating gaps. It exhibits a predominantly quadratic energy-density curve that is amenable to…

Chemical Physics · Physics 2016-12-21 Glenn Moynihan , Gilberto Teobaldi , David D. O'Regan

The method of electronic structure calculations for strongly correlated disordered materials is developed employing the basic idea of coherent potential approximation (CPA). Evolution of electronic structure and spin magnetic moment value…

Strongly Correlated Electrons · Physics 2014-02-28 M. A. Korotin , Z. V. Pchelkina , N. A. Skorikov , E. Z. Kurmaev , V. I. Anisimov

We propose a smooth pseudopotential for the contact interaction acting between ultracold atoms confined to two dimensions. The pseudopotential reproduces the scattering properties of the repulsive contact interaction up to 200 times more…

Quantum Gases · Physics 2016-04-15 T. M. Whitehead , L. M. Schonenberg , N. Kongsuwan , R. J. Needs , G. J. Conduit

The description of realistic strongly correlated systems has recently advanced through the combination of density functional theory in the local density approximation (LDA) and dynamical mean field theory (DMFT). This LDA+DMFT method is…

Strongly Correlated Electrons · Physics 2009-11-13 B. Amadon , F. Lechermann , A. Georges , F. Jollet , T. O. Wehling , A. I. Lichtenstein

We propose and analyze a technique to collectively enhance interactions between solid-state quantum registers composed from random networks of spin qubits. In such systems, disordered dipolar interactions generically result in localization.…

Quantum Physics · Physics 2013-04-29 Hendrik Weimer , Norman Y. Yao , Mikhail D. Lukin

We present a new formulation of the time-dependent self-interaction correction (TDSIC). It is derived variationally obeying explicitly the constraints on orthonormality of the occupied single-particle orbitals. The thus emerging rather…

Quantum Physics · Physics 2009-03-02 J. Messud , P. M. Dinh , P. -G. Reinhard , E. Suraud

Accurate description of the excess charge in water cluster anions is challenging for standard semi-local and (global) hybrid density functional approximations (DFAs). Using the recent unitary invariant implementation of the Perdew-Zunger…

Chemical Physics · Physics 2020-02-11 Jorge Vargas , Peter Ufondu , Tunna Baruah , Yoh Yamamoto , Koblar A. Jackson , Rajendra R. Zope

It is demonstrated that the commonly applied self interaction correction (SIC) used in density functional theory does not remove all self interaction. We present as an alternative a novel method which, by construction, is totally free from…

Materials Science · Physics 2007-05-23 Urban Lundin , Olle Eriksson

Experimental implementations of quantum simulation must balance the controllability of the quantum system under test with decoherence typically introduced through interaction with external control fields. The ratio of coherent interaction…

This article reviews recent inverse statistical-mechanical methodologies that we have devised to optimize interaction potentials in soft matter systems that correspond to stable "target" structures. We are interested in finding the…

Soft Condensed Matter · Physics 2008-11-05 Salvatore Torquato

We present an effective non-relativistic theory of self-interacting dark matter. We classify the long range interactions and discuss how they can be generated from quantum field theories. Generic dark sectors can generate singular…

High Energy Physics - Phenomenology · Physics 2013-10-30 Brando Bellazzini , Mathieu Cliche , Philip Tanedo

Non-gravitational interactions between dark matter particles with strong scattering, but relatively small annihilation and dissipation, has been proposed to match various observables on cluster and group scales. In this paper, we present…

Cosmology and Nongalactic Astrophysics · Physics 2020-03-04 Arka Banerjee , Susmita Adhikari , Neal Dalal , Surhud More , Andrey Kravtsov

The $GW$ approximation is a widely used framework for studying correlated materials, but it struggles with certain limitations, such as its inability to explain pseudogap phenomena. To overcome these problems, we propose a systematic…

Strongly Correlated Electrons · Physics 2024-09-26 Hui Li , Yingze Su , Junnian Xiong , Haiqing Lin , Huaqing Huang , Dingping Li