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Polyelectrolytes such as single and double stranded DNA and many synthetic polymers undergo two structural transitions upon increasing the concentration of multivalent salt or molecules. First, the expanded-stretched chains in low…

Soft Condensed Matter · Physics 2009-10-31 Francisco J. Solis , Monica Olvera de la Cruz

We report on a study of the shape of a stiff, charged rod that is subjected to equal and opposite force couples at its two ends. Unlike a neutral elastic rod, which forms a constant curvature configuration under such influences, the charged…

Soft Condensed Matter · Physics 2009-11-07 Roya Zandi , Joseph Rudnick , Ramin Golestanian

We address the long standing problem of the dependence of the electrostatic persistence length $l_e$ of a flexible polyelectrolyte (PE) on the screening length $r_s$ of the solution within the linear Debye-Huckel theory. The standard Odijk,…

Soft Condensed Matter · Physics 2009-11-07 T. T. Nguyen , B. I. Shklovskii

We investigate the electrostatic contribution to the persistence length of a semiflexible polymer chain whose segments interact via a screened Debye-H\" uckel dipolar interaction potential. We derive the expressions for the renormalized…

Soft Condensed Matter · Physics 2009-11-10 R. Podgornik

This study investigates the interplay between Strong Coupling (SC) attraction and hydration repulsion in nanoconfined water between like-charged phospholipid layers. It challenges the assumption that SC attraction requires multivalent…

We present a study of the solvation properties of model aqueous electrode interfaces. The exposed electrodes we study strongly bind water and have closed packed crystalline surfaces, which template an ordered water adlayer adjacent to the…

Statistical Mechanics · Physics 2015-06-11 David T. Limmer , Adam P. Willard , Paul A. Madden , David Chandler

A self-consistent mode-coupling theory is presented for the viscosity of solutions of charged rod-like polymers. The static structure factor used in the theory is obtained from polymer integral equation theory; the Debye-H\"{u}ckel…

Soft Condensed Matter · Physics 2009-11-10 Kunimasa Miyazaki , Biman Bagchi , Arun Yethiraj

We report results from a molecular dynamics (MD) simulation on the conformations of a long flexible polyelectrolyte complexed to a charged sphere, \textit{both negatively charged}, in the presence of neutralizing counterions in the strong…

Soft Condensed Matter · Physics 2009-11-07 Rene Messina , Christian Holm , Kurt Kremer

We report grand canonical Monte Carlo simulations of the critical point properties of homopolymers within the Bond Fluctuation model. By employing Configurational Bias Monte Carlo methods, chain lengths of up to N=60 monomers could be…

Condensed Matter · Physics 2009-10-28 N. B. Wilding , M. Mueller , K. Binder

Polymeric materials that couple deformation and electrostatics have the potential for use in soft sensors and actuators with potential applications ranging from robotic, biomedical, energy, aerospace and automotive technologies. In contrast…

Soft Condensed Matter · Physics 2020-06-02 Matthew Grasinger , Kaushik Dayal

A weakly charged flexible polyelectrolyte chain in a neutral spherical cavity is analyzed using self-consistent field theory (SCFT) within an explicit solvent model. Assuming the radial symmetry for the system, it is found that the…

Soft Condensed Matter · Physics 2009-11-13 Rajeev Kumar , M. Muthukumar

Polyelectrolyte (PE) brushes are widely used in biomaterials and nanotechnology to regulate surface properties and interactions. Here, we apply the electrostatic correlation augmented self-consistent field theory to investigate the…

Soft Condensed Matter · Physics 2024-08-16 Chao Duan , Rui Wang

The influence of the patchiness and correlations in the distribution of hydrophobic and polar residues at the interface between two rigid biomolecules on their recognition ability is investigated in idealised coarse-grained lattice models.…

Biological Physics · Physics 2009-11-13 Hans Behringer , Friederike Schmid

A variational approach is considered to calculate the free energy and the conformational properties of a polyelectrolyte chain in $d$ dimensions. We consider in detail the case of pure Coulombic interactions between the monomers, when…

Soft Condensed Matter · Physics 2007-05-23 G. Migliorini , V. G. Rostiashvili , T. A. Vilgis

The electron-hole correlation length serves as an intrinsic length scale for analyzing excitonic interactions in semiconductor nanoparticles. In this work, the derivation of electron-hole correlation length using the two-particle reduced…

Atomic and Molecular Clusters · Physics 2014-06-03 Christopher J. Blanton , Arindam Chakraborty

We have studied the molecular scale hydrophobicity of an apolar solute, argon, confined between hydrophobic planar surfaces with different confinement widths. Specifically, we find that the hydrophobicity exhibits a non-monotonic behavior…

Soft Condensed Matter · Physics 2015-01-27 Sudip Nepal , Pradeep Kumar

The temperature and length scale dependence of solvation properties of spherical hard solvophobic solutes is investigated in the Jagla liquid, a simple liquid that consists of particles interacting via a spherically symmetric potential…

Soft Condensed Matter · Physics 2015-06-12 John R. Dowdle , Sergey V. Buldyrev , H. Eugene Stanley , Pablo G. Debenedetti , Peter J. Rossky

Polyelectrolyte complexation plays an important role in materials science and biology. The internal structure of the resultant polyelectrolyte complex (PEC) phase dictates properties such as physical state, response to external stimuli, and…

The thermodynamic properties of disks moving in a channel sufficiently narrow that they can collide only with their nearest neighbors can be solved exactly by determining the eigenvalues and eigenfunctions of an integral equation. Using it…

Soft Condensed Matter · Physics 2014-03-17 M. J. Godfrey , M. A. Moore

Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach