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The vibrational properties of three sodosilicate glasses have been investigated in the framework of Density Functional Theory. The pure vibrational density of states has been calculated for all systems and the different vibrational modes…

Materials Science · Physics 2019-02-21 Dimitrios Kilymis , Simona Ispas , Bernard Hehlen , Sylvain Peuget , Jean-Marc Delaye

First-principles molecular dynamics simulations having a duration of 8 ps have been used to study the static, dynamic and electronic properties of l-Ga at the temperatures 702 K and 982 K. The simulations use the density-functional…

mtrl-th · Physics 2016-09-07 Janusz M. Holender , Mike J. Gillan , Mike C. Payne , Allan Simpson

We use event driven simulations to analyze glassy dynamics as a function of density and energy dissipation in a two-dimensional bidisperse granular fluid under stationary conditions. Clear signatures of a glass transition are identified,…

Statistical Mechanics · Physics 2011-10-05 Iraj Gholami , Andrea Fiege , Annette Zippelius

We report the results of ab initio molecular dynamics simulations of liquid Ga_xAs_{1-x} alloys at five different concentrations, at a temperature of 1600 K, just above the melting point of GaAs. The liquid is predicted to be metallic at…

Condensed Matter · Physics 2009-10-31 R. V. Kulkarni , D. Stroud

We study by Molecular Dynamics simulation a dense one-component system of particles confined on a spherical substrate. We more specifically investigate the evolution of the structural and dynamical properties of the system when changing the…

Soft Condensed Matter · Physics 2018-05-23 Julien-Piera Vest , Gilles Tarjus , Pascal Viot

The dynamics of dislocations is reported to exhibit glassy properties. We study numerically various versions of 2d edge dislocation systems in the absence of externally applied stress. Two types of glassy behavior are identified: (i)…

Disordered Systems and Neural Networks · Physics 2009-11-13 B. Bako , I. Groma , G. Gyorgyi , G. T. Zimanyi

We have determined the vibrational properties of a sodium tetrasilicate (Na$_{2}$Si$_{4}$O$_{9}$) glass model generated by molecular dynamics simulations. The study has been carried out using a classical valence force fields approach as…

Disordered Systems and Neural Networks · Physics 2007-05-23 S. Ispas , N. Zotov , S. De Wispelaere , W. Kob

We study the structural and dynamical characteristics of the sodium atoms inside and outside the ``diffusion channels'' in glassy Na$_2$O-4SiO$_2$ (NS4) using classical molecular dynamics. We show that on average neither energetic arguments…

Disordered Systems and Neural Networks · Physics 2009-11-07 Emmanuel Sunyer , Philippe Jund , Remi Jullien

Direct atomically resolved observation of dynamics deep in the glassy regime has proved elusive for atomic and molecular glasses. Studies below the glass transition temperature Tg are especially rare due to long waiting times required to…

Mesoscale and Nanoscale Physics · Physics 2010-06-10 Sumit Ashtekar , Gregory Scott , Joseph Lyding , Martin Gruebele

We introduce the ideal Gaussian glass-forming system as a model to describe the thermodynamics and dynamics of supercooled liquids on a local scale in terms of the properties of the potential energy landscape (PEL). The first ingredient is…

Materials Science · Physics 2009-11-13 A. Heuer , A. Saksaengwijit

Measuring, characterizing and modelling the slow dynamics of glassy soft matter is a great challenge, with an impact that ranges from industrial applications to fundamental issues in modern statistical physics, such as the glass transition…

Soft Condensed Matter · Physics 2009-11-11 Luca Cipelletti , Laurence Ramos

It is demonstrated that the width of the uncorrelated atomic-charge distribution in glasses can be extracted from the frequency dependence of the coupling coefficient for the far-infrared absorption measured experimentally by the…

Disordered Systems and Neural Networks · Physics 2009-11-13 S. N. Taraskin , S. I. Simdyankin , S. R. Elliott

We report a detailed experimental study of the structure and dynamics of glassy states in hard spheres with short-range attraction. The system is a suspension of nearly-hard-sphere colloidal particles and non-adsorbing linear polymer which…

Soft Condensed Matter · Physics 2009-11-10 K. N. Pham , S. U. Egelhaaf , P. N. Pusey , W. C. K. Poon

We use ab initio simulations to investigate the properties of a sodium borosilicate glass of composition 3Na_2O-B_2O_3-6SiO_2. We find that the broadening of the first peak in the radial distribution functions g_BO(r) and g_BNa(r) is due to…

Disordered Systems and Neural Networks · Physics 2018-02-28 Laurent Pedesseau , Simona Ispas , Walter Kob

Simple binary oxide glasses can exhibit a compression behavior distinct from that of their crystalline counterparts. In this study, we employed high-pressure X-ray absorption spectroscopy coupled to the diamond anvil cell to investigate in…

The unifying feature of glass formers (such as polymers, supercooled liquids, colloids, granulars, spin glasses, superconductors, ...) is a sluggish dynamics at low temperatures. Indeed, their dynamics is so slow that thermal equilibrium is…

We investigated the structural and dynamical properties of a tetrahedrally coordinated crystalline ice from first principles based on density functional theory within the generalized gradient approximation with the projected augmented wave…

Materials Science · Physics 2007-05-23 W. A. Adeagbo , A. Zayak , P. Entel

Despite the enormous theoretical and application interests, a fundamental understanding of the glassy dynamics remains elusive. The static properties of glassy and ordinary liquids are similar, but their dynamics are dramatically different.…

Soft Condensed Matter · Physics 2023-11-21 Puneet Pareek , Monoj Adhikari , Chandan Dasgupta , Saroj Kumar Nandi

We present a computational study of the electronic properties of amorphous SiO2. The ionic configurations used are the ones generated by an earlier molecular dynamics simulations in which the system was cooled with different cooling rates…

Disordered Systems and Neural Networks · Physics 2009-10-30 Thorsten Koslowski , Walter Kob , Katharina Vollmayr

Atomic vibrations in perfect, slightly defective or mixed crystals are to a large extent well understood since many decades. Theoretical descriptions are thus in excellent agreement with the experiments. As a consequence, phonon-related…

Disordered Systems and Neural Networks · Physics 2021-01-12 Benoit Rufflé , Marie Foret , Bernard Hehlen