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We report on the magnetic excitation spectrum of the coupled spin tetrahedral system Cu$_{2}$Te$_{2}$O$_{5}$Cl$_{2}$ using Raman scattering on single crystals. The transition to an ordered state at T$_{N}^{Cl}$=18.2 K evidenced from…

Strongly Correlated Electrons · Physics 2009-11-13 Kwang-Yong Choi , Hiroyuki Nojiri , Naresh S. Dalal , Helmuth Berger , Wolfram Brenig , Peter Lemmens

Raman light-scattering experiments in the antiferromagnetic phase of the Cu_2Te_2O_5(Br_(1-x)Cl_x)_2 compounds are analyzed in terms of a dimerized spin model for the tetrahedral Cu-clusters. It is shown that the longitudinal magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 J. Jensen , P. Lemmens , C. Gros

Thermodynamic experiments as well as Raman scattering have been used to study the magnetic instabilities in the spin-tetrahedra systems Cu_2Te_2O_5X_2, X=Cl and Br. While the phase transition observed in the Cl system at T_o=18.2 K is…

Strongly Correlated Electrons · Physics 2009-11-07 P. Lemmens , K. -Y. Choi , E. E. Kaul , Ch. Geibel , K. Becker , W. Brenig , R. Valenti , C. Gros , M. Johnsson , P. Millet , F. Mila

Low energy Raman scattering of the s=1/2 spin tetrahedra system Cu_2Te_2O_5Br_2 is dominated by an excitation at 18 cm^{-1} corresponding to an energy E_S=0.6\Delta, with \Delta the spin gap of the compound. For elevated temperatures this…

Strongly Correlated Electrons · Physics 2009-11-07 P. Lemmens , K. Y. Choi , A. Ionescu , J. Pommer , G. Guentherodt , R. Valenti , C. Gros , W. Brenig , M. Johnsson , P. Millet , F. Mila

Neutron scattering studies on powder and single crystals have provided new evidences for unconventional magnetism in Cu2Te2O5Cl2. The compound is built from tetrahedral clusters of S=1/2 Cu2+ spins located on a tetragonal lattice. Magnetic…

Strongly Correlated Electrons · Physics 2009-11-11 O. Zaharko , H. M. Ronnow , A. Daoud-Aladine , S. Streule , F. Juranyi , J. Mesot , H. Berger , P. J. Brown

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

Strongly Correlated Electrons · Physics 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

The magnetic properties of the layered oxypnictide LaMnAsO have been revisited using neutron scattering and magnetization measurements. The present measurements identify the N\'{e}el temperature $T_N$ = 360(1) K. Below $T_N$ the critical…

Strongly Correlated Electrons · Physics 2016-02-10 Michael A. McGuire , V. Ovidiu Garlea

When an ordered spin system of a given dimensionality undergoes a second order phase transition the dependence of the order parameter i.e. magnetization on temperature can be well-described by thermal excitations of elementary collective…

Materials Science · Physics 2017-03-30 H. J. Qin , Kh. Zakeri , A. Ernst , J. Kirschner

We report on zero-field muon spin rotation, electron spin resonance and polarized Raman scattering measurements of the coupled quantum spin ladder Ba2CuTeO6. Zero-field muon spin rotation and electron spin resonance probes disclose a…

Strongly Correlated Electrons · Physics 2017-06-28 A. Glamazda , Y. S. Choi , S. -H. Do , S. Lee , P. Lemmens , A. N. Ponomaryov , S. A. Zvyagin , J. Wosnitza , Dita Puspita Sari , I. Watanabe , K. -Y. Choi

We present high-field magnetization and $^{79}$Br nuclear quadrupole resonance (NQR) and $^{125}$Te nuclear magnetic resonance (NMR) studies in the weakly coupled Cu$^{2+}$ ($S=1/2$) tetrahedral system Cu$_2$Te$_2$O$_5$Br$_2$. The…

Strongly Correlated Electrons · Physics 2012-11-28 S. -H. Baek , K. -Y. Choi , H. Berger , B. Büchner , H. -J. Grafe

Neutron inelastic scattering investigations have been performed on the spin tetrahedral system Cu_2Te_2O_5X_2 (X = Cl, Br). We report the observation of magnetic excitations with a dispersive component in both compounds, associated with the…

Other Condensed Matter · Physics 2009-11-11 S. J. Crowe , S. Majumdar , M. R. Lees , D. McK. Paul , R. I. Bewley , S. J. Levett , C. Ritter

An incommensurate elliptical helical magnetic structure in the frustrated coupled-spin-chain system FeTe2O5Br is surprisingly found to persist down to 53(3) mK (T/T_N ~ 1/200), according to neutron scattering and muon spin relaxation. In…

Strongly Correlated Electrons · Physics 2012-11-29 M. Pregelj , A. Zorko , O. Zaharko , D. Arcon , M. Komelj , A. D. Hillier , H. Berger

High-resolution ac susceptibility and thermal conductivity measurement on Cu2Te2O5X2(X=Br,Cl) single crystals are reported. For Br-sample, sample dependence prevents to distinguish between possibilities of magnetically ordered and…

Strongly Correlated Electrons · Physics 2009-11-10 M. Prester , A. Smontara , I. Zivkovic , A. Bilusic , D. Drobac , H. Berger , F. Bussy

We study the magnetism of a lattice of coupled tetrahedral spin-1/2 clusters which might be of relevance to the tellurate compounds Cu2Te2O5X2, with X=Cl, Br. Using the flow equation method we perform a series expansion in terms of the…

Strongly Correlated Electrons · Physics 2009-11-07 Wolfram Brenig

Two magnon excitations and the nodal spin density wave (SDW) gap were observed in BaFe2As2 by Raman scattering. Below the SDW transition temperature (TSDW) nodal SDW gap opens together with new excitations in reconstructed electronic…

Superconductivity · Physics 2010-11-01 S. Sugai , Y. Mizuno , R. Watanabe , T. Kawaguchi , K. Takenaka , H. Ikuta , Y. Takayanagi , N. Hayamizu , Y. Sone

Magnetic systems with spins sitting on a lattice of corner sharing regular tetrahedra have been particularly prolific for the discovery of new magnetic states for the last two decades. The pyrochlore compounds have offered the playground…

Strongly Correlated Electrons · Physics 2017-10-05 P. Dalmas de Reotier , C. Marin , A. Yaouanc , C. Ritter , A. Maisuradze , B. Roessli , A. Bertin , P. J. Baker , A. Amato

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

Elastic and inelastic neutron scattering measurements have been performed on powder and single-crystal samples of orthorhombic CeRu2Al10. The order forming below T0 = 27 K was identified as a long-range antiferromagnetic state with the wave…

We consider a three-dimensional quantum antiferromagnet in the vicinity of a quantum critical point separating the magnetically ordered and the magnetically disordered phases. A specific example is TlCuCl$_3$ where the quantum phase…

Strongly Correlated Electrons · Physics 2015-03-19 Yakov Kulik , Oleg P. Sushkov
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