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We have attempted to find the global minima of clusters containing between 20 and 80 atoms bound by the Morse potential as a function of the range of the interatomic force. The effect of decreasing the range is to destabilize strained…

Condensed Matter · Physics 2008-02-03 Jonathan Doye , David Wales

Using the basin-hopping Monte Carlo minimization approach we report the global minima for aluminium, gold and platinum metal clusters modelled by the Voter-Chen version of the embedded-atom model potential containing up to 80 atoms. The…

Atomic and Molecular Clusters · Physics 2009-11-10 Ali Sebetci , Ziya B. Guvenc

Zinc and cadmium clusters interacting with a Gupta potential have previously been identified as prototypical metallic systems that exhibiting disordered cluster structures. Here, putative global minima of the potential energy have been…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye

We have located the global minimum for all lead clusters with up to 160 atoms using a glue potential to model the interatomic interactions. The lowest-energy structures are not face-centred cubic as suggested previously. Rather, for N<40…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye , Shaun C. Hendy

The melting of Al clusters in the size range 49 <= N <= 62 has been studied using two model interatomic potentials. The results for the two models are significantly different. The glue potential exhibits a smooth relatively featureless heat…

Other Condensed Matter · Physics 2007-05-23 Eva G. Noya , Jonathan P. K. Doye , Florent Calvo

Using a Monte Carlo minimization approach we report the global minima for metal clusters modelled by the Sutton-Chen family of potentials with N<81, where N is the number of atoms. The resulting structures are discussed in the light of both…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , David Wales

We examine the favoured cluster structures for two new potentials, which both behave as monatomic model glass-formers in bulk. We find that the oscillations in the interatomic potential lead to global minima that are non-compact…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye , David J. Wales , Fredrik H. M. Zetterling , Mikhail Dzugutov

Putative global minima of sodium clusters with up to 380 atoms have been located for two model interatomic potentials. Structures based upon the Mackay icosahedra predominate for both potentials, and the magic numbers for the…

Other Condensed Matter · Physics 2007-06-13 Eva G. Noya , Jonathan P. K. Doye , David J. Wales

A series of electronic and structural transitions are predicted in molten lithium from first principles. A new phase with tetrahedral local order characteristic of $sp^3$ bonded materials and poor electrical conductivity is found at…

Materials Science · Physics 2009-07-09 Isaac Tamblyn , Jean-Yves Raty , Stanimir A. Bonev

The global minima of clusters bound by a Dzugutov potential form non-compact polytetrahedral clusters mainly composed of interpenetrating and face-sharing 13-atom icosahedra. As the size increases, these icosahedral units first form linear…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , David Wales , Sergei Simdyankin

We locate putative global minima for (C_60)_N clusters modelled by the potential of Pacheco and Prates-Ramalho up to N=105. These minima are based on icosahedral packing up to N=15, but above this size the lowest-energy structures are…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye , David J. Wales , Wolfgang Branz , Florent Calvo

The lowest-energy structures of lead clusters interacting via a Gupta potential are obtained for N<151. Structures based on Marks decahedra dominate at the larger sizes. These results are very different from those obtained previously using…

Other Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye

Classical molecular dynamics simulation with embedded atom method potential had been performed to investigate the surface structure and solidification morphology of aluminum nanoclusters Aln (n = 256, 604, 1220 and 2048). It is found that…

Materials Science · Physics 2015-05-13 F. L. Tang , W. J. Lu , G. B. Chen , Y. Xie , W. Y. Yu

We report on the structures of aluminum hydrides derived from a tetrahedral aluminum Al4 cluster using ab initio quantum chemical calculation. Our calculation of binding energies of the aluminum hydrides reveals that stability of these…

Atomic and Molecular Clusters · Physics 2011-09-15 Kazuhide Ichikawa , Yuji Ikeda , Ayumu Wagatsuma , Kouhei Watanabe , Pawel Szarek , Akitomo Tachibana

We investigate the interplay of particle number, N, and structural properties of selected clusters with N=12 up to N=562 by employing Gupta potentials parameterized for Aluminum and extensive Monte-Carlo simulations. Our analysis focuses on…

Materials Science · Physics 2015-05-14 A. Bagrets , R. Werner , F. Evers , G. Schneider , D. Schooss , P. Woelfle

Using experiments and simulations, we investigate the clusters that form when colloidal spheres stick irreversibly to -- or "park" on -- smaller spheres. We use either oppositely charged particles or particles labeled with complementary DNA…

We present a new theoretical framework for modelling the fusion process of Lennard-Jones (LJ) clusters. Starting from the initial tetrahedral cluster configuration, adding new atoms to the system and absorbing its energy at each step, we…

Atomic and Molecular Clusters · Physics 2009-09-29 Ilia A. Solovyov , Andrey V. Solovyov , Walter Greiner

A new atomic cluster structure corresponding to the global minimum of the 98-atom Lennard-Jones cluster has been found using a variant of the basin-hopping global optimization algorithm. The new structure has an unusual tetrahedral symmetry…

Condensed Matter · Physics 2007-05-23 Robert Leary , Jonathan Doye

In order to study the performance of interatomic potentials and their reliability at higher pressures, the phase diagram of four different embedded-atom type potential models of iron is compared. The calculations were done by the nested…

Materials Science · Physics 2018-03-23 Livia B. Partay

We study why gold forms planar and cage-like clusters while copper and silver do not. We use density functional theory and norm-conserving pseudo-potentials with and without a scalar relativistic component. For the exchange-correlation…

Other Condensed Matter · Physics 2007-05-23 Eva M. Fernandez , Jose M. Soler , L. C. Balbas
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