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We test a hypothesis for the origin of dynamical heterogeneity in slowly relaxing systems, namely that it emerges from soft (Goldstone) modes associated with a broken continuous symmetry under time reparametrizations. We do this by…

Disordered Systems and Neural Networks · Physics 2013-10-30 Karina E. Avila , Horacio E. Castillo , Azita Parsaeian

In order to describe the slow response of a glass former we discuss some distribution of correlation times, e.g., the generalized gamma distribution (GG) and an extension thereof (GGE), the latter allowing to reproduce a simple peak…

Soft Condensed Matter · Physics 2009-11-07 T. Blochowicz , C. Tschirwitz , S. Benkhof , E. A. Rossler

To construct an N-representable time-dependent density-functional theory, a generalization to the time domain of the Levy-Lieb (LL) constrained search algorithm is required. That the action is only stationary in the Dirac-Frenkel…

Other Condensed Matter · Physics 2009-11-10 Morrel H. Cohen , Adam Wasserman

By means of molecular dynamics computer simulations we investigate the out of equilibrium relaxation dynamics of a simple glass former, a binary Lennard-Jones system, after a quench to low temperatures. We study both one time quantities and…

Disordered Systems and Neural Networks · Physics 2009-10-31 Walter Kob , Jean-Louis Barrat

We have computed the time-dependent susceptibility for the finite-size mean-field Random Orthogonal model (ROM). We find that for temperatures above the mode-coupling temperature the imaginary part of the susceptibility $\chi''(\nu)$ obeys…

Statistical Mechanics · Physics 2009-11-10 F. Rao , A. Crisanti , F. Ritort

A fractional relaxation equation in dielectrics with response function of the Havriliak-Negami type is derived. An explicit expression for the fractional operator in this equation is obtained and Monte Carlo algorithm for calculation of…

Other Condensed Matter · Physics 2010-08-25 Renat T. Sibatov , Dmitry V. Uchaikin

Experimental data collected to provide us with information on the course of dielectric relaxation phenomena are got according to two distinct schemes: one can measure either the time decay of depolarization current or use methods of the…

Mesoscale and Nanoscale Physics · Physics 2022-03-29 K. Górska , A. Horzela , K. A. Penson

Amorphous materials have a rich relaxation spectrum, which is usually described in terms of a hierarchy of relaxation mechanisms. In this work, we investigate the local dynamic modulus spectra in a model glass just above the glass…

Disordered Systems and Neural Networks · Physics 2019-03-27 Baoshuang Shang , Jörg Rottler , Pengfei Guan , Jean-Louis Barrat

We study approximate cloaking using transformation optics for electromagnetic waves in the time domain. Our approach is based on estimates of the degree of visibility in the frequency domain for all frequencies in which the frequency…

Analysis of PDEs · Mathematics 2019-01-15 Hoai-Minh Nguyen , Loc Tran

Dynamical heterogeneities -- strong fluctuations near the glass transition -- are believed to be crucial to explain much of the glass transition phenomenology. One possible hypothesis for their origin is that they emerge from soft…

Soft Condensed Matter · Physics 2012-01-10 Karina E. Avila , Horacio E. Castillo , Azita Parsaeian

Dynamical four-point susceptibilities measure the extent of spatial correlations in the dynamics of glass forming systems. We show how these susceptibilities depend on the length scales that necessarily form part of their definition. The…

Statistical Mechanics · Physics 2007-05-23 David Chandler , Juan P. Garrahan , Robert L. Jack , Lutz Maibaum , Albert C. Pan

While lot of measurements describe the relaxation dynamics of the liquid state, experimental data of the glass dynamics at high temperatures are much scarcer. We use ultrafast scanning calorimetry to expand the timescales of the glass to…

A formally exact set of equations is derived for the description of nonequilibrium phenomena in classical liquids and glasses. With the help of a non equilibrium projection operator formalism, the correlation functions and fluctuation…

Disordered Systems and Neural Networks · Physics 2009-10-31 A. Latz

We propose an alternative theory for the relaxation of density fluctuations in glass-forming fluids. We derive an equation of motion for the density correlation function which is local in time and is similar in spirit to the equation of…

Soft Condensed Matter · Physics 2022-06-01 Grzegorz Szamel

Structural relaxation in hard-sphere colloidal glasses has been studied using confocal microscopy. The motion of individual particles is followed over long time scales to detect the rearranging regions in the system. We have used normal…

Soft Condensed Matter · Physics 2015-05-30 Antina Ghosh , Vijayakumar Chikkadi , Peter Schall , Daniel Bonn

We present a new time-dependent Density Functional approach to study the relaxational dynamics of an assembly of interacting particles subject to thermal noise. Starting from the Langevin stochastic equations of motion for the velocities of…

Statistical Mechanics · Physics 2016-08-31 Umberto Marini Bettolo Marconi , Pedro Tarazona

A relaxation process, with the associated phenomenology of sound attenuation and sound velocity dispersion, is found in a simulated harmonic Lennard-Jones glass. We propose to identify this process with the so called microscopic (or…

Disordered Systems and Neural Networks · Physics 2009-10-31 G. Ruocco , F. Sette , R. Di Leonardo , G. Monaco , M. Sampoli , T. Scopigno , G. Viliani

Recent experiments and computer simulations show that supercooled liquids around the glass transition temperature are "dynamically heterogeneous" [1]. Such heterogeneity is expected from the random first order transition theory of the glass…

Disordered Systems and Neural Networks · Physics 2009-10-31 Xiaoyu Xia , Peter G. Wolynes

Relaxation in glasses is often approximated by a stretched-exponential form: $f(t) = A \exp [-(t/\tau)^{\beta}]$. Here, we show that the relaxation in a model of sheared non-Brownian suspensions developed by Cort\'e et al. [Nature Phys. 4,…

Soft Condensed Matter · Physics 2017-02-02 Joseph D. Paulsen , Sidney R. Nagel

We derive an equation for the glass relaxation. In the derivation, the Zwanzig-Mori projection method is not applied explicitly, which makes our equation different from the mode coupling theory. Due to the nonlinearity, it is difficult to…

Disordered Systems and Neural Networks · Physics 2023-02-17 Li Wan