Related papers: Quadrupolar interactions in Pr compounds: PrFe4P12…
Current status is described toward identifying unconventional order parameters in filled skutterudites with unique ordering phenomena. The order parameters in PrFe$_4$P$_{12}$ and PrRu$_4$P$_{12}$ are discussed in relation to associated…
We measured the electrical resistivity, AC magnetic susceptibility, and specific heat of the cubic double perovskite Ba$_2$MgReO$_6$ under pressure. The application of pressure leads to a gradual increase in the transition temperature to…
We present a theoretical model of the "isostructural" \gamma-\alpha phase transition in Ce which is based on quadrupolar interactions due to coupled charge density fluctuations of 4f electrons and of conduction electrons. Conduction…
The invariant form of the hyperfine interaction between multipolar moments and the nuclear spin is derived, and applied to discuss possibilities to identify the antiferro-octupolar (AFO) moments by NMR experiments. The ordered phase of…
The low-carrier ordered phase below the metal-non-metal transition temperature T_MI ~ 63 K of PrRu4P12 is explored by probing magnetoresistance, magnetic susceptibility, thermoelectric power, and Hall effect on high quality single crystals.…
Characteristics of magnetic transitions in NpTGa$_5$ with T=Co, Ni, Rh are explained in a unified way with use of a crystalline electric field (CEF) model of localized 5$f^4$ electrons. The model takes a CEF doublet and a singlet as local…
We describe a general method to model multicomponent ordered crystals using the phase-field crystal (PFC) formalism. As a test case, a generic B2 compound is investigated. We are able to produce a line of either first-order or second-order…
We present a comprehensive experimental and theoretical study of the pyrochlore Tb$_2$Ge$_2$O$_7$, an exemplary realization of a material whose properties are dominated by competition between magnetic dipolar and electric quadrupolar…
We study the ground state ordering of quadrupolar ordered $S=1$ magnets as a function of spin dilution probability $p$ on the triangular lattice. In sharp contrast to the ordering of $S=1/2$ dipolar N\'eel magnets on percolating clusters,…
Magnetic ordering phenomena in CexPr1-xB6 solid solutions have been studied using both powder and single-crystal neutron diffraction. A variety of magnetic structures are observed depending on temperature and Ce concentration. Over a broad…
Resistivity measurements were performed on Pr$_{1-x}$La$_x$Os$_4$Sb$_{12}$ single crystals at temperatures down to 20 mK and in fields up to 18 T. The results for dilute-Pr samples ($x=0.3$ and 0.67) are consistent with model calculations…
In this article we report on the experimental realization of dimensional crossover phenomena in the chain compound PrBa$_2$Cu$_4$O$_8$ using temperature, high magnetic fields and disorder as independent tuning parameters. In purer crystals…
In the context of perovskite quantum paraelectrics, we study the effects of a quadrupolar interaction $J_q$, in addition to the standard dipolar one $J_d$. We concentrate here on the nonlinear dielectric response $\chi_{P}^{(3)}$, as the…
The crystal structure of the MAPbI$_3$ hybrid perovskite forms an intricate electrostatic puzzle with different ordering patterns of the MA molecules at elevated temperatures. For this perovskite three published model Hamiltonians based on…
TmGa$_{3}$ (AuCu$_3$ structure) undergoes two phase transitions, an antiferroquadrupolar transition at $\sim$ 4.29 K and long-range antiferromagnetic ordering at $\sim$ 4.26 K. Due to the close vicinity of the two phase transitions,…
All symmetry allowed couplings between the 4f^2-electron ground state doublet of trivalent praseodymium in PrRu4P12 and PrFe4P12 and displacements of the phosphorus, iron or ruthenium ions are considered. Two types of displacements can…
A new class of strongly infrared active structures is identified for phase III of compressed molecular H2 by constant-pressure ab initio molecular dynamics and density-functional perturbation calculations. These are planar quadrupolar…
We study a realistic Kondo model for crystal field quartet ground states having magnetic and non-magnetic (quadrupolar) exchange couplings with conduction electrons, using the numerical renormalization group method. We focus on a local…
We present a mean-field calculation of the phase diagram of a simple model of localized moments, in the hexagonal uranium heavy-fermion compounds. The model considers a non-Kramers quadrupolar doublet ground state magnetically coupled with…
It is shown that unconventional nature of superconducting state of PrOs_4Sb_12, a Pr-based heavy electron compound with the filled-Skutterudite structure, can be explained in a unified way by taking into account the structure of the…