Related papers: Transition from molecular complex to quantum solva…
Liquid helium under negative pressures represents a unique possibility for studying nucleation and growth dynamics of cavities at low temperatures down to absolute zero. We analyze the growth dynamics of cavities and determine the…
The rotational transitions of carbon monoxide (CO) are the primary means of investigating the density and velocity structure of the molecular interstellar medium. Here we study the lowest four rotational transitions of CO towards…
An approach to correlated dynamics of quantum nuclei and electrons both in dynamical interaction with external environments is presented. This stochastic quantum molecular dynamics rests on a theorem that establishes a one-to-one…
Precision spectroscopy of simple atomic systems has refined our understanding of the fundamental laws of quantum physics. In particular, helium spectroscopy has played a crucial role in describing two-electron interactions, determining the…
A decrease in the rotational period observed in torsional oscillator measurements was recently taken as a possible indication of a supersolid state of helium. We reexamine this interpretation and note that the decrease in the rotation…
Heavy nuclei exhibit a crossover from vibrational to rotational collectivity as the number of neutrons or protons increases from shell closure towards midshell, but the microscopic description of this crossover has been a major challenge.…
We have studied natural purity $^{4}$He single crystals and polycrystals between 10 and 600 mK using a torsional oscillator with a 2 cm$^{3}$ rigid cell made of sapphire with a smooth geometry. As the temperature was lowered, we observed…
Using an ab-initio molecular dynamics scheme (the Fireball scheme), we determined the equilibrium structure of intermediate size Si_nGe_m (n+m=71) nanoclusters with/without hydrogen passivation on the surface. Due to the strong surface…
Carbon tetrachloride (CCl$_4$) is one of the simplest compounds having a translationally stable monoclinic phase while exhibiting a rich rotational dynamics below 226 K. Recent nuclear quadrupolar resonance (NQR) experiments revealed that…
We discuss the dependence of the phase diagram of a hypothetical isotope of helium with nuclear mass less than 4 atomic mass units. We argue that with decreasing nucleus mass, the temperature of the superfluid phase transition (about 2.2 K…
The changes that vacancies produce in the properties of hcp solid 4He are studied by means of quantum Monte Carlo methods. Our results show that the introduction of vacancies produces significant changes in the behavior of solid 4He, even…
We combine experimental and theoretical approaches to explore excited rotational states of molecules embedded in helium nanodroplets using CS$_2$ and I$_2$ as examples. Laser-induced nonadiabatic molecular alignment is employed to measure…
Recently, the dynamics of quantum systems that involve both unitary evolution and quantum measurements have attracted attention due to the exotic phenomenon of measurement-induced phase transitions. The latter refers to a sudden change in a…
The burn-up for SC56-1472 sample of the natural Oklo reactor zone 3 was calculated using the modern Monte Carlo codes. We reconstructed the neutron spectrum in the core by means of the isotope ratios: $^{147}$Sm/$^{148}$Sm and…
We critically examine the current status of theoretical calculations of the energies, the fine structure, and the isotope shift of the lowest-lying states of helium, searching for unresolved discrepancies with experiments. Calculations are…
Determining the properties of molecules and materials is one of the premier applications of quantum computing. A major question in the field is how to use imperfect near-term quantum computers to solve problems of practical value. Inspired…
Solid helium (3He and 4He) in the hcp and fcc phases has been studied by path-integral Monte Carlo. Simulations were carried out in the isothermal-isobaric (NPT) ensemble at pressures up to 52 GPa. This allows one to study the temperature…
High-precision spectroscopy of simple atomic systems can be used to advance the theory of atomic energy levels but can also serve as a sensitive probe of nuclear charge radii. For this last purpose, we report an improved measurement of the…
The equation of state (EOS) of finite nuclei is constructed in the relativistic Thomas-Fermi theory using the non-linear $\sigma-\omega -\rho$ model. The caloric curves are calculated by confining the nuclei in the freeze-out volume taken…
The quantum simulation of quantum chemistry is a promising application of quantum computers. However, for N molecular orbitals, the $\mathcal{O}(N^4)$ gate complexity of performing Hamiltonian and unitary Coupled Cluster Trotter steps makes…