Related papers: Theoretical study of photon emission from molecula…
Recent experimental advances have made it possible to detect individual quantum jumps in open quantum systems, such as the tunneling of single electrons in nanoscale conductors or the emission of photons from non-classical light sources.…
We study the dc conductance of organic single-molecule contacts in the presence of external electromagnetic radiation (photoconductance). In agreement with previous predictions, we find that the radiation can lead to large enhancements of…
The explicit expressions for a nonresonant tunneling current mediated by the bridging units of the molecular wire embedded between the metallic electrodes, are derived. The specific regimes of the charge transmission controlled by…
Comparison of the measured spectral emission properties of single-crystal Cu(001) and W(111) photocathodes to established photoemission theories reveal evidence for an additional one photon emission process predominantly affecting electron…
Electrical quantum conductors coupled to microwave resonators have in the last decade emerged as a versatile testbed for controllable light-matter interaction on the nanometer scale. Recent experimental progress with high impedance…
We study the transport properties of a long non-uniform quantum wire where the electron-electron interactions and the density vary smoothly at large length scales. We show that these inhomogeneities lead to a finite resistivity of the wire,…
A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…
The conductance of a contact, having a radius smaller than the Fermi wave length, on the surface of a thin metal film is investigated theoretically. It is shown that quantization of the electron energy spectrum in the film leads to a…
The quasistatic electric current density of fermions in the presence of an external electric field is determined through the utilization of a time-ordered Schwinger propagator. The study encompasses the necessary conditions for establishing…
A numerical modeling of the radiation emitted from a Luminescent dye embedded in a finite one-dimensional photonic crystal is presented. The Photonic Band Structure and the Photonic Density of States are derived using classical…
Here we study incoherent transport through molecular wire treated as a linear chain of absorbers, where the phase-breaking processes are modeled by the use of imaginary point-like potentials. The calculations are performed within a…
If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…
Recent advances in single atom manipulation have made it possible to create "wires" in the form of atomic scale linear structures on a semiconductor surface. If such structures are to be used in future electronic devices, it will be…
We develop a microscopic model to investigate current-induced light emission in single-molecule tunnel junctions, where a two-level system interacts with a plasmonic field. Using the quantum master equation, we explore the transition from…
We present an atomistic theory of electronic transport through single organic molecules that reproduces the important features of the current-voltage characteristics observed in recent experiments. We trace these features to their origin in…
When a thin-film ring with supercurrent is irradiated by coherent microwave field, the field induces coherent oscillations of all the Cooper pairs involved in the supercurrent. The oscillating charged condensate will emit photons with…
We present a rigorous formulation of the time-dependent density functional theory for interacting lattice electrons strongly coupled to cavity photons. We start with an example of one particle on a Hubbard dimer coupled to a single photonic…
We predict that conduction electrons in a semiconductor film containing a centered square array of metal nanowires normal to its plane are bound in quantum states around the central wires, if a positive bias voltage is applied between the…
This thesis investigates the mechanically controlled break junctions, with a particular emphasis on elucidating the behaviour of molecular currents at room temperature. The core of this experimental investigation involves a detailed…
A theory for light-induced current by strong optical pulses in molecular-tunneling junctions is described. We consider a molecular bridge represented by its highest occupied and lowest unoccupied levels, HOMO and LUMO, respectively. We take…