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Flux-grown single crystals of PuPt$_2$In$_7$ are characterized and found to be both non-superconducting and non-magnetic down to 2 K. The Sommerfeld specific heat coefficient of $\sim 250$ mJ/mol K$^2$ indicates heavy fermion behavior. We…

The best p-type skutterudites so far are didymium filled, Fe/Co substituted, Sb-based skutterudites. Substitution at the Sb-sites influences the electronic structure, deforms the Sb4-rings, enhances the scattering of phonons on electrons…

Materials Science · Physics 2017-02-16 G. Rogl , A. Grytsiv , P. Heinrich , E. Bauerb , P. Kumar , N. Peranio , O. Eibl , J. Horky , M. Zehetbauer , P. Rogl

We report specific-heat experiments under the influence of high pressure on a strongly underdoped Co-substituted BaFe2As2 single crystal. This allows us to study the phase diagram of this iron pnictide superconductor with a bulk…

Superconductivity · Physics 2015-06-12 Yan Zheng , Yuxing Wang , Frederic Hardy , Anna E. Böhmer , Thomas Wolf , Christoph Meingast , Rolf Lortz

Based on the interplay of theory and experiment, a large new family of filled group 9 (Co, Rh and Ir) skutterudites is designed and synthesized. The new materials fill the empty cages in the structures of the known binary CoSb3, RhSb3 and…

X-ray diffraction, electrical resistivity, magnetization, specific heat, and thermoelectric power measurements are presented for single crystals of the new filled skutterudite compound {\CeOsAs}, which reveal phenomena that are associated…

Strongly Correlated Electrons · Physics 2009-11-13 R. E. Baumbach , P. C. Ho , T. A. Sayles , M. B. Maple , R. Wawryk , T. Cichorek , A. Pietraszko , Z. Henkie

We studied nanoprecipitates and defects in p-type filled skutterudite CeFe4Sb12 prepared by non-equilibrium melt-spinning plus spark plasma sintering method using transmission electron microscopy. Nanoprecipitates with mostly spherical…

Materials Science · Physics 2015-05-20 Juan Zhou , Qing Jie , Lijun Wu , Ivo Dimitrov , Xun Shi , Qiang Li

Half metallic ferromagnetic compounds (HMF) are intensively explored for their potential in spintronics application. According to theoretical studies, HMF are those materials where the conduction mechanism is due to one type of spin state,…

Materials Science · Physics 2018-09-28 B. Santhosh Kumar P. Manimuthu N. Praveen Shanker , C. Venkateswaran

The optical conductivity [$\sigma(\omega)$] spectra of alkaline-earth-filled skutterudites with the chemical formula $A^{2+}M_{4}$Sb$_{12}$ ($A$ = Sr, Ba, $M$ = Fe, Ru, Os) and a reference material La$^{3+}$Fe$_{4}$Sb$_{12}$ were obtained…

Strongly Correlated Electrons · Physics 2009-11-13 Shin-ichi Kimura , Hojun Im , Takafumi Mizuno , Shota Narazu , Eiichi Matsuoka , Toshiro Takabatake

p-type Ce1.05Fe4Sb12.04 filled skutterudites with much improved thermoelectric properties have been synthesized by rapidly converting nearly amorphous ribbons into crystalline pellets under pressure. It is found that this process greatly…

Materials Science · Physics 2010-07-01 Qing Jie , Juan Zhou , Xun Shi , Ivo K. Dimitrov , Qiang Li

Specific heat, dc- and ac-magnetic susceptibility are reported for a large single crystal of PrOs$_4$Sb$_{12}$ and, after grinding, its powder. The room temperature effective paramagnetic moment of the crystal was consistent with the…

Superconductivity · Physics 2007-06-01 M. E. McBriarty , P. Kumar , G. R. Stewart , B. Andraka

We report measurements of the London penetration depth $\Delta\lambda(T)$ and the electronic specific heat $C_e(T)$ on high-quality single crystals of the filled-skutterudite superconductor PrPt$_4$Ge$_{12}$ ($T_c\simeq$8K). Both quantities…

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is…

Strongly Correlated Electrons · Physics 2009-11-10 C. H. Lee , H. Matsuhata , H. Yamaguchi , C. Sekine , K. Kihou , T. Suzuki , T. Noro , I. Shirotani

We report synthesis and superconductivity at 3.7K in PrO0.5F0.5BiS2. The newly discovered material belongs to the layered sulfide based REO0.5F0.5BiS2 compounds having ZrCuSiAs type structure. The bulk polycrystalline compound is…

Superconductivity · Physics 2013-03-08 Rajveer Jha , Anuj Kumar , Shiva Kumar Singh , V. P. S. Awana

Using finite-temperature phonon calculations and machine-learning methods, we calculate the mechanical stability of about 400 semiconducting oxides and fluorides with cubic perovskite structures at 0 K, 300 K and 1000 K. We find 92…

Materials Science · Physics 2017-02-10 Ambroise van Roekeghem , Jesús Carrete , Corey Oses , Stefano Curtarolo , Natalio Mingo

CeIrIn5 is a member of a new family of heavy-fermion compounds and has a Sommerfeld specific heat coefficient of 720 mJ/mol-K2. It exhibits a bulk, thermodynamic transition to a superconducting state at Tc=0.40 K, below which the specific…

Strongly Correlated Electrons · Physics 2009-10-31 C. Petrovic , R. Movshovich , M. Jaime , P. G. Pagliuso , M. F. Hundley , J. L. Sarrao , Z. Fisk , J. D. Thompson

We present scanning tunnelling spectroscopy measurements on the heavy fermion superconductor PrOs$_4$Sb$_{12}$. Our results show that the superconducting gap opens over a large part of the Fermi surface. The deviations from isotropic BCS…

Superconductivity · Physics 2009-11-10 H. Suderow , S. Vieira , J. D. Strand , S. Bud'ko , P. C. Canfield

The compound Ce3Co4Sn13 is an extremely heavy cubic heavy fermion system with a low temperature electronic specific heat of order ~4 J/mol-K2. If the compound is nonmagnetic, it would be one of the heaviest nonmagnetic Ce-based heavy…

Strongly Correlated Electrons · Physics 2009-11-11 A. D. Christianson , J. S. Gardner , H. J. Kang , J. -H. Chung , S. Bobev , J. L. Sarrao , J. M. Lawrence

We report on a new state of matter manifested by strongly correlated Fermi systems including various heavy-fermion (HF) metals, two-dimensional quantum liquids such as $\rm ^3He$ films, certain quasicrystals, and systems behaving as quantum…

PrCo$_2$Ga$_8$ is an orthorhombic quasi-skutterudite type compound which crystallizes in the CaCo$_2$Al$_8$ structure type, with space group $Pbam$ (No. 55). The Pr$^{3+}$ ion has a site symmetry of $C_s$ which predicts a crystal electric…

Strongly Correlated Electrons · Physics 2019-04-02 Michael O. Ogunbunmi , Buyisiwe M. Sondezi , Harikrishnan S. Nair , André M. Strydom

A technique for measuring the electrical resistivity and absolute thermopower is presented for pressures up to 30 GPa, temperatures down to 25 mK and magnetic fields up to 10 T. With the examples of CeCu2Ge2 and CeCu2Si2 we focus on the…

Strongly Correlated Electrons · Physics 2007-05-23 D. Jaccard , E. Vargoz , K. Alami-Yadri , H. Wilhelm
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