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We report on muon spin relaxation measurements of the 4f^2-based heavy-fermion superconductor filled-skutterudite PrOs4Sb12. The results reveal the spontaneous appearance of static internal magnetic fields below the superconducting…

Superconductivity · Physics 2009-11-10 Y. Aoki , A. Tsuchiya , T. Kanayama , S. R. Saha , H. Sugawara , H. Sato , W. Higemoto , A. Koda , K. Ohishi , K. Nishiyama , R. Kadono

We report $^{121,123}$Sb nuclear quadrupole resonance (NQR) measurements in the filled-skutterudite superconductor PrOs$_4$Sb$_{12}$ in the temperature range of 0.05-30 K. The electric field gradients (EFG), $V_{zz}$ and $V_{xx}-V_{yy}$, at…

Strongly Correlated Electrons · Physics 2009-11-11 Hideki Tou , Masahiro Doi , Masafumi Sera , Mamoru Yogi , Hitoshi Sugawara , Ryousuke Shiina , Hideyuki Sato

MHz conductivity, torque magnetometer and magnetization measurements are reported on single crystals of CeOs$_4$Sb$_{12}$ and NdOs$_4$Sb$_{12}$ using temperatures down to 0.5~K and magnetic fields of up to 60~tesla. The field-orientation…

We report a study of the superconducting and normal-state properties of the filled-skutterudite system PrPt$_{4}$Ge$_{12-x}$Sb$_x$. Polycrystalline samples with Sb concentrations up to $x =$ 5 were synthesized and investigated by means of…

Superconductivity · Physics 2016-03-09 I. Jeon , K. Huang , D. Yazici , N. Kanchanavatee , B. D. White , P. -C. Ho , S. Jang , N. Pouse , M. B. Maple

We report on Sb nuclear-quadrupole-resonance (NQR) study in filled-skutterudite compounds (Pr_1-xLa_x)Os_4Sb_12. The Sb-NQR spectra have split into two sets, arising from different Sb_12 cages containing either Pr or La, which enables us to…

Superconductivity · Physics 2015-06-25 M. Yogi , T. Nagai , Y. Imamura , H. Mukuda , Y. Kitaoka , D. Kikuchi , H. Sugawara , Y. Aoki , H. Sato , H. Harima

First principles calculations are used to investigate the band structure and the transport related properties of unfilled and filled 4d skutterudite antimonides. The calculations show that, while RhSb3 and p-type La(Rh,Ru)4Sb12 are…

Materials Science · Physics 2009-10-31 Marco Fornari , David J. Singh

To get insight into the electronic properties of PrFe4P12 skutterudite, band electronic structure calculations, Total and Projected Density of States, Crystal Orbital Overlap Population and Mulliken Population Analysis were performed. The…

Computational Physics · Physics 2009-11-10 Donald H. Galvan

The filled skutterudite superconductor PrPt4Ge12 was studied in muon-spin rotation (muSR), specific heat, and electrical resistivity experiments. The continuous increase of the superfluid density with decreasing temperature and the…

Superconductivity · Physics 2015-05-13 A. Maisuradze , M. Nicklas , R. Gumeniuk , C. Baines , W. Schnelle , H. Rosner , A. Leithe-Jasper , Yu. Grin , R. Khasanov

The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

Strongly Correlated Electrons · Physics 2009-11-11 Annamaria Kiss , Yoshio Kuramoto

The structural, elastic, thermodynamic and thermoelectric characteristics of the $\textrm{CeIr}_\textrm{4} \textrm{P}_\textrm{12}$ skutterudite have been predicted for the first time by applying density functional theory and the…

Materials Science · Physics 2025-04-01 M. Bouchenaki , L. I. Karaouzène , B. N. Brahmi , M. Kaid Slimane

Characteristics of hybridization and multipole orders of $4f$-electrons in Pr skutterudites are explained in terms of a pseudo-quartet composed of crystalline electric field (CEF) singlet and the triplet. It is shown that the contrasting…

Strongly Correlated Electrons · Physics 2015-06-25 Yoshio Kuramoto , Annamaria Kiss , Junya Otsuki , Hiroaki Kusunose

The two superconducting phases recently discovered in skutterudite PrOs4Sb12 are discussed by using the phenomenological Ginzburg-Landau theory in the cubic (tetrahedral) crystal symmetry T_h. Building on experimental imput coming from the…

Superconductivity · Physics 2009-11-07 Jun Goryo

We have investigated the de Haas-van Alphen effect in the Pr-based heavy fermion superconductor PrOs$_4$Sb$_{12}$.The topology of Fermi surface is close to the reference compound LaOs$_4$Sb$_{12}$ and well explained by the band structure…

Strongly Correlated Electrons · Physics 2009-11-07 H. Sugawara , S. Osaki , S. R. Saha , Y. Aoki , H. Sato , Y. Inada , H. Shishido , R. Settai , Y. Onuki , H. Harima , K. Oikawa

We investigated the magnetic phase diagram of the first Pr-based heavy fermion superconductor PrOs4Sb12 by means of high-resolution dc magnetization measurements in low temperatures down to 0.06K. The temperature dependence of the…

Superconductivity · Physics 2009-11-10 T. Tayama , T. Sakakibara , H. Sugawara , Y. Aoki , H. Sato

The spin polarization of ferromagnetic alkali-metal iron antimonides KFe4Sb12 and NaFe4Sb12 is studied by point-contact Andreev reflection using superconducting Nb and Pb tips. From these measurements an intrinsic transport spin…

We propose a model of nodal order parameters for the superconducting A and B - phase of skutterudite PrOs_4Sb_{12} and discuss the associated angular dependent magnetothermal conductivity at low temperatures. The model for the hybrid gap…

Superconductivity · Physics 2009-11-07 K. Maki , H. Won , P. Thalmeier , Q. Yuan , K. Izawa , Y. Matsuda

We use neutron scattering to study the Pr$^{3+}$ crystalline electric field (CEF) excitations in the filled skutterudite PrOs$_4$As$_{12}$. By comparing the observed levels and their strengths under neutron excitation with the theoretical…

Strongly Correlated Electrons · Physics 2008-10-22 Songxue Chi , Pengcheng Dai , T. Barnes , H. J. Kang , J. W. Lynn , R. Bewley , F. Ye , M. B. Maple , Z. Henkie , A. Pietraszko

Specific heat $C(T)$ measurements were made on single crystals of the superconducting filled skutterudite series Pr(Os$_{1-x}$Ru$_x$)$_4$Sb$_{12}$ down to 0.6 K. Crystalline electric field fits in the normal state produced parameters which…

Superconductivity · Physics 2009-11-10 N. A. Frederick , T. A. Sayles , M. B. Maple

Infrared reflectance spectroscopy measurements were made on four members of the MFe_4P_12 family of filled skutterudites, with M=La, Th, Ce and U. In progressing from M=La to U the system undergoes a metal-insulator transition. It is shown…

Strongly Correlated Electrons · Physics 2009-10-31 S. V. Dordevic , N. R. Dilley , E. D. Bauer , D. N. Basov , M. B. Maple , L. Degiorgi

We have performed $^{139}$La,$^{31}$P-NMR studies on a filled skutterudite superconductor LaFe$_{4}$P$_{12}$ with a critical temperature $T_c=4.1$ K. In the normal state, the presence of antiferromagnetic (AFM) fluctuations at finite wave…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Nakai , K. Ishida , D. Kikuchi , H. Sugawara , H. Sato