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Recent theories predict that when a supercooled liquid approaches the glass transition, particle clusters with a special "amorphous order" nucleate within the liquid, which lead to static correlations dictating the dramatic slowdown of…

Soft Condensed Matter · Physics 2016-03-04 Bo Zhang , Xiang Cheng

We combine the hyper-netted chain approximation of liquid state theory with the mode-coupling theory of the glass transition to analyze the structure and dynamics of soft spheres interacting via harmonic repulsion. We determine the locus of…

Statistical Mechanics · Physics 2010-03-29 Ludovic Berthier , Elijah Flenner , Hugo Jacquin , Grzegorz Szamel

We report the combined results of molecular dynamics simulations and theoretical calculations concerning various dynamical arrest transitions in a model system representing a dipolar fluid, namely, N (softcore) rigid spheres interacting…

The interplay of slow dynamics and thermodynamic features of dense liquids is studied by examinining how the glass transition changes depending on the presence or absence of Lennard-Jones-like attractions. Quite different thermodynamic…

Materials Science · Physics 2009-11-13 Th. Voigtmann

The synergetic approach proposed here is based on characteristic instability of chemical bonding in the form of the bond wave considered as the spatiotemporal correlation between the elementary acts of bond exchange. In frames of the model,…

Materials Science · Physics 2024-07-02 Elena A. Chechetkina

The nature of the glass transition is theoretically understood in the mean-field limit of infinite spatial dimensions, but the problem remains totally open in physical dimensions. Nontrivial finite-dimensional fluctuations are hard to…

Statistical Mechanics · Physics 2019-04-05 Ludovic Berthier , Patrick Charbonneau , Andrea Ninarello , Misaki Ozawa , Sho Yaida

We review the Random First Order Transition Theory of the glass transition, emphasizing the experimental tests of the theory. Many distinct phenomena are quantitatively predicted or explained by the theory, both above and below the glass…

Disordered Systems and Neural Networks · Physics 2015-06-25 Vassiliy Lubchenko , P. G. Wolynes

We consider a tracer particle on a lattice in the presence of immobile obstacles. Starting from equilibrium, a force pulling on the particle is switched on, driving the system to a new stationary state. We solve for the complete transient…

Soft Condensed Matter · Physics 2017-01-04 Sebastian Leitmann , Thomas Franosch

In a preceding paper, Mukhopadhyay and I studied the diffusive motion of a tagged molecule in a heterogeneous glass-forming liquid at temperatures just above a glass transition. Among other features of this system, we postulated a relation…

Statistical Mechanics · Physics 2009-11-13 J. S. Langer

The mean-square displacement (MSD) was measured by neutron scattering at various temperatures and pressures for a number of molecular glass-forming liquids. The MSD is invariant along the glass-transition line at the pressure studied, thus…

Soft Condensed Matter · Physics 2012-03-27 K. Niss , C. Dalle-Ferrier , B. Frick , D. Russo , J. Dyre , C. Alba-Simionesco

Within the mode-coupling theory for ideal glass-transitions, the mean-squared displacement and the correlation function for density fluctuations are evaluated for a colloidal liquid of particles interacting with a square-well potential for…

Soft Condensed Matter · Physics 2007-05-23 M. Sperl

Understanding glass formation is a challenge because the existence of a true glass state, distinct from liquid and solid, remains elusive: Glasses are liquids that have become too viscous to flow. An old idea, as yet unproven…

We study the static as well as the glassy or dynamical transition in the mean-field $p$-state Potts glass. By numerical solution of the saddle point equations we investigate the static and the dynamical transition for all values of $p$ in…

Condensed Matter · Physics 2007-05-23 Emilio de Santis , Giorgio Parisi , Felix Ritort

We review a theoretical perspective of the dynamics of glass forming liquids and the glass transition. It is a perspective we have developed with our collaborators during this decade. It is based upon the structure of trajectory space. This…

Soft Condensed Matter · Physics 2010-04-20 David Chandler , Juan P. Garrahan

Metallic glasses possess outstanding mechanical and physical properties, making them promising candidates for advanced structural and functional applications; however, the lack of understanding and control over their glass transition and…

Soft Condensed Matter · Physics 2025-06-04 Wei Chu , Zheng Wang , Christopher Ness , Konrad Samwer , Alessio Zaccone , Lina Hu

Several theories of the glass transition propose that the structural relaxation time {\tau}{\alpha} is controlled by a growing static length scale {\xi} that is determined by the free energy landscape but not by the local dynamical rules…

Disordered Systems and Neural Networks · Physics 2017-11-15 Matthieu Wyart , Michael E. Cates

Despite decades of research, it remains to be established whether the transformation of a liquid into a glass is fundamentally thermodynamic or dynamic in origin. While observations of growing length scales are consistent with thermodynamic…

Soft Condensed Matter · Physics 2015-06-22 Shreyas Gokhale , K. Hima Nagamanasa , Rajesh Ganapathy , A. K. Sood

We investigate dynamic scaling properties of the two-dimensional gauge glass model for the vortex glass phase in superconductors with quenched disorder. From extensive Monte Carlo simulations we obtain static and dynamic finite size scaling…

Disordered Systems and Neural Networks · Physics 2007-05-23 Marios Nikolaou , Mats Wallin

This paper explores a mathematical technique for deriving dynamical invariants (i.e. constants of motion) in time-dependent gravitational potentials. The method relies on the construction of a canonical transformation that removes the…

Astrophysics of Galaxies · Physics 2015-06-16 Jorge Peñarrubia

We report a detailed experimental study of the structure and dynamics of glassy states in hard spheres with short-range attraction. The system is a suspension of nearly-hard-sphere colloidal particles and non-adsorbing linear polymer which…

Soft Condensed Matter · Physics 2009-11-10 K. N. Pham , S. U. Egelhaaf , P. N. Pusey , W. C. K. Poon