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We report detailed neutron scattering studies on Ba$_2$Cu$_3$O$_4$Cl$_2$. The compound consists of two interpenetrating sublattices of Cu, labeled as Cu$_{\rm A}$ and Cu$_{\rm B}$, each of which forms a square-lattice Heisenberg…

We study the spin-3/2 Heisenberg model including easy-plane and exchange anisotropies in one and two dimensions. In the Ising limit, when the off-diagonal exchange interaction J is zero, the phase diagram in magnetic field is characterized…

Strongly Correlated Electrons · Physics 2011-12-02 Judit Romhanyi , Frank Pollmann , Karlo Penc

The Shastry-Sutherland model, which consists of a set of spin 1/2 dimers on a 2-dimensional square lattice, is simple and soluble, but captures a central theme of condensed matter physics by sitting precariously on the quantum edge between…

Strongly Correlated Electrons · Physics 2012-02-20 S. Haravifard , A. Banerjee , J. C. Lang , G. Srajer , D. M. Silevitch , B. D. Gaulin , H. A. Dabkowska , T. F. Rosenbaum

We have carried out $^{63,65}$Cu NMR spectra measurements in magnetic field up to about 45~T on single crystal of a multiferroic triangular antiferromagnet CuCrO$_2$. The measurements were performed for magnetic fields aligned along the…

Strongly Correlated Electrons · Physics 2016-12-21 Yu. A. Sakhratov , L. E. Svistov , P. L. Kuhns , H. D. Zhou , A. P. Reyes

We report on high-field magnetization, specific-heat and electron spin resonance (ESR) studies of the quasi-two-dimensional spin-1/2 Heisenberg antiferromagnet [Cu(pyz)2(HF2)]PF6. The frequency-field diagram of ESR modes below TN = 4.38 K…

Strongly Correlated Electrons · Physics 2011-03-10 E. Cizmar , S. A. Zvyagin , R. Beyer , M. Uhlarz , M. Ozerov , Y. Skourski , J. L. Manson , J. A. Schlueter , J. Wosnitza

We study the magnetization process of the spin-1/2 antiferromagnetic Heisenberg model on a layered triangular lattice by means of a numerical cluster mean-field method with a scaling scheme (CMF+S). It has been known that antiferromagnetic…

Strongly Correlated Electrons · Physics 2016-06-01 Daisuke Yamamoto , Giacomo Marmorini , Ippei Danshita

The two dimensional Heisenberg model for SrCu_2(BO_3)_2 has the exact dimer ground state which was proven by Shastry and Sutherland almost twenty years ago. The critical value of the quantum phase transition from the dimer state to the…

Strongly Correlated Electrons · Physics 2019-08-17 Shin Miyahara , Kazuo Ueda

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

Materials Science · Physics 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

Multiferroicity in LiCu2O2 single crystals is studied using resonant soft x-ray magnetic scattering, hard x-ray diffraction, heat capacity, magnetic susceptibility, and electrical polarization. Two magnetic transitions are found at 24.6 K…

A spin-1/2 Heisenberg model on honeycomb lattice is investigated by doing triplon analysis and quantum Monte Carlo calculations. This model, inspired by Cu$_2$(pymca)$_3$(ClO$_4$), has three different antiferromagnetic exchange interactions…

Strongly Correlated Electrons · Physics 2021-09-15 Meghadeepa Adhikary , Arnaud Ralko , Brijesh Kumar

Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus…

Strongly Correlated Electrons · Physics 2018-01-19 K. Morita , T. Sugimoto , S. Sota , T. Tohyama

We generalize a class of Heisenberg antiferromagnets in one, two and three dimensions, which have been shown to exhibit magnetization plateaus for spin-1/2. In a certain parameter range of the general model, which is formally defined in D…

Strongly Correlated Electrons · Physics 2009-11-11 V. Ravi Chandra , Naveen Surendran

We investigate the $S=2$ antiferromagnetic quantum spin chain with the exchange and single-ion anisotropies in a magnetic field, using the numerical exact diagonalization of finite-size clusters and the level spectroscopy analysis. It is…

Strongly Correlated Electrons · Physics 2019-08-09 Tôru Sakai , Kiyomi Okamoto , Takashi Tonegawa

RbFe(MoO4)2 is a rare example of a nearly two-dimensional Heisenberg antiferromagnet on a triangular lattice. Magnetic resonance spectra and magnetization curves reveal that the system has a layered spin structure with six magnetic…

Strongly Correlated Electrons · Physics 2015-06-24 L. E. Svistov , A. I. Smirnov , L. A. Prozorova , O. A. Petrenko , L. N. Demianets , A. Ya. Shapiro

LiCu$_3$O$_3$ is a novel 2D S=1/2 antiferromagnet with randomly depleted square lattice. The crystal structure contains two types of square planes with different Cu$^{2+}\rightarrow$ Li$^{+}$ substitution rates (20% and 40%). $^7$Li NMR and…

Strongly Correlated Electrons · Physics 2024-09-09 A. A. Bush , S. K. Gotovko , V. Yu. Ivanov , V. I. Kozlov , E. G. Nikolaev , L. E. Svistov

We study the magnetisation process of the one dimensional spin-1/2 antiferromagnetic Heisenberg model with modulated couplings over j=1,2,3 sites. It turns out that the evolution of magnetisation plateaus depends on j and on the wave number…

Strongly Correlated Electrons · Physics 2016-08-31 R. M. Wiessner , A. Fledderjohann , K. -H. Muetter , M. Karbach

We report the synthesis and characterization of a new quantum magnet [2-[Bis(2-hydroxybenzyl)aminomethyl]pyridine]Ni(II)-trimer (BHAP-Ni3) in single-crystalline form. Our combined experimental and theoretical investigations reveal an exotic…

We report on the microscopic model of the recently synthesized one-dimensional quantum magnet (NO)Cu(NO3)3. Applying density functional theory band structure calculations, we obtain a leading antiferromagnetic exchange coupling J ~ 200 K,…

Strongly Correlated Electrons · Physics 2010-11-15 O. Janson , A. A. Tsirlin , H. Rosner

The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

Strongly Correlated Electrons · Physics 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…