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The properties of semidilute polymer solutions are investigated at equilibrium and under shear flow by mesoscale simulations, which combine molecular dynamics simulations and the multiparticle collision dynamics approach. In semidilute…

Soft Condensed Matter · Physics 2015-03-19 Chien-Cheng Huang , Roland G. Winkler , Godehard Sutmann , Gerhard Gompper

We study theoretically the viscoelastic properties of sheared binary fluids that have strong dynamical asymmetry between the two components. The dynamical asymmetry arises due to asymmetry between the viscoelastic stresses, particularly the…

Soft Condensed Matter · Physics 2009-11-10 Vinay Dwivedi , Rajeev Ahluwalia , Turab Lookman , Avadh Saxena

We investigate the effect of flow kinematics on the extensional viscosity of dilute polymer solutions by conducting dissipative particle dynamics simulations under uniaxial, planar, and biaxial extensional flows. At high extension rates,…

Soft Condensed Matter · Physics 2026-03-13 Yusuke Koide , Takato Ishida , Takashi Uneyama , Yuichi Masubuchi

The emergent fluctuating hydrodynamics of a viscoelastic fluid modeled by the multiparticle collision dynamics (MPC) approach is studied. The fluid is composed of flexible, Gaussian phantom polymers, which interact by local…

Soft Condensed Matter · Physics 2020-01-29 David Toneian , Gerhard Kahl , Gerhard Gompper , Roland G. Winkler

We investigate previously unclarified effects of fluid elasticity on shear-thickening in dilute suspensions in an Oldroyd-B viscoelastic fluid using a novel direct numerical simulation based on the smoothed profile method. Fluid elasticity…

Soft Condensed Matter · Physics 2020-12-21 Yuki Matsuoka , Yasuya Nakayama , Toshihisa Kajiwara

We numerically investigate viscoelastic phase separation in polymer solutions under shear using a time-dependent Ginzburg-Landau model. The gross variables in our model are the polymer volume fraction and a conformation tensor. The latter…

Soft Condensed Matter · Physics 2009-11-10 Tatsuhiro Imaeda , Akira Furukawa , Akira Onuki

The progressive onset of slip at the wall, which corresponds to a slip length increasing with the solicitation time before reaching a plateau, has been investigated for model viscoelastic polymer solutions, allowing one to vary the longest…

The linear viscoelastic response of flexible polymer solutions in the dilute and semidilute unentangled regimes is investigated using Brownian dynamics simulations. The relaxation modulus and dynamic moduli are computed over a wide range of…

Soft Condensed Matter · Physics 2026-04-08 Amit Varakhedkar , P. Sunthar , J. Ravi Prakash

The effect of fluctuating internal viscosity and hydrodynamic interactions on a range of rheological properties of dilute polymer solutions is examined using a finitely extensible dumbbell model for a polymer. Brownian dynamics simulations…

Soft Condensed Matter · Physics 2020-07-03 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

The hydrodynamics of viscoelastic materials (for example polymer melts and solutions) presents interesting and complex phenomena, for example instabilities and turbulent flow at very low Reynolds numbers due to normal stress effects and the…

Soft Condensed Matter · Physics 2007-05-23 Ellak Somfai , Alexander N. Morozov , Wim van Saarloos

We study the viscoelasticity of surface polymer monolayers by measuring the dynamics of thermal concentration fluctuations with surface light scattering. For various systems of proteins and synthetic polymers we find a semi-dilute regime in…

Soft Condensed Matter · Physics 2009-11-10 Pietro Cicuta , Ian Hopkinson

Two distinct effects that polymers exhibit are shear thinning and viscoelasticity. The shear thinning effect is important as the polymers used in chemical enhanced oil recovery usually have this property. We propose a novel approach to…

Fluid Dynamics · Physics 2023-05-10 Prabir Daripa , Rohit Mishra

The tumbling dynamics of individual polymers in semidilute solution is studied by large-scale non-equilibrium mesoscale hydrodynamic simulations. We find that the tumbling time is equal to the non-equilibrium relaxation time of the polymer…

Soft Condensed Matter · Physics 2011-03-21 C. -C. Huang , G. Sutmann , G. Gompper , R. G. Winkler

The influence of an external flow on the relaxation dynamics of a single polymer is investigated theoretically and numerically. We show that a pronounced dynamical slowdown occurs in the vicinity of the coil-stretch transition, especially…

Chaotic Dynamics · Physics 2007-05-23 Antonio Celani , Alberto Puliafito , Dario Vincenzi

Shear flow is known to induce huge density fluctuations in otherwise clear and uniform polymer solutions. This effect is rooted in the elasticity of the entangled polymer network, and can span distances over a thousand chains wide. It has…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas

Buckling induced by viscous flow changes the shape of sheet-like nanomaterial particles suspended in liquids. This instability at the particle scale affects collective behavior of suspension flows and has many technological and biological…

Fluid Dynamics · Physics 2023-03-10 Hugo Perrin , Heng Li , Lorenzo Botto

The development of a coherent conceptual basis for the treatment of non-linear microscopic phenomena, such as, hydrodynamic interaction, finite extensibility, excluded volume and internal viscosity, in molecular theories of dilute polymer…

Statistical Mechanics · Physics 2021-07-16 J. Ravi Prakash

Transient dynamics in viscoelastic fluids exhibits notable difference with their Newtonian counterpart. In this work we study the changes in the formation and decay of vortex of viscoelastic fluids due to degradation caused by shear stress.…

Fluid Dynamics · Physics 2023-12-29 Renzo Guido , Luis G. Sarasua , Arturo C. Marti

The non-equilibrium structural and dynamical properties of semiflexible polymers confined to two dimensions are investigated by molecular dynamics simulations. Three different scenarios are considered: The force-extension relation of…

Soft Condensed Matter · Physics 2013-01-08 A. Lamura , R. G. Winkler

The nonequilibrium structural and dynamical properties of semiflexible active polar polymers subject to linear flow are studied by numerical simulations. Filaments are confined in two dimensions and immersed in a fluid described by the…

Soft Condensed Matter · Physics 2026-04-23 A. Lamura , R. G. Winkler
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