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The dielectric properties of CaCu3Ti4O12, a material showing colossal values of the dielectric constant, were investigated in a broad temperature and frequency range extending up to 1.3 GHz. A detailed equivalent circuit analysis of the…

Materials Science · Physics 2009-11-10 P. Lunkenheimer , R. Fichtl , S. G. Ebbinghaus , A. Loidl

In the present work we demonstrate that in addition to the well-known colossal-dielectric-constant material CaCu3Ti4O12 also various members of the series Ln2/3Cu3Ti4O12 with Ln = La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er and Tm, exhibit…

Materials Science · Physics 2010-03-25 J. Sebald , S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , S. Riegg , A. Reller , A. Loidl

Many transition-metal oxides show very large ("colossal") magnitudes of the dielectric constant and thus have immense potential for applications in modern microelectronics and for the development of new capacitance-based energy-storage…

Strongly Correlated Electrons · Physics 2015-03-13 P. Lunkenheimer , S. Krohns , S. Riegg , S. G. Ebbinghaus , A. Reller , A. Loidl

The cubic perovskite-related ceramic CaCu3Ti4O12 has a very high static dielectric constant ~10000 at room temperature (RT), which drops to about 100 below about 100 K. Substituting Cd for Ca reduces the RT value of the dielectric constant…

Strongly Correlated Electrons · Physics 2007-05-23 C. C. Homes , T. Vogt , S. M. Shapiro , W. Si , S. Wakimoto , M. A. Subramanian

A thorough investigation of the dielectric properties of Cu2Ta4O12, a material crystallizing in a pseudo-cubic, perovskite-derived structure is presented. We measured the dielectric constant and conductivity of single crystals in an…

Materials Science · Physics 2009-11-10 B. Renner , P. Lunkenheimer , M. Schetter , A. Loidl , A. Reller , S. G. Ebbinghaus

We present dielectric measurements of the colossal dielectric constant material CaCu3Ti4O12 extending up to 1.3 GHz also covering so far only rarely investigated single crystalline samples. Special emphasis is put on the second relaxation…

Materials Science · Physics 2007-07-19 S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

Low-temperature specific-heat study has been performed on the insulating giant dielectric constant material CaCu3Ti4O12 and two related compounds, Bi2/3Cu3Ti4O12 and La0.5Na0.5Cu3Ti4O12, from 0.6 to 10 K. From analyzing the specific heat…

Materials Science · Physics 2009-11-13 C. P. Sun , Jianjun Liu , J. -Y. Lin , Chun-gang Duan , W. N. Mei , H. D. Yang

In the present work the authors report results of broadband dielectric spectroscopy on various samples of CaCu3Ti4O12, including so far only rarely investigated single crystalline material. The measurements extend up to 1.3 GHz, covering…

Materials Science · Physics 2008-09-03 S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

The large, temperature-independent, low-frequency dielectric constant recently observed in single-crystal CaCu{3}Ti{4}O{12} is most plausibly interpreted as arising from spatial inhomogenities of its local dielectric response. Probable…

Materials Science · Physics 2009-11-10 Morrel H. Cohen , J. B. Neaton , Lixin He , David Vanderbilt

Recently, materials exhibiting colossal dielectric constant ($CDC$) have attracted significant attention because of their high dielectric constant and potential applications in electronic devices, such as high dielectric capacitors,…

Materials Science · Physics 2013-09-19 K. Liu , X. Y. Zhang

Structural and electronic properties of CaCu{3}Ti{4}O{12} have been calculated using density-functional theory within the local spin-density approximation. After an analysis of structural stability, zone-center optical phonon frequencies…

Materials Science · Physics 2009-11-07 Lixin He , J. B. Neaton , Morrel H. Cohen , David Vanderbilt , C. C. Homes

The search for new materials with extremely high ("colossal") dielectric constants, required for future electronics, is one of the most active fields of modern materials science. However, the applicability of the colossal-epsilon'…

Materials Science · Physics 2009-03-24 S. Krohns , P. Lunkenheimer , Ch. Kant , A. V. Pronin , H. B. Brom , A. A. Nugroho , M. Diantoro , A. Loidl

Frequency dependence of the dielectric constant of complex perovskite oxide Ba(1-x)La(x)Ti(1-x)Cr(x)O3 (BLTC) ceramics with the composition ratio 0.4<= x <= 0.7 is precisely measured in the temperature range from 20 K to 300 K, and the…

Materials Science · Physics 2007-05-23 Mamoru Fukunaga , Yoshiaki Uesu

Structural, vibrational, and lattice dielectric properties of CdCu{3}Ti{4}O{12} are studied using density-functional theory within the local spin-density approximation, and the results are compared with those computed previously for…

Materials Science · Physics 2009-11-07 Lixin He , J. B. Neaton , David Vanderbilt , Morrel H. Cohen

Using transmission electron microscopy (TEM) we studied CaCu3Ti4O12, an intriguing material that exhibits a huge dielectric response, up to kilohertz frequencies, over a wide range of temperature. Neither in single crystals, nor in…

Materials Science · Physics 2009-11-10 L. Wu , Y. Zhu , S. Park , S. Shapiro , G. Shirane , J. Tafto

Materials with high dielectric constant are in great demand for the miniaturization of electronic devices. More specifically, high dielectric constant polymer-ceramic composites are useful for embedded capacitor applications. A composite…

Materials Science · Physics 2013-01-18 P. Thomas , R. S. Ernest Ravindran , K. B. R. Varma

We report on phonon properties and electronic transitions in CaCu3Ti4O12, a material which reveals a colossal dielectric constant at room temperature without any ferroelectric transition. The results of far- and mid-infrared measurements…

Strongly Correlated Electrons · Physics 2008-01-28 Ch. Kant , T. Rudolf , F. Mayr , S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , A. Loidl

We have measured dielectric properties of Ca$_{1+x}$Cu$_{3-x}$Ti$_4$O$_{12}$ ($x$ = 0, 0.1, 0.5, 1, 1.5, 2, 2.9 and 3), and have found that Ca$_2$Cu$_2$Ti$_4$O$_{12}$ (a composite of CaCu$_3$Ti$_4$O$_{12}$ and CaTiO$_3$) exhibits a high…

Materials Science · Physics 2009-11-11 W. Kobayashi , I. Terasaki

Experimental evidence is provided that colossal dielectric constants, epsilon >= 1000, sometimes reported to exist in a broad temperature range, can often be explained by Maxwell-Wagner type contributions of depletion layers at the…

Condensed Matter · Physics 2009-11-07 P. Lunkenheimer , V. Bobnar , A. V. Pronin , A. I. Ritus , A. A. Volkov , A. Loidl

The possibility of obtaining relatively high dielectric constant polymer-ceramic composite by incorporating the giant dielectric constant material, CaCu3Ti4O12 (CCTO) in a Poly(vinylidene fluoride) (PVDF) polymer matrix by melt mixing and…

Materials Science · Physics 2013-01-18 P. Thomasa , K. T. Varughese , K. Dwarakanath , K. B. R. Varma
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